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Beausoleil, Geoffrey

Publications and source records attributed to Beausoleil, Geoffrey.

Progress in Fast Modular Reactor Conceptual Design

The Fast Modular Reactor (FMR) is a 100-MW(thermal) gas-cooled fast reactor being developed by General Atomics Electromagnetic System with the goal of developing a FMR for flexible and dispatchable power to the U.S. electricity market in the mid-2030s. The conceptual design aims to develop and verify simplified design features. These include an inert helium gas coolant, pellet-loaded fuel rods, installations with air cooling as ultimate heat sink, and small and passive heat removal systems. The goal is to ensure the development of a safe, maintainable, cost-effective, and distributed nuclear energy-generating station. The baseline technologies selected to achieve this goal are a helium coolant that is an inert gas with no chemical reaction with structural components, not activated, single phase, enabling high-temperature operation and a high thermal efficiency Brayton cycle; conventional uranium dioxide (UO 2 ) fuel, which is the most widely used and well-known fuel material, capable of high burnup (100 MWd/kg) and a long fuel life; and silicon carbide composite (SiGA®) cladding and internal structures that are chemically inert in the helium environment, exceptionally radiation tolerant, and being derisked by accident tolerant fuel technology development. Further, the reactor was specifically designed with passive safety features, including high-temperature in-core materials and a reactor vessel cooling system consisting of cooling panels of naturally circulating water. The passive safety of the core was confirmed for the depressurized loss-of–forced cooling accident, which showed the peak cladding temperature at ~1600°C during the transient, which is below the current design limit of 1800°C. The conceptual design of the FMR has been conducted for the reactor system, vessel system, generator and turbomachine, instrumentation and control, residual heat removal system, plant service system, and containment, as well as pre-application licensing documents.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Designing Nuclear Fuels with a Multi-Principal Element Alloying Approach

Previous research has shown that multi-principal element alloys (MPEAs) using chromium, molybdenum, niobium, tantalum, titanium, vanadium, and zirconium can form stable body-centered-cubic (BCC) structures across a large temperature region (25°C to 1000°C). This is the same crystal structure as γ-uranium (U), which has shown desirable thermal and irradiation behavior in previous alloy fuel research. It is hypothesized then that the MPEA alloying approach can be used to produce a stable BCC uranium-bearing alloy and to retain its stability throughout anticipated operating regimes of power-producing reactors. Candidate elements were assessed using Monte Carlo N-Particle (MCNP) analysis to determine uranium densities necessary to make the alloy an economically viable fuel compared to conventional fuel forms. Following neutronic considerations, materials property databases and empirical predictors were used to determine the compositions with a high potential to form a BCC solid solution alloy. The final four alloys were MoNbTaU 2 , MoNbTiU 2 , NbTaTiU 2 , and NbTaVU 2 , which were cast using arc melting of raw elemental foils and chunks. Characterization of the fabricated alloys included scanning electron microscopy, X-ray diffraction, energy dispersive X-ray spectroscopy, and transmission electron microscopy. The results showed a two-phase system with a U-rich matrix phase surrounding the refractory precipitates. The U phase was found to contain varying concentrations of the alloying elements and was a BCC γ-U phase. These results warrant further research to identify ideal compositions for use as an advanced alloy fuel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A Square Pulse Thermoreflectance Technique for the Measurement of Thermal Properties

We report on a laser-based square pulse thermoreflectance (SPTR) technique for the measurement of thermal properties for a wide range of materials. SPTR adopts the pump-probe thermoreflectance principle to monitor the evolution of local temperature after square pulse excitation. The technique features a compact setup, high spatial resolution, and fast data collection. By comparing the acquired SPTR signals with a continuum heat transfer model, material thermal properties can be obtained. Taking advantage of various spot sizes and modulation frequencies, SPTR can measure both the thermal diffusivity and thermal conductivity of poorly to moderately conductive materials and the thermal conductivity of conductive materials with satisfactory accuracy, with potential to be applied to more conductive materials. The technique was validated on three materials: fused silica, single crystal CaF2 and single crystal nickel (with conductivities ranging from 1 W·m -1 ·K -1 to 100 W·m -1 ·K -1 ) with typical measurement errors of 5 % to 20 %. The leading sources of error have been identified by Monte Carlo simulations, and the primary limitations of SPTR are discussed. The compact, fiberized platform we describe here will allow instruments based on this methodology to be deployed in complex, multi-analytical environments for the type of high-throughput correlative analyses that are key to materials design and discovery.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A Revised Capsule Design for the Accelerated Testing of Advanced Reactor Fuels

Testing of fast reactor fuel is currently challenging because of the thermal neutron spectrum of the Advanced Test Reactor (ATR) and the fact that ATR coolant is substantially below typical temperatures found in liquid metal-cooled fast reactors. Despite these issues, since 2003 the Idaho National Laboratory (INL) has successfully tested a variety of metallic, oxide, and nitride fuels for fast reactor applications. There are, however, opportunities to improve the experiments so that the time required to reach a desired burnup can be reduced, and so the sensitivity of the experiments to fabrication tolerances can be minimized. A revised capsule design exploits the use of smaller diameter rodlets to increase power densities and correspondingly reduce the irradiation time required to reach high burnup. Thermal and nuclear analyses indicate that the time to reach 30at% burnup could be reduced from about 12 years to approximately 2-3 years if the fuel diameter is reduced by one-half and to around 1-2 years if the diameter is reduced by one-third. In addition, reducing fuel diameter improves the radial power distribution in the fuel without the use of cadmium shrouding. This observation opens up the possibility of testing advanced reactor fuel systems in Small I locations in the ATR where there is substantial unused capacity. Although not directly tied to a revised capsule design, post-irradiation furnace testing is proposed to provide time-to-failure data that will be helpful in the benchmarking of fuel performance models and in assessing the performance of new fuel designs relative to more standard fast reactor fuel systems. In this paradigm, ATR irradiation experiments will be viewed more as preparation for furnace testing than as experiments that exist in isolation. An added benefit to furnace testing is that uncertainties in temperatures will significantly be reduced relative to non-instrumented capsules in the ATR. The time and cost in developing this experimental capability is expected to be reduced considerably because of the availability of the blister anneal furnace used by the HPRR program. A key issue in the experiment approach is the potential for non-prototypical rodlet dimensions to influence the observed performance of a given fuel design. For example, a qualitative assessment indicates that the effects of fuel-cladding chemical interactions during furnace testing might be more pronounced in reduced diameter rodlets simply because thinner cladding would be more sensitive to a given depth of fission product penetration. In a traditional empirically-driven approach to fuel qualification, any change from prototypical behavior is undesirable because the resulting data cannot easily be assimilated into a statistical correlation. However, in the current approach, systematic variations in fuel diameter provide the opportunity to benchmark fuel performance models over a wider range of parameter space, which in turn is expected to improve understanding and result in better, more physically based models in the long term.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗