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Choi, Mun Y.

Publications and source records attributed to Choi, Mun Y..

Quantitative investigation of sooting dynamics in droplet combustion using an automated image analysis algorithm

This paper reports an image analysis approach using a newly-developed open-source program to extract quantitative measurements of soot volume fraction (SVF) from digital video images of burning n-heptane droplets. The automated program developed in this work can analyze images of fixed and untethered droplets to quantify sooting dynamics. The images analyzed in the program were taken from experiments carried out in the Multi-user Droplet Combustion Apparatus (MDCA) onboard the International Space Station (ISS). In these experiments, video imaging of burning droplets was obtained using backlighting by a laser diode with a wavelength of 653 nm. Here, the light was collimated before it passed through the droplet and soot-containing region, after which the light was then attenuated and projected onto the camera’s sensors. This technique facilitates the measurements of SVF based on the principles of the full field light extinction method (FFLEM). The measurements provide quantitative data that reveal the sooting dynamics of liquid fuels during droplet combustion processes. The analyses of a soot-attenuating image (ISS n-heptane, untethered droplet) at an instant during the burning show that the SVF distribution has a peak at the soot shell location. It then decreases due to soot oxidation when the location is further away from the burning droplet. Regarding temporal effects on the maximum SVF (SVF max ), results show that SVF max first increases after the burning is initiated until a peak value is reached, after which SVF max decreases. The SVF max values identified in this study for n-heptane are quantitatively consistent with previously reported values for fiber-supported droplets and are reached relatively early in the burning history. n-Heptane images are also analyzed to show the effects of initial droplet sizes on the maximum soot volume fraction. Results show that SVF max decreases with increasing initial droplet size, which is consistent with visual observations of less soot formed and dimmer flame brightness as Do increases.

42 ENGINEERING↗

Detailed Results from the Flame Extinguishment Experiment (FLEX) March 2009 to December 2011

The Flame Extinguishment Experiment (FLEX) program is a continuing set of experiments on droplet combustion, performed employing the Multi-User Droplet Combustion Apparatus (MDCA), inside the chamber of the Combustion Integrated Rack (CIR), which is located in the Destiny module of the International Space Station (ISS). This report describes the experimental hardware, the diagnostic equipment, the experimental procedures, and the methods of data analysis for FLEX. It also presents the results of the first 284 tests performed. The intent is not to interpret the experimental results but rather to make them available to the entire scientific community for possible future interpretations.

International Space Station↗

Multi-User Droplet Combustion Apparatus - Flame Extinguishment Experiment

Multi-User Droplet Combustion Apparatus Flame Extinguishment Experiment (MDCA-FLEX) will assess the effectiveness of fire suppressants in microgravity and quantify the effect of different possible crew exploration atmospheres on fire suppression. The goal of this research is to provide definition and direction for large scale fire suppression tests and selection of the fire suppressant for next generation crew exploration vehicles.

Williams, Forman A.↗

Development and applications of laser-induced incandescence

Several NASA-funded investigations focus on soot processes and radiative influences of soot in diffusion flames given their simplicity, practical significance, and potential for theoretical modeling. Among the physical parameters characterizing soot, soot volume fraction, f(sub v), a function of particle size and number density, is often of chief practical interest in these investigations, as this is the geometrical property that directly impacts radiative characteristics and the temperature field of the flame and is basic to understanding soot growth and oxidation processes. Diffusion flames, however, present a number of challenges to the determination of f(sub v) via traditional extinction measurements. Laser-induced incandescence (LII) possesses several advantages compared to line-of-sight extinction techniques for determination of f(sub v). Since LII is not a line-of-sight technique, similar to fluorescence, it possesses geometric versatility allowing spatially resolved measurements of f(sub v) in real time in nonaxisymmetric systems without using deconvolution techniques. The spatial resolution of LII is determined by the detector and imaging magnification used. Neither absorption by polycyclic aromatic hydrocarbons (PAH's) nor scattering contributes to the signal. Temporal capabilities are limited only by the laser pulse and camera gate duration, with measurements having been demonstrated with 10 ns resolution. Because of these advantages, LII should be applicable to a variety of combustion processes involving both homogeneous and heterogeneous phases. Our work has focussed on characterization of the technique as well as exploration of its capabilities and is briefly described.

Vanderwal, Randy L.↗

Theoretical Basis for Estimated Test Times and Conditions for Drop Tower and Space-Based Droplet Burning Experiments With Methanol and N-Heptane

In order to develop an extensive envelope of test conditions for NASA's space-based Droplet Combustion Experiment (DCE) as well those droplet experiments which can be performed using a drop tower, the transient vaporization and combustion of methanol and n-heptane droplets were simulated using a recently developed fully time-dependent, spherically symmetric droplet combustion model. The transient vaporization of methanol and n-heptane was modeled to characterize the instantaneous gas phase composition surrounding the droplet prior to the introduction of an ignition source. The results for methanol/air showed that the entire gas phase surrounding a 2 mm methanol droplet deployed in zero-g .quickly falls outside the lean flammability limit. The gas phase surrounding an identically-sized n-heptane droplet, on the other hand, remains flammable. The combustion of methanol was then modeled considering a detailed gas phase chemical kinetic mechanism (168 steps, 26 species) and the effect of the dissolution of flame-generated water into the liquid droplet. These results were used to determine the critical ignition diameter required to achieve quasi-steady droplet combustion in a given oxidizing environment. For droplet diameters greater than the critical ignition diameter, the model predicted a finite diameter at which the flame would extinguish. These extinction diameters were found to vary significantly with initial droplet diameter. This phenomenon appears to be unique to the transient heat transfer, mass transfer and chemical kinetics of the system and thus has not been reported elsewhere to date. The extinction diameter was also shown to vary significantly with the liquid phase Lewis number since the amount of water present in the droplet at extinction is largely governed by the rate at which water is transported into the droplet via mass diffusion. Finally, the numerical results for n-heptane combustion were obtained using both 2 step and 96 step semi-emperical chemical kinetic mechanisms. Neither mechanism exhibited the variation of extinction diameter with initial diameter.

Marchese, Anthony J.↗

Microgravity combustion of isolated n-decane and n-heptane droplets

This paper presents recent experimental results on n-heptane droplet combustion from a 5.0 second Zero-Gravity Facility. For these experiments, droplet sizes from 1 mm to 1.75 mm were studied, oxygen mole fractions in nitrogen ranged from 12 to 21 percent, and the pressure was varied from 0.25 to 1 atm. Disruptive burning mechanisms were observed in some of the experiments conducted in air environments. However, this behavior was inhibited by reducing the oxygen concentration and/or the system pressure. The above results suggest that combinations of lower oxygen indices and reduced ambient pressures are important to reducing the effects of sooting on droplet vaporization-rates.

Choi, Mun Y.↗

Computational/experimental basis for conducting alkane droplet combustion experiments on space-based-platforms

An analysis is conducted of the requirement for the conduct of spherically symmetric droplet-combustion experiments on space platforms, on the basis of a novel time-dependent computational droplet combustion model that allows the time- and temperature-dependent transport characteristics to be incorporated. While at low oxygen indices the droplet burning extinction becomes a strong function of oxygen index, it becomes a weaker function at higher oxygen index values. The oxygen index that separates these two ranges are dependent on the diluent, being higher for He and lower for N.

Choi, Mun Y.↗

N-Decane Droplet Combustion in the NASA-Lewis 5 Second Zero-Gravity Facility - Results in Test Gas Environments Other than Air

The burning rate of single droplets of n-decane in a microgravity environment of the NASA-Lewis 5 Second Zero-Gravity Facility was investigated as a function of time, together with the flame diameter/droplet diameter ratio, for a wide range of test environments other than normal air conditions, using an engineering model of the flight experiment. Oxygen mole fractions were varied from 18 to 50 percent, the total test chamber pressure was varied from 0.5 to 2 atmospheres, and the initial droplet diameter was varied from 0.98 to 2.41 mm. Measurements showed that the average burning rates for n-decane droplets exhibited the same qualitative trends as are found in two current models. Temporal analysis of the local burning rates showed variable rates of change in local burning as the droplet combustion progressed. The causes and implications of these findings are discussed.

Haggard, John B.↗

Some further observations on droplet combustion characteristics - NASA LeRC-Princeton results

Experimental and numerical studies are reviewed which are designed to examine the effects of droplet/gas motion, product-intermediate absorption, extinction, and sooting on droplet combustion. The experimental work at the NASA-Lewis Research Center involves a 2.2-s droptower for investigating microgravitational effects of droplet combustion over a relatively extended range. The droplet-gas velocities are very low because the spherosymmetrical nature of the major combustion processes produces a quiescent environment. The refined experimental results are combined with numerical modeling based on a technique that is fully transient, comprehensive, and has few empirical simplifications. The combination of techniques improves the present understanding of convection-induced effects, reducing soot formation, and promoting quiescent droplet combustion.

Choi, Mun Y.↗

Observations on a Slow Burning Regime for Hydrocarbon Droplets - N-Heptane/Air Results

Experiments on n-heptane/airdroplet combustion under reduced gravity have served as a benchmark for much of the existing theoretical efforts on the modeling of sphero-synmmetric droplet burning. New experiments conducted in the NASA-Lewis Research Center 2.2 second droptower (at less than 10 exp -5 g) which emphasize the production of sphero-symmetry and low relative droplet/gas convection produce burning rates in air (for about 1 mm droplets) as much as 40-percent lower than the classical result (0.78 sq mm/s). The burning rate is proportional to the measured droplet/gas relative velocity, and the observed functional dependence is much larger than predicted by published convective correlations. New results clearly indicate that the droplet/laboratory velocity does not correspond to the relative droplet/gas velocity. Thus, the convective effects on droplet combustion is not properly characterized by droplet motion alone. Differences in the burning rates are speculated to result from the effects of the accumulated soot as well as the asymmetry (caused by convection) in the temperature and species distributions surrounding the droplet.

Choi, Mun Y.↗

N-Decane-Air Droplet Combustion Experiments in the NASA-Lewis 5 Second Zero-Gravity Facility

The burning of single fuel (n-decane) droplets in a microgravity environment (below 0.00001 of the earth's gravity, achieved in the NASA-Lewis 5-Second Zero-Gravity Facility) was studied, as part of the development of the Droplet Combustion Experiment for eventual operation aboard either the Shuttle middeck or Spacelab. Special attention is given to the combustion equipment used and its operations and performance. Temporal analysis of the local burning rates in these tests showed increasing rates of change in the local burning as droplet combustion progressed. Result point to the need of studying large droplets, with long droplet combustion lifetimes as well as low gas/droplet motion to understand reasons for this unsteadiness.

Haggard, John B.↗