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NASA NTRS2016

A Pervasive Role for Biomass Burning in Tropical High Ozonelow Water Structures

Air parcels with mixing ratios of high O3 and low H2O (HOLW) are common features in the tropical western Pacific (TWP) mid-troposphere (300-700 hPa). Here, using data collected during aircraft sampling of the TWP in winter 2014, we find strong, positive correlations of O3 with multiple biomass burning tracers in these HOLW structures. Ozone levels in these structures are about a factor of three larger than background. Models, satellite data and aircraft observations are used to show fires in tropical Africa and Southeast Asia are the dominant source of high O3 and that low H2O results from large-scale descent within the tropical troposphere. Previous explanations that attribute HOLW structures to transport from the stratosphere or mid-latitude troposphere are inconsistent with our observations. This study suggest a larger role for biomass burning in the radiative forcing of climate in the remote TWP than is commonly appreciated.

Satellite data↗

NASA NTRS2014

A Method for Obtaining High Time and Spatial Resolution Convective Cloud Top Data for the TTL

A method for obtaining high time and spatial resolution convective cloud top data for the TTL Leonhard Pfister, Eric Jensen, Rei Ueyama, Eliot Atlas, and Maria Navarro Convective systems in the tropics have a maximum in the cloud top altitude distribution of about 13.5 km. However, there is a significant tail to this distribution -- a few percent reach the cold point tropopause (CPT) at 16.5 km, and there has been clear evidence of convective mass deposited as high as 19 km in the tropics. The region between 13.5 km and the cold point tropopause is transitional, between the free tropical troposphere where convective mixing dominates, and the stratosphere where slow upward ascent dominates. In this region (the Tropical Tropopause Layer), convective injection, slow ascent, and mixing from midlatitudes all have similar time scales. So, even though only a few percent of convective systems reach the CPT, convection is important. Space Based Lidar and cloud radar measurements have yielded information about long term average statistical distributions of cloud altitude as a function of location. However, we also need time-dependent cloud top altitude and cloud top potential temperature information, primarily to understand the water vapor and TTL cloud distributions. This is because the effect of convection depends on the local temperature, and on the subsequent temperature history. Time dependent cloud top information is also needed to understand short-lived tracers because cross-isentropic flow is time and space dependent. This paper presents a method of obtaining time and space dependent convective cloud top theta (and altitude) information using 3-hourly geostationary brightness temperature data, coupled with global 3 -hourly rainfall estimates and temperature analyses. We explore different mixing algorithms to obtain the most reasonable agreement with near-simultaneous observations by cloudsat and calipso. Observations of short-lived tracers from ATTREX, coupled with short-term trajectories are used to test the method's accuracy. An important caveat is the ambiguity of evaluating convective cloud top altitudes under from combined cloudsat and calipso measurements.

cold point tropopause (CPT)↗

NASA NTRS2004

Measurement of Selected Organic Trace Gases During TRACE-P

Major goals of the TRACE-P mission were: 1) to investigate the chemical composition of radiatively important gases, aerosols, and their precursors in the Asian outflow over the western Pacific, and 2) to describe and understand the chemical evolution of the Asian outflow as it is transported and mixed into the global troposphere. The research performed as part of this proposal addressed these major goals with a study of the organic chemical composition of gases in the TRACE-P region. This work was a close collaboration with the Blake/Rowland research group at UC-Irvine, and they have provided a separate report for their funded effort.

Atlas, Elliot↗