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Buckley, Robert L.

Publications and source records attributed to Buckley, Robert L..

ALGE Contaminant Transport Model for Emergency Response

Model Description • ALGE is a 3-dimensional hydrodynamic code to predict the movement of a dissolved tracer throughout a water body. • It has been recoded as an emergency response tool. • Can model large-scale bays and estuaries (Chesapeake Bay, Lake Michigan, etc.) • Model includes suspended sediment transport, dissolved and particulate chemical transport, radioactive decay, and dynamic salinity.

Werth, David W.↗

Ultra-low-level measurements of airborne fission products from the Fukushima Daiichi reactor accident using high volume collection systems at Savannah River National Laboratory

For this study, ultra-low-level measurements of radionuclides in air have been conducted at the Savannah River National Laboratory (SRNL) to determine the atmospheric concentration of fission products released following the Fukushima Daiichi reactor accident on March 11, 2011. Air filter samples were acquired from two high-volume collection systems (a traditional filter-based system and an electrostatic precipitator-based system) to monitor airborne radionuclide concentrations in the period covering from 2 weeks to 3 years after the disaster. The world-wide spread of low-level concentrations of airborne fission products from the Fukushima event provided a unique opportunity to demonstrate SRNL's electrostatic particle collection technology and other improvements in environmental monitoring developed at the Savannah River Site (SRS). Detecting and analyzing the release allowed a comprehensive test of SRS systems for monitoring environmental radioactivity. Gamma-ray-emitting fission products ( 131,132 I, 134,136,137 Cs, and 129,132 Te) and cosmogenic isotopes ( 7 Be and 22 Na) in air were detected and quantified by high-resolution gamma-ray spectroscopy at concentrations as low as 0.07 μBq per standard cubic meter (SCM) (50 mBq total 137 Cs), while plutonium content was quantified by thermal ionization mass spectrometry (TIMS) at concentrations as low as 6.5 × 10 –21 g/SCM (3.0 fg 239+240 Pu). Isotope concentrations measured at SRNL from gamma-ray spectroscopy were compared to independent measurements from Chapel Hill, NC, located approximately 370 km (230 mi) NE of SRNL. Meteorological modeling was also used to predict radionuclide transport from the location of release to both measurement locations.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗

Evaluation and Uncertainty of Radioxenon Transport with a Mesoscale Model after the February 2013 Underground Test in North Korea

Abstract The transport of radioxenon released from the February 2013 underground nuclear weapons test in North Korea was analyzed at two receptors—one at the Comprehensive Nuclear Test Ban Treaty site Rn58 in Russia (400 km downwind) and a second at Rn38 in Japan (1000 km downwind). Transport was modeled with two ensembles of mesoscale simulations, one generated with varying initial and lateral boundary conditions taken from the Global Forecasting System uncertainty ensemble, and a second created from different parameterizations and surface conditions. The wind variability was similar for the two ensembles and consistent with observations at 925 mb (1 mb = 1 hPa) but not at the surface. Biases in calculated surface winds and the radioxenon concentration in the ensembles were attributed mainly to poor simulation of the sea breeze at both locations and mountain lee affects at Rn38 in Japan. These wind regimes affected the timing of the surface radioxenon plume at Rn58 and its duration at Rn38. Surface wind variability induced by terrain and land–sea contrast (the sea breeze) also had a significant effect on the surface winds and plume dynamics, including blocking of flow approaching elevated terrain near Vladivostok and the west side of Japan. Increased plume uncertainty was seen at night because of surface wind variability. Measured surface chemical variability was larger than found in the first European Tracer Experiment in central Europe. The study found that horizontal model resolution contributes to uncertainty but not as much as vertical resolution, boundary layer parameterizations, and assimilation of surface meteorological data near the receptor.

54 ENVIRONMENTAL SCIENCES↗