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Chu, William P.

Publications and source records attributed to Chu, William P..

Ground-based microwave monitoring of middle atmosphere ozone: Comparison to lidar and Stratospheric and Gas Experiment 2 satellite observations

A dedicated ground-based microwave radiometer was in operation to monitor the middle atmospheric ozone concentration at Table Mountain Facility (TMF) of the Jet Propulsion Laboratory (JPL), California (34.4 deg N, 117.7 deg W) from July 1989 to June 1992, as a part of the Network for Detection of Stratospheric Change. Ozone profiles from 56 to 0.04 mbar (approximately 20 - 70 km) were retrieved from the microwave data. The focus in this paper is to validate the microwave ozone observations from 56 to 1 mbar by comparing the results from a JPL ground-based lidar located at the same site and from the Stratospheric Aerosol and Gas Experiment 2 (SAGE 2) satellite overpasses within 1000 km of TMF and to examine the ability of these instruments to detect short-term, seasonal, and annual variations in ozone. The profile comparison results show that the mean differences of microwave ozone from lidar and SAGE 2 are about 5% or less and the root-mean-square scatter about the mean is mainly from the precision of the instruments. A correlation analysis of ozone time series suggests highly significant correlations up to 2.4 mbar between lidar and microwave measurements and up to 1 mbar between SAGE 2 and microwave. The short-term and seasonal variation of the ozone profile seen in the microwave measurements is shown to be consistent with the observations of lidar and SAGE 2, and the interannual variation of ozone appears to be detectable within an accuracy of a few percent with the microwave instrument.

Tsou, J. J.

Stratospheric Aerosol and Gas Experiments 1 and 2: Comparisons with ozonesondes

Ozone profiles measured by the Stratospheric Aerosol and Gas Experiments (SAGE) 1 and 2 are compared with ozonesonde profiles at 24 stations over the period extending from 1979 through 1991. Ozonesonde/satellite differences at 21 stations with SAGE 2 overpasses were computed down to 11.5 km in midlatitudes, to 15.5 km in the lower latitudes, and for nine stations with SAGE 1 overpasses down to 15.5 km. The set of individual satellite and ozonesonde profile comparisons most closely colocated in time and space shows mean absolute differences relative to the satellite measurement of 6 +/- 2% for SAGE 2 and 8 +/- 3% for SAGE 1. The ensemble of ozonesonde/satellite differences, when averaged over all altitudes, shows that for SAGE 2, 70% were less than 5%, whereas for SAGE 1, 50% were less than 5%. The best agreement occurred in the altitude region near the ozone density maximum where almost all the relative differences were less than 5%. Most of the statistically significant differences occurred below the ozone maximum down to the tropopause in the region of steepest ozone gradients and typically ranged between 0 and -20%. Correlations between ozone and aerosol extinction in the northern midlatitudes indicate that aerosols had no discernible impact on the ozonesonde/satellite differences and on the SAGE 2 ozone retrieval for the levels of extinction encountered in the lower stratosphere during 1984 to mid-1991.

Veiga, Robert E.

Estimation of solar backscatter ultraviolet albedo using ground-based Umkehr measurements

A retrieval method was developed to estimate the solar backscatter ultraviolet (SBUV) satellite albedo for the ozone profiler wavelengths using ground-based ultraviolet measurements. For the present investigation the Umkehr was used as the ground-based ultraviolet measurement. Simulated SBUV data and Umkehr data theoretically computed from a priori ozone profiles observed by the SAGE II satellite were used to develop the retrieval algorithm and to test its capability. The test indicated that albedos for the SBUV ozone profiler wavelengths should allow estimates to a precision of +/- 5 percent or better, depending on the accuracy of the ultraviolet measurement. Retrievals using actual Umkehr observations were also performed to provide a preliminary look at the magnitude and annual variation of retrieved albedos. A case study was performed, comparing retrieved albedos with SBUV-measured albedos. The SBUV albedo change was seen to be approximately twice as large as the albedo changes estimated by the Umkehr method. Results of the investigation suggest that the method of estimation may be useful for determining the drift rate of the SBUV calibration.

Deluisi, John J.

SAGE 1 data user's guide

A guide for using the data products from the Stratospheric Aerosol and Gas Experiment 1 (SAGE 1) for scientific investigations of stratospheric chemistry related to aerosol, ozone, nitrogen dioxide, dynamics, and climate change is presented. A detailed description of the aerosol profile tape, the ozone profile tape, and the nitrogen dioxide profile tape is included. These tapes are the SAGE 1 data products containing aerosol extinction data and ozone and nitrogen dioxide concentration data for use in the different scientific investigations. Brief descriptions of the instrument operation, data collection, processing, and validation, and some of the scientific analyses that were conducted are also included.

Mcmaster, Leonard R.

Stratospheric ozone profile and total ozone trends derived from the SAGE I and SAGE II data

Global trends in both stratospheric column ozone and as a function of altitude are derived on the basis of SAGE I/II ozone data from the period 1979-1991. A statistical model containing quasi-biennial, seasonal, and semiannual oscillations, a linear component, and a first-order autoregressive noise process was fit to the time series of SAGE I/II monthly zonal mean data. The linear trend in column ozone above 17-km altitude, averaged between 65 deg S and 65 deg N, is -0.30 +/-0.19 percent/yr, or -3.6 percent over the time period February 1979 through April 1991. The data show that the column trend above 17 km is nearly zero in the tropics and increases towards the high latitudes with values of -0.6 percent/yr at 60 deg S and -0.35 percent/yr at 60 deg N. Both these results are in agreement with the recent TOMS results. The profile trend analyses show that the column ozone losses are occurring below 25 km, with most of the loss coming from the region between 17 and 20 km. Negative trend values on the order of -2 percent/yr are found at 17 km in midlatitudes.

Mccormick, M. P.

Stratospheric aerosol and gas experiment II and ROCOZ-A ozone profiles at Natal, Brazil - A basis for comparison with other satellite instruments

Satellite measurements of ozone carried out during the Stratospheric Aerosol and Gas Experiment II (SAGE II) are compared with in situ measurements made by the ROCOZ-A and electrochemical concentration cell ozonesondes at Natal (Brazil) during the Southern Hemisphere autumn of 1985. It was found that the SAGE II values were higher than the ROCOZ-A values by 3.4 percent, with an average absolute difference of 3.8 percent. It is suggested that the differences between the ozone density and mixing ratio results are due to the auxiliary temperature and pressure values for the satellite and in situ instruments.

Barnes, Robert A.

Collecting, analyzing and archiving of ground based infrared solar spectra obtained from several locations

The infrared solar spectrum as observed from the ground under high resolution contains thousands of absorption lines. The majority of these lines are due to compounds that are present in the Earth's atmosphere. Ground based infrared solar spectra contain information concerning the composition of the atmosphere at the time the spectra were obtained. The objective of this program is to record solar spectra from various ground locations, and to analyze and archive these spectra. The analysis consists of determining, for as many of the absorption lines as possible, the molecular species responsible for the absorption, and to verify that current models of infrared transmission match the observed spectra. Archiving is an important part of the program, since a number of the features in the spectra have not been identified. At some later time, when the features are identified, it will be possible to determine the amount of that compound that was present in the atmosphere at the time the spectrum was taken.

Murcray, David G.