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Connor Flynn

Publications and source records attributed to Connor Flynn.

Multi-Campaign Ship and Aircraft Observations of Marine Cloud Condensation Nuclei and Droplet Concentrations

In-situ marine cloud droplet number concentrations (CDNCs), cloud condensation nuclei (CCN), and CCN proxies, based on particle sizes and optical properties, are accumulated from seven field campaigns: ACTIVATE; NAAMES; CAMP2EX; ORACLES; SOCRATES; MARCUS; and CAPRICORN2. Each campaign involves aircraft measurements, ship-based measurements, or both. Measurements collected over the North and Central Atlantic, Indo-Pacific, and Southern Oceans, represent a range of clean to polluted conditions in various climate regimes. With the extensive range of environmental conditions sampled, this data collection is ideal for testing satellite remote detection methods of CDNC and CCN in marine environments. Remote measurement methods are vital to expanding the available data in these difficult-to-reach regions of the Earth and improving our understanding of aerosolcloud interactions. The data collection includes particle composition and continental tracers to identify potential contributing CCN sources. Several of these campaigns include High Spectral Resolution Lidar (HSRL) and polarimetric imaging measurements and retrievals that will be the basis for the next generation of space-based remote sensors and, thus, can be utilized as satellite surrogates.

Atmospheric chemistry↗

Airborne and Ground-Based Measurements of Aerosol Optical Depth of Freshly Emitted Anthropogenic Plumes in the Athabasca Oil Sands Region

In this work we report the airborne aerosol optical depth (AOD) from measurements within freshly emitted anthropogenic plumes arising from mining and processing operations in the Athabasca Oil Sands Region (AOSR) in the context of ground-based AERONET climatological daily averaged AODs at Fort McMurray (Alberta, Canada). During two flights on 9 and 18 June 2018, the NASA airborne 4STAR (Spectrometers for Sky-Scanning, Sun-Tracking Atmospheric Research) Sun photometer registered high fine-mode (FM, <1 µm) in-plume AODs of up to 0.4 and 0.9, respectively, in the vicinity of the plume source (<20 km). Particle composition shows that the plumes were associated with elevated concentrations of sulfates and ammonium. These high AODs significantly exceed climatological averages for June and were not captured by the nearby AERONET instrument (mean daily AODs of 0.10±0.01 and 0.07±0.02, maximum AOD of 0.12) due possibly to horizontal inhomogeneity of the plumes, plume dilution and winds which in certain cases were carrying the plume away from the ground-based instrument. The average 4STAR out-of-plume (background) AODs deviated only marginally from AERONET daily averaged values. While 4STAR AOD peaks were generally well correlated in time with peaks in the in situ-measured particle concentrations, we show that differences in particle size are the dominant factor in determining the 4STAR-derived AOD. During the two flights of 24 June and 5 July 2018 when plumes likely travelled distances of 60 km or more, the average 4STAR FM AOD increased by 0.01–0.02 over ∼50 km of downwind particle evolution, which was supported by the increases in layer AODs calculated from the in situ extinction measurements. Based on these observations as well as the increases in organic mass, we attribute the observed AOD increase, at least in part, to secondary organic aerosol formation. The in-plume and out-of-plume AODs for this second pair of flights, in contrast to clear differences in in situ optical and other measurements, were practically indistinguishable and compared favourably to AERONET within 0.01–0.02 AOD. This means that AERONET was generally successful in capturing the background AODs, but missed some of the spatially constrained high-AOD plumes with sources as close as 30–50 km, which is important to note since the AERONET measurements are generally thought to be representative of the regional AOD loading. The fact that industrial plumes can be associated with significantly higher AODs in the vicinity of the emission sources than previously reported from AERONET can potentially have an effect on estimating the AOSR radiative impact.

AERONET↗

Evaluation of Novel NASA MODIS and VIIRS Aerosol Products and Assessment of Smoke Height Boundary Layer Ratio During Extreme Smoke Events in the Western U.S.

We analyze new aerosol products from NASA satellite retrievals over the western U.S. during August 2013, with special attention to locally generated wildfire smoke and downwind plume structures. Aerosol optical depth (AOD) at 550 nm from MODIS (Terra and Aqua Collections 6 and 6.1) and VIIRS Deep Blue (DB) and MODIS (Terra and Aqua) Multi‐Angle Implementation of Atmospheric Correction (MAIAC) retrievals are evaluated against ground‐based AErosol RObotic NETwork (AERONET) observations. We find a significant improvement in correlation with AERONET and other metrics in the latest DB AOD (MODIS C6.1 r^2=0.75, VIIRS r^2=0.79) compared to MODIS C6 (r2=0.62). In general, MAIAC (r^2=0.84) and DB (MODIS C6.1 and VIIRS) present similar statistical evaluation metrics for the western U.S. and are useful tools to characterize aerosol loading associated with wildfire smoke. We also evaluate three novel NASA MODIS plume injection height (PIH) products, one from MAIAC and two from the Aerosol Single scattering albedo and layer Height Estimation (ASHE) (MODIS and VIIRS) algorithm. Both Terra and Aqua MAIAC PIHs statistically agree with ground‐based and satellite lidar observations near the fire source, as do ASHE, although the latter is sensitive to assumptions about aerosol absorption properties. We introduce a first‐order approximation Smoke Height Boundary Layer Ratio (SHBLR) to qualitatively distinguish between aerosol pollution within the planetary boundary layer and the free troposphere. We summarize the scope, limitations, and suggestions for scientific applications of surface level aerosol concentrations specific to wildfire emissions and smoke plumes using these novel NASA MODIS and VIIRS aerosol products.

Plume injection height↗

Sky-Scanning Sun-Tracking Airborne Radiometer (3STAR): Instrument Design, Flight Testing, and Tracking Performance

The Sky-Scanning, Sun-Tracking Airborne Radiometer (3STAR) adapts commercial radiometer technology developed for the ocean color research community to airborne measurement of spectrally resolved solar irradiance and sky radiance. These atmospheric observations are used to derive aerosol optical depth (AOD), supporting localized AOD inputs for atmospheric correction of satellite and airborne data over terrestrial and aquatic (including optically dark) targets. The ability to regionally “tune” atmospheric correction schemes with relevant spatial AOD supports constraining atmospheric correction of remote sensing reflectance. Very wide dynamic range has been achieved for multi-channel band-pass-filter-radiometers originally designed for deployment into the water column. By actively tracking and directly pointing to the Sun, the light attenuation by aerosol particles in the atmospheric column can be quantified. These measurements improve knowledge of atmospheric constituents and the atmospheric corrections required to improve remote sensing capabilities for interpreting reflectance measurements from the Earth surface. 3STAR incorporates a custom Sun-tracking/sky-scanning pointing head, a Sun-tracking camera, and a commercially available, cylindrical, 19-channel radiometer tube assembly. An accurate and responsive mount and tracking system has been developed and certified to NASA and Naval Air Systems Command (NAVAIR) airworthiness standards for deployment into the aircraft slipstream. Ground and flight testing indicate typical tracking errors of less than 0.1 degrees, well within the field of view of the radiometer as required to minimize measurement uncertainty from alignment error. Preliminary AOD measurements compare to within 0.013 with 15 measurements from an Aerosol Robotic Network (AERONET) Cimel instrument at 500 nm wavelength and low solar angle.

Atmosphere↗

Modeling the smoky troposphere of the southeast Atlantic: a comparison to ORACLES airborne observations from September of 2016

In the southeast Atlantic, well-defined smoke plumes from Africa advect over marine boundary layer cloud decks; both are most extensive around September, when most of the smoke resides in the free troposphere. A framework is put forth for evaluating the performance of a range of global and regional atmospheric composition models against observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) airborne mission in September 2016. A strength of the comparison is a focus on the spatial distribution of a wider range of aerosol composition and optical properties than has been done previously. The sparse airborne observations are aggregated into approximately 2° grid boxes and into three vertical layers: 3–6 km, the layer from cloud top to 3 km, and the cloud-topped marine boundary layer. Simulated aerosol extensive properties suggest that the flight-day observations are reasonably representative of the regional monthly average, with systematic deviations of 30 % or less. Evaluation against observations indicates that all models have strengths and weaknesses, and there is no single model that is superior to all the others in all metrics evaluated. Whereas all six models typically place the top of the smoke layer within 0–500 m of the airborne lidar observations, the models tend to place the smoke layer bottom 300–1400 m lower than the observations. A spatial pattern emerges, in which most models underestimate the mean of most smoke quantities (black carbon, extinction, carbon monoxide) on the diagonal corridor between 16° S, 6° E, and 10° S, 0° E, in the 3–6 km layer, and overestimate them further south, closer to the coast, where less aerosol is present. Model representations of the above-cloud aerosol optical depth differ more widely. Most models overestimate the organic aerosol mass concentrations relative to those of black carbon, and with less skill, indicating model uncertainties in secondary organic aerosol processes. Regional-mean free-tropospheric model ambient single scattering albedos vary widely, between 0.83 and 0.93 compared with in situ dry measurements centered at 0.86, despite minimal impact of humidification on particulate scattering. The modeled ratios of the particulate extinction to the sum of the black carbon and organic aerosol mass concentrations (a mass extinction efficiency proxy) are typically too low and vary too little spatially, with significant inter-model differences. Most models overestimate the carbonaceous mass within the offshore boundary layer. Overall, the diversity in the model biases suggests that different model processes are responsible. The wide range of model optical properties requires further scrutiny because of their importance for radiative effect estimates.

Yohei Shinozuka↗

Above-Cloud Aerosol Radiative Effects based on ORACLES 2016 and ORACLES 2017 Aircraft Experiments

Determining the direct aerosol radiative effect (DARE) of absorbing aerosols above clouds from satellite observations alone is a challenging task, in part because the radiative signal of the aerosol layer is not easily untangled from that of the clouds below. In this study, we use aircraft measurements from the NASA ObseRvations of CLouds above Aerosols and their intEractionS (ORACLES) project in the southeastern Atlantic to derive it with as few assumptions as possible. This is accomplished by using spectral irradiance measurements (Solar Spectral Flux Radiometer, SSFR) and aerosol optical depth (AOD) retrievals (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research, 4STAR) during vertical profiles (spirals) that minimize the albedo variability of the underlying cloud field – thus isolating aerosol radiative effects from those of the cloud field below. For two representative cases, we retrieve spectral aerosol single scattering albedo (SSA) and the asymmetry parameter (g) from these profile measurements and calculate DARE given the albedo range measured by SSFR on horizontal legs above clouds. For mid-visible wavelengths, we find SSA values from 0.80 to 0.85 and a significant spectral dependence of g. As the cloud albedo increases, the aerosol increasingly warms the column. The transition from a cooling to a warming top-of-aerosol radiative effect occurs at an albedo value (critical albedo) just above 0.2 in the mid-visible wavelength range. In a companion paper, we use the techniques introduced here to generalize our findings to all 2016 and 2017 measurements and parameterize aerosol radiative effects.

Cloud aerosol↗

Airborne Remote Sensing Measurements of Particles in Different Parts of the World

Around the globe, atmospheric aerosols pose a significant yet uncertain impact on the Earth's climate, environmental air quality and human health. Suborbital sunphotometer measurements of Aerosol Optical Depth (AOD) (i.e., the amount of direct-beam solar light attenuated by aerosols within the atmospheric column) are used to validate satellite aerosol retrievals and are valuable when studying aerosol-solar radiation and/ or aerosol-cloud interactions. Since 1985, NASA Ames Research Center (ARC) has been using airborne sun-tracking sunphotometers to measure atmospheric constituents such as aerosols, clouds, and gases. The NASA Ames Airborne Tracking Sunphotometer (AATS-6) and then (AATS-14) operate by tracking the sun and measuring the transmission of solar radiation in 6 to 14 discrete spectral channels (Russell et al., 1986). The AATS systems were followed by the more advanced hyperspectral 4STAR instrument (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research; Dunagan et al., 2013), which combines the airborne sun-tracking capability of the AATS-14 with a sky scanning feature similar to the ground-based Aerosol Robotic Network Sun/sky photometers (AERONET). We present a comprehensive analysis of ~30 airborne campaigns undertaken by NASA and DoE based on a new database of airborne sunphotometer measurements. Using this database, we present a clear picture of airborne AODs over the range of historical campaigns and the aerosol sizes per region, especially over the ocean where AERONET data is limited. With this database, we can investigate systematic differences in AOD such as those observed over different land and ocean surfaces in specific geographical regions. Finally, we will briefly show comparisons with satellite aerosol retrievals from MODIS and/or VIIRS. Russell, P. B., T. Matsumoto, V. J. Banta, J. M. Livingston, C. Mina, D. S. Colburn, and R. F. Pueschel (1986), Measurements with an airborne, autotracking, external-head sunphotometer, Preprint Volume, Sixth Conference on Atmospheric Radiation, May 13–16, 1986, Amer. Meteor.Soc., Boston, MA, 55–58. Dunagan, Stephen E., et al. "Spectrometer for sky-scanning sun-tracking atmospheric research (4STAR): Instrument technology." Remote Sensing 5.8 (2013): 3872-3895

Brendan Stover Cornelison↗

Robotic Sunphotometry to Enable Over-ocean Aerosol Characterization

We present developmentsforthe Sea-going Sky-Scanning Sun-tracking Advanced Research Ra-diometer(SeaSTAR), a ship-basedinstrument for aerosol characterizationover the ocean. Sun-tracking measurements of spectral solar irradiance are madein the conventional manner using filter-photodiode radiometers, and co-aligned polarizing filters are switched into the optical paths of the radiometersto measure polarized sky-radiance measurements. A robust high-performance robot with camera-feedback sun-tracking, and inertial measurement unit feed-forward motion-compensationis used for the sun-and sky-viewing modes respectively. An inverse-kinematics solver is used to point the instrument at the chosen position relative to the sunand ensure that the polarizer axis remains in the desired orientation, allowing the Stokes vector components of the sky radiance to be resolved by rotating the measurement barrel about a third robot axis. SeaSTAR aims to provide a resource for cost-effective validation of aerosol property measurements over the oceans in support of satellite missions such as PACE, SBG and GLIMR.

Robotic↗