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Church, J. A.

Publications and source records attributed to Church, J. A..

Determining the 9 $\mathrm{Be}$($n, γ$) 10 $\mathrm{Be}$ integral cross section at fission neutron energies

The 9 B neutron capture cross section has significant implications for Be materials in the nuclear industry as well as the α process in stellar nucleosynthesis. While the cross section is well constrained at thermal neutron energies, there is a lack of experimental data at higher neutron energies, and the evaluated nuclear data libraries can differ by up to two orders of magnitude. We calculate the 9 Be(n, γ) 10 Be integral cross section at fission neutron energies in an effort to resolve disagreements amongst the nuclear data libraries. Foil irradiation experiments were performed using the Flattop critical assembly at the National Criticality Experiments Research Center with either the highly enriched U or Pu cores, with target foil stacks placed at multiple locations to exploit different neutron energy profiles. Accelerator mass spectrometry was used to measure the 10 Be/ 9 Be ratio in irradiated Be foils, while all other activation products were quantified through gamma spectrometry. The experiments were simulated using the Monte Carlo N-Particle radiation transport code and combined with experimental results to determine the total neutron fluence, while the staysl-pnnl suite and fispact-ii code were used to validate the model and assess the systematic uncertainty. The new 9 Be(n, γ) 10 Be integral cross sections calculated in this work are 26.5 ± 2.2µb at 0.59 ± 0.07 MeV, 24 ± 3 µb at 0.98 ± 0.14 MeV, 21.7 ± 1.3 µb at 1.26 ± 0.11 MeV, 21.8 ± 1.4 µb at 1.32 ± 0.11 MeV, and 18.6 ± 1.1 µb at 1.46 ± 0.13 MeV. These results do not agree with integral cross sections from any of the nuclear data library evaluations. Discrepancies between the new integral cross sections reported here and the nuclear data libraries suggest a more complex cross-section structure in the MeV range which allows for more resonance contributions, and more work is needed to further constrain the evaluated cross sections.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

A High-End Estimate of Sea Level Rise for Practitioners

Sea level rise (SLR) is a long-lasting consequence of climate change because global anthropogenic warming takes centuries to millennia to equilibrate for the deep ocean and ice sheets. SLR projections based on climate models support policy analysis, risk assessment and adaptation planning today, despite their large uncertainties. The central range of the SLR distribution is estimated by process-based models. However, risk-averse practitioners often require information about plausible future conditions that lie in the tails of the SLR distribution, which are poorly defined by existing models. Here, a community effort combining scientists and practitioners builds on a framework of discussing physical evidence to quantify high-end global SLR for practitioners. The approach is complementary to the IPCC AR6 report and provides further physically plausible high-end scenarios. High-end estimates for the different SLR components are developed for two climate scenarios at two timescales. For global warming of +2°C in 2100 (RCP2.6/SSP1-2.6) relative to pre-industrial values our high-end global SLR estimates are up to 0.9 m in 2100 and 2.5 m in 2300. Similarly, for a (RCP8.5/SSP5-8.5), we estimate up to 1.6 m in 2100 and up to 10.4 m in 2300. The large and growing differences between the scenarios beyond 2100 emphasize the long-term benefits of mitigation. However, even a modest 2°C warming may cause multi-meter SLR on centennial time scales with profound consequences for coastal areas. Earlier high-end assessments focused on instability mechanisms in Antarctica, while here we emphasize the importance of the timing of ice shelf collapse around Antarctica. This is highly uncertain due to low understanding of the driving processes. Hence both process understanding and emission scenario control high-end SLR.

54 ENVIRONMENTAL SCIENCES↗

Total fusion yield measurements using deuterium–tritium gamma rays

The deuterium–tritium (DT) fusion reaction, D ( T , γ ) 5 He , has a rare (4.2 × 10 – 5 ) branching ratio that releases a ~16 MeV gamma ray instead of the more common 14.1 MeV fusion neutron. These fusion gamma rays can be used as a complementary source of measuring the net fusion yield of experiments. Fusion gamma rays have the advantage of having negligible Doppler broadening, being isotropic and less down-scattered compared to fusion neutrons. At the National Ignition Facility, we measured the DT fusion gamma rays by the Gamma Reaction History diagnostic that thresholds to only measure >10 MeV gamma rays. After removing a ~12% contribution from neutron capture interactions in deuterium, D ( n , γ ) T , and carbon, 12 C ( n , γ ) 13 C , the deviation between GRH measurements and neutron-based yield measurements has been reduced to 10%. Further improvements are needed for detailed physics comparison.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

First spectral measurement of deuterium-tritium fusion γ rays in inertial fusion experiments

Here, the R-matrix analysis of A = 5 nuclear systems has been partially validated by applying the technique to the 5 Li system and comparing the predicted γ-ray spectrum with historical data. R-matrix analysis of the similar 5 He system was then used to predict the γ-ray spectral shape for the deuterium-tritium (DT) reaction. The resulting spectra have been used in the analysis of DT implosions on the Omega laser where the γ-ray interaction rate was measured by a gas Cherenkov detector. Comparison of predictions to experiment confirmed the presence of both 16.75 and ≈ 13 MeV γ-ray contributions; analysis, using R-matrix spectra, yielded a ratio of γ-ray emission from a transition to the intermediate excited state to that from a transition to the ground state of (2.1 ± 0.4):1, substantiating the first spectral measurement of the DT fusion γ ray in an inertial fusion environment.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗