Engineering topics

Beirle, S.

Publications and source records attributed to Beirle, S..

4 records

NASA NTRS2012

The Cabauw Intercomparison Campaign for Nitrogen Dioxide Measuring Instruments (CINDI): Design, Execution, and Early Results

From June to July 2009 more than thirty different in-situ and remote sensing instruments from all over the world participated in the Cabauw Intercomparison campaign for Nitrogen Dioxide measuring Instruments (CINDI). The campaign took place at KNMI's Cabauw Experimental Site for Atmospheric Research (CESAR) in the Netherlands. Its main objectives were to determine the accuracy of state-ofthe- art ground-based measurement techniques for the detection of atmospheric nitrogen dioxide (both in-situ and remote sensing), and to investigate their usability in satellite data validation. The expected outcomes are recommendations regarding the operation and calibration of such instruments, retrieval settings, and observation strategies for the use in ground-based networks for air quality monitoring and satellite data validation. Twenty-four optical spectrometers participated in the campaign, of which twenty-one had the capability to scan different elevation angles consecutively, the so-called Multi-axis DOAS systems, thereby collecting vertical profile information, in particular for nitrogen dioxide and aerosol. Various in-situ samplers and lidar instruments simultaneously characterized the variability of atmospheric trace gases and the physical properties of aerosol particles. A large data set of continuous measurements of these atmospheric constituents has been collected under various meteorological conditions and air pollution levels. Together with the permanent measurement capability at the CESAR site characterizing the meteorological state of the atmosphere, the CINDI campaign provided a comprehensive observational data set of atmospheric constituents in a highly polluted region of the world during summertime. First detailed comparisons performed with the CINDI data show that slant column measurements of NO2, O4 and HCHO with MAX-DOAS agree within 5 to 15%, vertical profiles of NO2 derived from several independent instruments agree within 25% of one another, and MAX-DOAS aerosol optical thickness agrees within 20-30% with AERONET data. For the in-situ NO2 instrument using a molybdenum converter, a bias was found as large as 5 ppbv during day time, when compared to the other in-situ instruments using photolytic converters.

Atmospheric composition↗

NASA NTRS2010

Global Patterns of Lightning Properties Derived by LIS

The Lightning Imaging Sensor LIS aboard the TRMM satellite provides unmatched empirical data of the global lightning distribution (up to approx.35deg S/N) since end of 1997. Climatological flash rate densities derived from LIS are standard references, e.g. for flash rate parameterizations used in GCMs. It is known that flash characteristics are quite variable, and that various quantities (like the flash energy or the NOx production per flash) vary considerably, statistically as well as systematically on regional and seasonal scales. LIS provides information beyond flash counts, in particular radiance and flash footprint. Here we present an analysis of global patterns of various lightning properties derived from LIS, in relation to the number of flashes. These normalized flash characteristics show consistent spatial patterns of regions with "strong" versus regions with "weak" lightning. Most striking is a clear land-ocean contrast, with oceanic flashes being "stronger" than continental flashes. But also over continents, flash strength shows systematic variations. Highest continental values are found over the US, while values over South America and India are quite low. These regional variations cannot be simply parameterized as function of latitude. Information on spatial patterns of mean flash "strength", though rather qualitative up to now, is potentially a valuable input for improving empirical parameterizations based on flash counts (like precipitation or lightning NOx). Further investigation is in progress to come to a more physical and quantitative understanding of the spatial patterns of the different LIS properties. In particular, it has to be checked how far they could be related to established lightning properties (like energy or the fraction of intra-cloud to cloud-to-ground flashes) or to meteorological quantities (like CAPE).

Beirle, S.↗

NASA NTRS2006

Estimating the NO(x) produced by lightning from GOME and NLDN data: A case study in the Gulf of Mexico

Nitrogen oxides (NO(x)=NO+NO2) play an important role in tropospheric chemistry, in particular in catalytic ozone production. Lightning provides a natural source of nitrogen oxides, dominating the production in the tropical upper troposphere, with strong impact on tropospheric ozone and the atmosphere s oxidizing capacity. Recent estimates of lightning produced NO(x) (LNO(x)) are of the order of 5 Tg [N] per year with still high uncertainties in the range of one order of magnitude. The Global Ozone Monitoring Experiment (GOME) on board the ESA-satellite ERS-2 allows the retrieval of tropospheric column densities of NO2 on a global scale. Here we present the GOME NO2 measurement directly over a large convective system over the Gulf of Mexico. Simultaneously, cloud-to-ground (CG) flashes are counted by the U.S. National Lightning Detection Network (NLDN(TradeMark)), and extrapolated to include intracloud (IC)+CG flashes based on a climatological IC:CG ratio derived from NASA s space-based lightning sensors. A series of 14 GOME pixels shows largely enhanced column densities over thick and high clouds, coinciding with strong lightning activity. The enhancements can not be explained by transport of anthropogenic NO(x) and must be due to fresh production of LNO(x). A quantitative analysis, accounting in particular for the visibility of LNO, from satellite, yields a LNO, production of 90 (32-240) moles of NO(x), or 1.3 (0.4-3.4) kg [N], per flash. If simply extrapolated, this corresponds to a global LNO(x) production of 1.7 (0.6-4.7) Tg [N]/yr.

Beirle, S.↗

NASA NTRS2003

Retrieval and Analysis of Stratospheric NO2 from GOME

In this paper we describe the retrieval of stratospheric NO2 from the GOME (Global Ozone Monitoring Experiment) spectrometer. For this retrieval the Differential Optical Absorption Spectroscopy (DOAS) is used and we describe the influence of the instrument s characteristics on this measurement technique. This analysis led to an improved version of the DOAS algorithm resulting in results with lower systematic errors. Subsequently these results were used to separate the tropospheric and stratospheric fraction of the measured NO;! in the atmosphere. This paper is focusing on the annual variations of the stratospheric distribution of nitrogen oxides. For this examination the satellite data from beginning of 1996 to the end of 2001 was used and has been visualized in a plot zonal means versus time of the year, a visualization which proved to be very useful for Ozone. Additionally the so called "Noxon Cliff", a drop of NO2 column densities Noxon measured in 1975-77 while traveling northwards towards the pole in Canada, is shown. Also its southern equivalent could be discovered in the GOME data.

Wenig, M.↗