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Clarity, Justin B.

Publications and source records attributed to Clarity, Justin B..

Temperature-Time Modeling of Spent Fuel Cladding in Dry Storage Casks

This report uses thermal and decay heat modeling to investigate spent fuel performance and the potential for cladding to anneal in dry storage conditions. Annealing is an important feature to investigate in SNF cladding because it has a direct relationship to cladding response in storage, transportation and disposal conditions. Annealed cladding may have lower strength than unannealed cladding, however its increased ductility would provide better protection against rupture in high strain rate situations such as severe accidents. These consequences are the driver for this work however are outside of the scope of this report. The modeling focused on three representative storage systems, the TN-32B, MAGNASTOR with TSC-37 canister, and NUHOMS AHSM with a 32PTH2 canister. This covers the vertical dual-purpose, vertical ventilated and horizontal ventilated casks respectively. Decay heat modeling using high and low enrichment assemblies was used to bound the decay heat curves that might be expected in dry storage. To bound the temperature relationship, the storage casks were modeled starting at the design basis heat loads with heat decaying through time. Although the results are bounding there is not an attempt to maximize conservatism, rather the intent to form a reasonable upper limit on temperature that will be broadly applicable to the U.S. cask fleet. This will allow materials testing to focus on relevant conditions for annealing that may affect the U.S. spent fuel inventory. The results show a clear dependence on heat load pattern in time in Figure S-1 and Figure S-2. This dependence is due to the different assembly decay heat curves for different assemblies in preferentially loaded casks. It shows the need for careful decay heat modeling when examining in service fuel temperatures that are less than the cask design basis heat load. The body of the report shows percent cladding cutoffs of 300°C and 350 °C as well. These results can be used to inform testing and conclusions about cladding performance through time and the potential for cladding annealing during dry storage.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A Comparison of As-loaded Dose Calculations to Measured Dose Rates

Demonstrating that the radiation dose fields surrounding spent nuclear fuel (SNF) storage and transportation systems meet the applicable limits set forth in 10 CFR 72 for storage and 10 CFR 71 for transportation is essential for the safe handling of radioactive material. The Used Nuclear Fuel-Storage, Transportation, and Disposal Analysis Resource and Data System (UNF-ST&DARDS) [2] is used to provide realistic estimates of SNF-related safety margins. The UNF-ST&DARDS dose rate analysis approach differs from that used in typical licensing approaches, which use design-basis assemblies with bounding source term characteristics to demonstrate the packaging design complies with the regulations. These bounding licensing approaches can increase the time needed to qualify fuel for loading into dry storage and the time a loaded system must wait prior to transportation. UNF-ST&DARDS dose rate assessments allow quantification of realistic, uncredited safety margins associated with actual fuel loading compared with the regulatory limits. While realistic estimation of the dose field surrounding SNF systems may allow for additional flexibility in operations, it is essential to understand how these predictions compare to measured doses. The U.S. Department of Energy Office of Integrated Waste Management and the Prairie Island Indian Community conducted a transportation dose assessment to estimate the site-specific incident-free radiation doses from shipping SNF by rail from the Prairie Island Nuclear Generating Plant (PINGP) through the Prairie Island Indian Community Reservation and Trust Land [5,6]. For that effort, the dose rates were obtained for 50 TN-40 and TN-40HT systems in storage configurations. This work compares the predicted dose rates from UNF-ST&DARDS as-loaded calculations with dose rates measured from 50 SNF storage systems at PINGP. The remainder of this paper discusses the data obtained for the evaluation, the modeling methods, and the results of the calculations.

spent nuclear fuel (SNF), UNF-ST&DARDS, Validation↗

UNF-ST&DARDS Enhancements for RCCA Data in As-loaded Dual Purpose Cask Models

This report summarizes the work performed to enable detailed modeling of rod cluster control assembly (RCCAs) in dual purpose canisters (DPCs) in as-loaded configurations using the Used Nuclear Fuel – Storage, Transportation & Disposal Analysis Resource and Data System (UNF-ST&DARDS). The goal of this project was to evaluate the reactivity impact that RCCAs have on k eff of DPCs with pressurized water reactor (PWR) fuel to potentially use the additional margin in future post-closure criticality safety analysis. This preliminary evaluation determined the number of DPCs that currently require compensatory actions prior to emplacement in a repository because of their high reactivity under post-closure criticality scenarios, which could be made acceptable by including the as-loaded RCCAs as specified in the Unified Database (UDB). This report briefly describes the modeling methods currently used within UNF-ST&DARDS and the modifications made to automate inclusion of the as-loaded RCCAs in the DPCs for post-closure criticality calculations for the loss of neutron absorber (NA) scenarios, or NA models. For the Zion site, the loss of basket scenarios, or degraded basket (DB) models, are also included. Discussion is also provided regarding the UDB data compared to available site-specific loading map data for the sites, which are specifically evaluated herein. This report compares the modifications to a similar evaluation for the Zion by site conducted by Walker as an initial validation. After the partial validation, all existing PWR sites with applicable NA models within the UDB were evaluated.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Preliminary Design of Critical Experiments Involving Commercially Available B 4 C Neutron Absorber Plates with Low-Enriched UO 2 Fuel [Slides]

Conclusions of this presentation conclude that the experiment is feasible with at least 10 critical configurations, and low expected benchmark uncertainty. Potential high impact for the understanding of commercially used neutron absorber plates. Next steps are to think about other configurations: rod pitch, other rods – Finalize plate support, uncertainty study. Additionally, the potential use of IER-441 central test region to safely place the plate in the core. Next steps include the Determination of the neutron absorber plate characterization path and the Potential SINBAD benchmark of neutron transmission measurements.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Modeling Non-UO2 Fuel With UNF-ST&DARDS

The U.S. Department of Energy’s Used Nuclear Fuel-Storage, Transportation & Disposal Analysis Resource and Data System (UNF-ST&DARDS) provides an easy-to-use interface to analyze irradiated UO2 fuel by allowing all analysis to be performed within the software and being able to store and use dozens of fuel assembly, canister, and cask designs [1]. However, performing these same analyses with non-UO2 fuel, such as UN or U3Si2, requires more user intervention in the process. This work uses UN, UN-ZrO2, and U3Si2 fuel to demonstrate how to perform criticality analyses in the current versions of UNF-ST&DARDS and how a non-UO2 fuel will compare to UO2. This work is part of a larger effort that also includes shielding and thermal analyses, but they will not be discussed.

Ivanusa, Pavlo↗

Optimization of Canister Loading Patterns in Dual Purpose Canisters for Criticality Suppression

This report documents work performed in support of the US Department of Energy Office of Nuclear Energy (NE) Spent Fuel and Waste Disposition, Spent Fuel and Waste Science and Technology, under work breakdown structure element 1.08.01.03.05, “Direct Disposal of Dual Purpose Canisters.” In particular, this report fulfills milestone M3SF-22PN010305094, “Application of AI/ML techniques to optimize DPC loading,” within work package SF-22PN01030509, “Direct Disposal of Dual Purpose Canisters - PNNL.” This report continues the process of examining the potential for using loading optimization as a disposal criticality suppression technique. This latest update to the report added: 1. A validation of the artificial neural network (ANN) reactivity prediction tool against as-loaded dual-purpose canisters from the UNF-ST&DARDS database 2. Refinement of the algorithm to incorporate an additional DPC design to improve the predictions 3. Investigation of a storage and transportation focused loading optimization algorithm. A key result from this year’s work is that the ANN performance was significantly improved by including the additional model for the NUHOMS canisters and it is apparent that fuel type specific modeling considerations should be incorporated into the ANN in future work. The GRASP-enabled adaptive multi-objective memetic algorithm with partial clustering (GAMMA-PC) algorithm was evaluated as a tool for storage and transportation oriented optimization. The GAMMA-PC optimization routine considers decay heat at loading, the time between loading and when the canister is eligible for transportation and minimizes the number of casks loaded. Future work will develop a dose minimization optimization routine.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Dual Purpose Canister Reactivity and Groundwater Absorption Analyses

The current spent nuclear fuel (SNF) management strategy includes reliance on dry storage. Utilities are meeting their interim storage needs on an individual basis with use of large-capacity dry storage casks, with a current focus on meeting existing storage and transportation requirements, as disposal requirements are not currently available. These casks are commonly known as dual-purpose (i.e., storage and transportation) canisters (DPCs). However, a small percentage of single-purpose (storage only) systems is also being used to meet storage needs. These are included under the “DPC” heading. This report investigates the postclosure criticality safety aspects of DPCs. Placing large, heavy waste packages containing DPCs into a repository for direct disposal has not yet been implemented domestically or internationally. Therefore, direct disposal of DPCs represents new engineering and scientific challenges. Some of the engineering challenges that have already been addressed include handling and placement, use of ramps vs. shafts, use of hoists, use of transport equipment, and thermal management. Additionally, some studies have been conducted in the past regarding the feasibility of direct disposal from a criticality analysis perspective and have concluded that while possible, demonstrating subcriticality over the disposal time period is a challenge. The alternative to direct disposal of DPCs into a repository is to repackage the SNF into different canisters. The direct disposal of DPCs without cutting them open and repackaging is appealing because it could be more cost-effective, reduce the complexity of fuel management operations both in and outside reactor facilities, and result in less cumulative worker dose during interim storage and handling before eventual disposal in a deep geologic repository.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Impact of Increased Latent Generations on Sensitivity Calculations with SCALE

Analyses of cross section sensitivity data from systems with fissile material allow analysts to associate an importance for each material, nuclide, reaction, and neutron energy by simulating real world criticality scenarios. Although criticality safety validation efforts can be guided by the cross-section sensitivity and uncertainty data generated for a particular system, these calculations can often be computationally expensive and sometimes cumbersome without proper guidance. The TSUNAMI suite within the SCALE code package has several methods for generating sensitivity data, including multigroup and continuous energy (CE) capabilities. The release of SCALE 6.3 has three different CE methods for generating cross section sensitivity data: (1) the Iterated Fission Probability (IFP) method with the KENO Monte Carlo transport solver, (2) the IFP method with the Shift Monte Carlo transport solver, and (3) the Contributon-Linked eigenvalue sensitivity/Uncertainty estimation via Tracklength importance CHaracterization (CLUTCH) method with the KENO Monte Carlo transport solver. Although the CLUTCH method has additional parameters for generating sensitivity data files relative to the IFP method, all three methods use latent generations, which are the generations between an event (i.e., fission) and the assessment of importance based on the asymptotic population of progeny neutrons. Increasing the number of latent generations in a calculation leads to increased discrimination of the sensitivity coefficients but at the cost of the increased uncertainty associated with those generated values. Analysts must balance the accuracy of the sensitivity calculations and its uncertainty with the associated computational cost involved in generating the values. This paper discusses the impact of adjusting the latent generation parameter for a range of sensitivity values and how these changes compare with the direct perturbation values obtained from a change of ±0.5% Δ k in both benchmark and safety application models. Two benchmarks from the International Handbook of Evaluated Criticality Safety Benchmark Experiments and the MPC-32 dual purpose canister for spent nuclear fuel are used for analysis.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Impact of Increased Latent Generations on Sensitivity Calculations with SCALE [Slides]

Depending on the system, energy, and/or nuclide, altering the number of latent generations can significantly impact generated sensitivity coefficients. In general, as the number of latent generations increases, the accuracy of the generated sensitivity value compared with the DP value increases and there is a significant increase in the uncertainty with generated sensitivity values. IFP generated sensitivities appear to be more stable than those with CLUTCH. Complex systems, even with IFP and increased latent generations can still produce poor results (i.e., MPC- 32). This reiterates the importance of performing DPs to confirm sensitivities. IFP-Shift and CLUTCH can take advantage of parallel computing abilities. Work continues in this area as additional parameters and calculational methods are examined to provide analysts insights to successfully generating sensitivity coefficients for confirmatory analyses and validation efforts.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Expansion of the ORNL VALID Library [Slides]

VALID continues as a library of high-quality models used for testing SCALE and nuclear data. Recent expansion of VALID was the largest impactful change in a decade. Adding 233 U experiments circa 2017 added more cases. There are a huge number of cases in the pipeline, but a lack of qualified staff and funding to complete reviews. Future plans should simplify the process and increase the availability of models and results for external users.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Horizontal Split Table Conceptual Design for Advanced Reactor Validation

Oak Ridge National Laboratory and Lawrence Livermore National Laboratory are collaborating to develop a conceptual design for a horizontal split table for use in performing critical experiments. The goal of this design effort is to provide nuclear data testing and validation capabilities for advanced reactors such as pebble-bed high-temperature gas-cooled reactors, molten salt reactors, and heat pipe microreactor, but it could also be used for the current generation of reactors. The first concept being explored for the horizontal split table, a pebble-bed design based on the HTR-10 reactor, is described in this paper. A critical configuration corresponding to a footprint of about 4.5 m 2 was determined with SCALE/KENO-VI to fit the planned dimensions of the horizontal split table. The similarity of the pebble-bed design and the HTR-10 reactor application was assessed using SCALE/TSUNAMI, and a similarity coefficient $c_k$ of 0.9982 was obtained, proving that the concept will be useful for nuclear data validation and assimilation of pebble-bed type advanced reactors. In the proposed design, the materials with the highest $k_{eff}$ sensitivity are graphite and uranium, demonstrating that particular care must be given to carbon-related cross-section data. The effect of mechanical uncertainties between the fixed and moving tables was also assessed by calculating the reactivity change caused by vertical and horizontal gaps, as well as angular and torsion offsets between the two sides of the horizontal split table concept. The highest relative changes on the concept’s reactivity were caused by angular perturbations. The same analysis process is currently being used to create a molten salt advanced reactor type horizontal split table concept based on the Molten Salt Reactor Experiment (MSRE).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Impacts of LEU+ and ATF on Fresh Fuel Storage Criticality Safety

The use of increased fuel enrichment, which is still in the realm of low-enriched uranium (LEU) fuel, has been of interest to commercial light water reactor operators as part of the next iteration in fuel cycle technological advances and research and development. Using increased enrichment fuel, or high-assay LEU (HALEU), in power plants has clear benefits for being able to load cores with additional power-producing fuel. Although HALEU enrichments can range up to 20%, the more guarded approach of investigating enrichments above current fuels within 10% enrichment is referred to as LEU plus (LEU+) to reflect the less drastic change in operating conditions and requirements and similarity to current fuel cycles. Of additional interest and increasing maturity is the incorporation of accident-tolerant fuel (ATF) concepts, which are also applicable to the current fleet. This class of technologies involves changes such as cladding (e.g., chromium coating or FeCrAl) and fuel composition (e.g., chromia dopant) alterations to demonstrate improved fuel performance under accident scenarios. The ability to properly store fuel before and after residence time in the reactor is crucial to plant operation. Typically, this is done in either a new fuel vault (NFV) or spent fuel pool (SFP). Storing, loading, and unloading dozens of fuel assemblies within the same general area provides opportunities for obvious criticality concerns. These concerns are addressed with regulations to the subcriticality margin that the NFV and SFP must maintain in certain conditions. Adopting LEU+ fuel results in inherent reactivity increases, which are extremely relevant for safe fuel storage. Therefore, a clear understanding of the effects of LEU+ fuel and ATF on criticality safety margins to regulatory limits is required, as well as an understanding of the degree of absorber crediting under normal and accident conditions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗