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Burnett, J. L.

Publications and source records attributed to Burnett, J. L..

Cosmogenic activation of silicon

In the production of 3 H, 7 Be, and 22 Na by interactions of cosmic-ray particles with silicon can produce radioactive backgrounds in detectors used to search for rare events. Through controlled irradiation of silicon CCDs and wafers with a neutron beam that mimics the cosmic-ray neutron spectrum, followed by direct counting, we determined that the production rate from cosmic-ray neutrons at sea level is (112 ± 24) atoms/( kg day ) for 3 H, (8.1 ± 1.9) atoms/( kg day ) for 7 Be, and (43.0 ± 7.2) atoms/( kg day ) for 22 Na . Complementing these results with the current best estimates of activation cross sections for cosmic-ray particles other than neutrons, we obtain a total sea-level cosmic-ray production rate of (124 ± 25) atoms/(kg day) for 3 H, (9.4 ± 2.0) atoms/( kg day ) for 7 Be, and (49.6 ± 7.4) atoms/( kg day ) for 22 Na. These measurements will help constrain background estimates and determine the maximum time that silicon-based detectors can remain unshielded during detector fabrication before cosmogenic backgrounds impact the sensitivity of next-generation rare-event searches.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Performance testing of a Compton suppressed coincidence measurements using the Advanced Radionuclide Gamma-spectrOmeter

A Compton-suppressed multidimensional gamma-spectrometer is being developed within the Shallow Underground Laboratory (SUL) at Pacific Northwest National Laboratory (PNNL, USA). This Advanced Radionuclide Gamma-spectrOmeter (ARGO) system consists of two Broad Energy Germanium (BEGe) detectors, surrounded by a 12-detector sodium iodide (NaI) Compton suppression shield, situated inside a low-background lead and copper shield, fitted with a cosmic veto background reduction system. The detector has advanced functionality, including operation in single or combined detector mode, coincidence mode and Compton suppressed coincidence mode. Validation experiments measuring a neutron irradiated natural uranium sample, have demonstrated order of magnitude improvements in gamma detection sensitivity compared to conventional gamma-spectrometry techniques. Importantly this research demonstrates the feasibility of processing and analysing high-multiplicity datasets and the potential for high-sensitivity radionuclide measurements.

ARGO↗

Time sequence gamma-spectrometry of irradiated salt

Persisted Memory Mapping File (MMF) techniques have developed for the processing and analysis of time-stamped list (TLIST) mode data collected from an irradiated salt sample. This is a new technique that is unique to this research and enables additional information to be obtained from a conventional pulse height analysis (PHA) gamma-spectrometry acquisition. A salt sample was irradiated using a DT neutron generator and immediately measured using TLIST acquisition for 1 month to generate a 22 GB data file. MMF techniques were used to process the file without size restrictions at a rate of 388.5 MB minute-1, with instant access to any position within the file, separating the file into a series of time sequenced spectra suitable for PHA analysis. This enabled 14 activation products to be identified at different time intervals (41Ar, 80Br, 80mBr, 47Ca, 34mCl, 38Cl, 42K, 43K, 56Mn, 22Na, 24Na, 85Sr, 87mSr and 69mZn), and 6 radionuclides (80Br, 47Ca, 34mCl, 56Mn, 24Na and 87mSr) to be definitively confirmed based upon their measured half-life. Using this technique, the detection of 47Ca, and in-growth of its 47Sc progeny, was demonstrated as useful for calculating the time since irradiation.

Burnett, Jonathan L.↗