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Canty, Timothy

Publications and source records attributed to Canty, Timothy.

The Impact of MISR-Derived Injection Height Initialization on Wildfire and Volcanic Plume Dispersion in the HYSPLIT Model

The dispersion of particles from wildfires, volcanic eruptions, dust storms, and other aerosol sources can affect air quality and other environmental factors downwind. Aerosol injection height is one source attribute that mediates downwind dispersion, as wind speed and direction can vary dramatically with elevation. Using plume heights derived from space-based, multi-angle imaging, we examine the impact of initializing plumes with satellite-measured vs. nominal (model-calculated or VAAC observations) injection height on the simulated dispersion of six large aerosol plumes. When there are significant differences in nominal vs. satellite-derived particle injection heights, or if one injection height is within the planetary boundary layer (PBL) and the other is above the PBL, differences in simulation results can arise. In the cases studied with significant nominal vs. satellite-derived injection height differences, the NOAA Air Resources Laboratory's Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model tends to represent plume evolution better if the injection height in the model is constrained by hyper-stereo satellite retrievals.

Plume heights↗

Quantifying the Causes of Differences in Tropospheric OH Within Global Models

The hydroxyl radical (OH) is the primary daytime oxidant in the troposphere and provides the main loss mechanism for many pollutants and greenhouse gases, including methane (CH4). Global mean tropospheric OH differs by as much as 80% among various global models, for reasons that are not well understood. We use neural networks (NNs), trained using archived output from eight chemical transport models (CTMs) that participated in the Polar Study using Aircraft, Remote Sensing, Surface Measurements and Models, of Climate, Chemistry, Aerosols and Transport Model Intercomparison Project (POLMIP), to quantify the factors responsible for differences in tropospheric OH and resulting CH4 lifetime (Tau CH4) between these models. Annual average Tau CH4, for loss by OH only, ranges from 8.0 to 11.6 years for the eight POLMIP CTMs. The factors driving these differences were quantified by inputting 3-D chemical fields from one CTM into the trained NN of another CTM. Across all CTMs, the largest mean differences in Tau CH4 (Delta Tau CH4) result from variations in chemical mechanisms (Delta Tau CH4 = 0.46 years), the photolysis frequency (J) of O3 yields O(D-1) (0.31 years), local O3 (0.30 years), and CO (0.23 years). The Delta Tau CH4 due to CTM differences in NO(x) (NO + NO2) is relatively low (0.17 years), although large regional variation in OH between the CTMs is attributed to NO(x). Differences in isoprene and J(NO2) have negligible overall effect on globally averaged tropospheric OH, although the extent of OH variations due to each factor depends on the model being examined. This study demonstrates that NNs can serve as a useful tool for quantifying why tropospheric OH varies between global models, provided that essential chemical fields are archived.

Surface Measurements and Models↗

Emissions Estimation from Satellite Retrievals: a Review of Current Capability

Since the mid-1990s a new generation of Earth-observing satellites has been able to detect tropospheric air pollution at increasingly high spatial and temporal resolution. Most primary emitted species can be measured by one or more of the instruments. This review article addresses the question of how well we can relate the satellite measurements to quantification of primary emissions and what advances are needed to improve the usability of the measurements by U.S. air quality managers. Built on a comprehensive literature review and comprising input by both satellite experts and emission inventory specialists, the review identifies several targets that seem promising: large point sources of NOx and SO2, species that are difficult to measure by other means (NH3 and CH4, for example), area sources that cannot easily be quantified by traditional bottom-up methods (such as unconventional oil and gas extraction, shipping, biomass burning, and biogenic sources), and the temporal variation of emissions (seasonal, diurnal, episodic). Techniques that enhance the usefulness of current retrievals (data assimilation, oversampling, multi-species retrievals, improved vertical profiles, etc.) are discussed. Finally, we point out the value of having new geostationary satellites like GEO-CAPE and TEMPO over North America that could provide measurements at high spatial (few km) and temporal (hourly) resolution.

air quality↗

Denitrification in the Arctic mid-winter 2004/2005 observed by airborne submillimeter radiometry

We present measurements of unusually low mixing ratios of HNO3 in the exceptionally cold Arctic vortex of late-January and early-February 2005. The measurements were obtained by the airborne submillimeter radiometer ASUR during the polar aura validation experiment (PAVE). The distribution of HNO3 inside the vortex reaches minima below 4 ppbv around 22 km altitude and maxima above 13 ppbv around 16 km altitude, with a considerable spatial variability.

measurements↗