Engineering topics

Aines, Roger D.

Publications and source records attributed to Aines, Roger D..

8 records

DOE OSTI2023

Roads to Removal: Options for Carbon Dioxide Removal in the United States

Our analysis shows it is feasible for the United States to remove a staggering amount of CO 2 from the air—this will be critical to becoming carbon neutral by 2050. Our comprehensive, first-of-its-kind, county-resolution analysis indicates that our country can accomplish this goal by relying on demonstrated technology, natural resources, and workforces we already have. Additionally, ongoing technology development can lower costs, shorten timelines, and deliver new solutions. Our analysis evaluated how we can use forests, cropland soils, and waste biomass, along with purpose-built machines, to get us to net-zero. Further, we considered community impacts and identified locations where certain solutions could be uniquely beneficial or potentially counterproductive. Our findings enable decisionmakers to weigh both opportunities and constraints and to decide what roads to use to meet our national climate goal for net-zero CO 2 emissions.

03 NATURAL GAS↗

DOE OSTI2023

Fabricating structured particles through rapid hardening and tailored collection methods

Fabrication of functional polymer-based particles by crosslinking UV-curable polymer drops in mid-air and collecting crosslinked particles in a solid container, a liquid suspension, or an air flow. The particles can contain different phases in the form or layered structures that contain one to multiple cores, or structures that are blended with dissolved or emulsified smaller domains. A curing system produces ultraviolet rays that are directed onto the particles in the jet stream from one side. A reflector positioned on other side of the jet stream reflects the ultraviolet rays back onto the particles in the jet stream.

Ye, Congwang↗

DOE OSTI2022

Radiocarbon analysis as a method for verifying atmospheric CO 2 uptake during carbon mineralization

Sequestration of atmospheric CO 2 is required to constrain the warming of Earth’s climate. Carbon mineralization refers to the precipitation of carbonate minerals by reaction of CO 2 and Mg- and Ca-rich rocks; if the source of the CO 2 is atmospheric and the precipitated carbonate is protected from subsequent dissolution, this process at sufficient scale may be able to reliably draw down atmospheric greenhouse gas levels. Such reactions occur passively in ultramafic settings and previous work has demonstrated that they actively draw down local CO 2 (g) concentrations. However, a method for unambiguously attributing the sequestered carbon solid product to atmospheric sources is still lacking. Here, we test if radiocarbon can be used to verify that the carbon being incorporated into carbonate minerals during carbon mineralization is atmospheric in origin. Additionally, samples from recently exposed ultramafic sites are analyzed and the results demonstrate the utility of this technique for verifying true atmospheric carbon reduction.

58 GEOSCIENCES↗

DOE OSTI2021

Fabricating structured particles through rapid hardening and tailored collection methods

Ye, Congwang↗

DOE OSTI2021

Comparative Techno-Economic and Life Cycle Analysis of Water Oxidation and Hydrogen Oxidation at the Anode in a CO 2 Electrolysis to Ethylene System

We compare the economic viability of employing hydrogen oxidation versus water oxidation at the anode of a commercial-scale electrolysis plant that converts CO 2 to ethylene. We vary the electrolyzer capital cost, membrane lifetime, and renewable electricity price to represent a current and future market scenario. We find that anodic hydrogen oxidation with membraneless reactor design can reduce the electrolyzer capital cost by up to 48% and reduce electricity demand by at least 50% with the current underdeveloped electrolyzer market. These capital and operating cost savings could further lead to a lower ethylene production cost from anodic hydrogen oxidation than the anodic water oxidation system with hydrogen supplied at less than $\$6$ kg. In the future scenario with a fully developed electrolyzer market and cheap renewable electricity, we find that the anodic hydrogen oxidation system requires hydrogen cheaper than $0.7/kg to compete with the anodic water oxidation system. Moreover, hydrogen oxidation at the anode enables extremely low cradle-to-gate emission ethylene by utilizing negative emission hydrogen such as biomass gasification with carbon capture and sequestration, ~240% lower than ethylene produced from the wind/solar electricity-driven water oxidation system. Furthermore, this low carbon footprint ethylene can further boost the economic competitiveness for anodic hydrogen oxidation with a future carbon credit market.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Composite 3D-printed reactors for gas absorption, purification, and reaction

A composite material for gas capture, notably CO 2 capture and storage. The composite material includes a mixture of a solid or liquid reactive filler and a gas-permeable polymer such that the reactive filler forms micron-scale domains in the polymer matrix.

Nguyen, Du T.↗

DOE OSTI2021

Separation of a target substance from a fluid or mixture using encapsulated sorbents

Method and apparatus for separating a target substance from a fluid or mixture. Capsules having a coating and stripping solvents encapsulated in the capsules are provided. The coating is permeable to the target substance. The capsules having a coating and stripping solvents encapsulated in the capsules are exposed to the fluid or mixture. The target substance migrates through the coating and is taken up by the stripping solvents. The target substance is separated from the fluid or mixture by driving off the target substance from the capsules.

Aines, Roger D.↗

DOE OSTI2021

Transport Cost for Carbon Removal Projects With Biomass and CO2 Storage

Strategies to remove carbon from the atmosphere are needed to meet global climate goals. Promising strategies include the conversion of waste biomass to hydrogen, methane, liquid fuels, or electricity coupled with CO 2 capture and storage (CCS). A key challenge for these projects is the need to connect geographically dispersed biomass supplies with geologic storage sites by either transporting biomass or CO 2 . We assess the cost of transport for biomass conversion projects with CCS using publicly available cost data for trucking, rail, and CO 2 pipelines in the United States. We find that for large projects (order of 1 Mt/yr CO 2 or greater), CO 2 by pipeline is the lowest cost option. However, for projects that send most of the biomass carbon to storage, such as gasification to hydrogen or electricity production, biomass by rail is a competitive option. For smaller projects and lower fractions of carbon sent to storage, such as for pyrolysis to liquid fuels, CO 2 by rail is the lowest cost option. Assessing three plausible example projects in the United States, we estimate that total transport costs range from $24/t-CO 2 stored for a gasification to hydrogen project traversing 670 km to $\$ 36$/t for a gasification to renewable natural gas project traversing 530 km. In general, if developers have flexibility in choosing transport mode and project type, biomass sources and storage sites can be connected across hundreds of kilometers for transport costs in the range of $20-40/t-CO 2 stored. Truck and rail are often viable modes when pipelines cannot be constructed. Distances of 1,000 km or more can be connected in the same cost range when shared CO 2 pipelines are employed.

09 BIOMASS FUELS↗