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Daw, Joshua

Publications and source records attributed to Daw, Joshua.

At least 19 records

Ultrasonic Transducer Irradiation Test Results

Ultrasonic technologies offer the potential for high accuracy and resolution in-pile measurement of a range of parameters, including geometry changes, temperature, crack initiation and growth, gas pressure and composition, and microstructural changes. Many Department of Energy-Office of Nuclear Energy (DOE-NE) programs are exploring the use of ultrasonic technologies to provide enhanced sensors for in-pile instrumentation during irradiation testing. For example, the ability of small diameter ultrasonic thermometers (UTs) to provide a temperature profile in candidate metallic and oxide fuel would provide much needed data for validating new fuel performance models. These efforts are limited by the lack of identified ultrasonic transducer materials capable of long term performance under irradiation test conditions. To address this need, the Pennsylvania State University (PSU) was awarded an Advanced Test Reactor National Scientific User Facility (ATR NSUF) project to evaluate the performance of promising magnetostrictive and piezoelectric transducers in the Massachusetts Institute of Technology Research Reactor (MITR) up to a fast fluence of at least 1021 n/cm2 . A multi-National Laboratory collaboration funded by the Nuclear Energy Enabling Technologies Advanced Sensors and Instrumentation (NEET ASI) program also provided initial support for this effort. This irradiation, which started in February 2014, is an instrumented lead test and real-time transducer performance data are collected along with temperature and neutron and gamma flux data. The irradiation is ongoing and will continue to approximately mid-2015. To date, very encouraging results have been attained as several transducers continue to operate under irradiation.

Daw, Joshua↗

Methods for making high-temperature thermocouples

Methods of manufacturing thermocouples having a first thermoelement wire comprises a molybdenum-lanthanum based material and a second thermoelement wire comprises a phosphorus-doped niobium, may involve exposing a first thermoelement wire and a second thermoelement wire to a temperature in a range extending from about 50° C. to about 60° C. above an intended operational temperature of the first and second thermoelement wires and until a rate of change of a normalized voltage output of the first thermoelement wire and the second thermoelement wire is about 0.001 normalized Volts per hour or less.

Skifton, Richard S.↗

Sensors for passively measuring a maximum temperature of a nuclear reactor, and related methods

A sensor for passively measuring a maximum temperature within a nuclear reactor comprises a substrate, and a plurality of melt wires within a cavity defined within the substrate, at least one melt wire of the plurality of melt wires exhibiting a variable melting temperature along a length of the at least one melt wire. Related sensors and methods of forming the sensors are also disclosed.

Daw, Joshua↗

Ultrasonic sensors and methods of using the ultrasonic sensors

An ultrasonic sensor comprises a transducer in operable communication with a power source, a waveguide comprising a metal and at least one of a fissile material or a fertile material in operable communication with the transducer and configured to propagate and reflect acoustic waves generated by the transducer, the transducer configured to convert reflected acoustic waves to an electric signal, a thermally insulative material proximate the waveguide, and a control system in operable communication with the transducer, the control system configured to determine at least a temperature of the waveguide based on the reflected acoustic waves. Related methods are also disclosed.

Woolstenhulme, Nicolas E.↗

Aerosol jet printing of piezoelectric surface acoustic wave thermometer

Abstract Surface acoustic wave (SAW) devices are a subclass of micro-electromechanical systems (MEMS) that generate an acoustic emission when electrically stimulated. These transducers also work as detectors, converting surface strain into readable electrical signals. Physical properties of the generated SAW are material dependent and influenced by external factors like temperature. By monitoring temperature-dependent scattering parameters a SAW device can function as a thermometer to elucidate substrate temperature. Traditional fabrication of SAW sensors requires labor- and cost- intensive subtractive processes that produce large volumes of hazardous waste. This study utilizes an innovative aerosol jet printer to directly write consistent, high-resolution, silver comb electrodes onto a Y-cut LiNbO 3 substrate. The printed, two-port, 20 MHz SAW sensor exhibited excellent linearity and repeatability while being verified as a thermometer from 25 to 200 ∘ C. Sensitivities of the printed SAW thermometer are $$-96.9\times 1{0{}^{-6}}^{\circ }$$ − 96.9 × 1 0 − 6 ∘ C −1 and $$-92.0\times 1{0{}^{-6}}^{\circ }$$ − 92.0 × 1 0 − 6 ∘ C −1 when operating in pulse-echo mode and pulse-receiver mode, respectively. These results highlight a repeatable path to the additive fabrication of compact high-frequency SAW thermometers.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Irradiation Behavior of Piezoelectric Materials for Nuclear Reactor Sensors

In-situ measurement of surface acoustic wave (SAW) resonators were used to characterize piezoelectric materials behavior in a nuclear reactor environment. Lithium niobate and aluminum nitride devices were tested up to 500°C temperature and 450 kW reactor power (1.9x10 12 n/cm 2 s). The resonant frequency responds to step changes in temperature and power. Materials’ response are inferred from the observed resonant frequency changes, in particular the kinetic behavior is used to determine mechanisms responsible for observed changes. The observed response is attributed to two mechanisms: temperature increase from gamma heating and accumulation of radiation-induced defects. Both of these mechanisms alter the physical properties of the piezoelectric materials, particularly the elastic constants. The demonstrated repeatability and reliability of SAW devices are attractive for sensor applications in extreme environments.

36 MATERIALS SCIENCE↗

Multi-core high-temperature, irradiation-resistant thermocouple, and related methods

A multi-core thermocouple includes a plurality of wires, an insulation core surrounding the plurality of wires, a sheath surrounding the insulation core, and a plurality of electrical junctions. The plurality of electrical junctions may include a first electrical junction formed between a first wire of the plurality of wires and the sheath at a first axial mid-section of the multi-core thermocouple, the first electrical junction including a first swaged axial mid-section of the sheath and a second electrical junction formed between a second wire of the plurality of wires and the sheath at a second, different axial mid-section of the multi-core thermocouple, the second electrical junction including a second swaged axial mid-section of the sheath.

Skifton, Richard S.↗

High-temperature, irradiation-resistant thermocouple, coaxial thermocouple, and related methods

A coaxial thermocouple includes a wire, an insulation layer surrounding the wire, a sheath surrounding the insulation layer, and an electrical junction formed between the wire and the sheath and at one longitudinal end of the coaxial thermocouple, the electrical junction including a swaged end with an outer diameter of the sheath reducing in diameter along a longitudinal length of the coaxial thermocouple until the sheath contacts the wire within the insulation layer. The wire includes a first material and the sheath includes a second material where the first material includes one of molybdenum (Mo) or niobium (Nb) and the second material includes the other of molybdenum (Mo) or niobium (Nb).

Skifton, Richard S.↗

Magnetostrictive Ultrasonic Waveguide Transducer for In-Pile Thermometry

Real-time and reliable temperature measurement on nuclear fuels is crucial for the safe operation of existing pressurized-water reactors and future advanced nuclear reactors. Magnetostrictive materials deform when subjected to a magnetic field or exhibit magnetization variation when stressed. Here, based on these properties, this study prototyped an ultrasonic thermometer (UT) consisting of a magnetostrictive waveguide, a dc coil providing appropriate magnetic biasing, and an ac coil generating an acoustic impulse and detecting the resulting acoustic echoes. By tracking the time of flight between the excitation pulse and the echoes, the UT can potentially detect nuclear fuel cladding temperature from a long distance. In this study, magnetostrictive iron–gallium alloys, or Galfenol, were selected as the waveguide due to their large magnetostriction, superior temperature survivability, excellent radiation resilience, and high mechanical robustness. A multiphysics finite-element model considering electrical, magnetic, and mechanical dynamics in the magnetostrictive UT was then developed. The model exhibited an error of 0.24% in time-of-flight simulation and, therefore, enabled computer-aided design and guided signal processing. Between room temperature and 120 °C, the new Galfenol-based UT exhibits a linear sensitivity of 162.8×10 ₋6 °C ₋1 , which is 51.7% higher than a previous magnetostrictive UT based on iron–cobalt–vanadium alloys.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Sensors for measuring thermal conductivity and related methods

A sensor for measuring thermal conductivity includes an insulator, a test material over the insulator, a conductor over the test material, and a gas within an open volume adjacent the test material and the conductor. An electrical source is configured to provide an alternating current through the conductor to heat the test material. Leads are connected to the conductor and configured to connect to a voltmeter. A method of measuring thermal conductivity includes disposing the sensor in a reactor core in which a nuclear fuel undergoes irradiation and radioactive decay. An alternating current is provided from the electrical source through the conductor to heat the test material. A voltage is measured as a function of time at the leads connected to the conductor. A thermal conductivity of the test material is calculated based on the voltage measured as a function of time. Methods of forming a sensor are also disclosed.

Daw, Joshua↗

Design Requirements for Ultrasonic Deformation Sensor for TREAT Experiments

Ultrasonic measurements of deformation can provide nondestructive measurements of dimensional changes rapidly (within tens to hundreds of microseconds). Further these methods are sensitive to both microstructural changes due to damage (from thermal, mechanical, and irradiation environments) and gross structural changes (such as swelling). As a result, ultrasonic methods have been applied to address needs in the nondestructive evaluation of structural components in nuclear power plants (including fuel cladding) during periodic pre-service and in-service inspection inspections. Ultrasonic measurements have been successfully used for nondestructive materials characterization, including nondestructive evaluation (NDE) of degradation and damage, microstructure characterization, and process control. Ultrasonic NDE is a critical element of the nuclear power industry’s in-service inspection program for maintaining the integrity of the pressure boundary, and is being actively investigated for post-irradiation examination of fuels. Ultrasonic measurements, typically performed at 10 MHz or higher, performed post irradiation show that fuel microstructural parameters, such as porosity and grain size, can be correlated to ultrasonic velocity. Ultrasonic methods historically have seen limited applicability to environments with high temperatures and irradiation. Though some environmental factors (such as temperature) affect the measurement (sound speed, for instance), the limitation is primarily due to the probes themselves. Most commonly, lead-zirconate-titanate (PZT) is used as the piezoelectric sensor material for ultrasonic nondestructive measurements. PZT is limited in its applicability at elevated temperatures (approximately above 300C). However, recent tests (through DOE-NE’s NEET-ASI program) have identified a number of alternatives that can operate at elevated temperatures (in excess of 400C) and can survive irradiation. Certain grades of PZT have also been demonstrated for use in imaging under-sodium in sodium fast reactors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Research plan for the development of optical fiber pressure sensors for nuclear applications

Fiber optic pressure sensors are desirable for nuclear applications because they are low mass/small size, immune to electromagnetic interference, high sensitivity, and have multiplexing and multimodal measurement capabilities. Much research and development has been conducted on developing fiber optic based sensors and they are now considered a class of standard instrumentation in many industries. Specifically, for pressure sensing, a wide range of fiber based sensors have been developed for various pressure ranges and environments. This vast body of research will be leveraged for the development of pressure sensors for nuclear applications. Four pressure measurement scenarios were considered which would benefit from a fiber optic based pressure sensor. These scenarios include pressure measurement in the fuel rod plenum, coolant pressure during LOCA testing, advanced coolant (helium, sodium, molten salt) pressure for flow loop operation, and high pressures resulting for direct fuel-coolant interaction. Each scenario has unique pressure, temperature, and material requirements for the sensor. From a survey of commercially available sensors and a literature review; it has been determined that an extrinsic Fabry-Perot interferometer approach is the most appropriate for the various measurement requirements. The experience and knowledge base for Fabry-Perot interferometers can be leveraged since they are the most common fiber optic based pressure sensors available commercially and found in literature. These pressure sensors rely on the interference of light in a gas filled cavity, which minimizes the impact of radiation induced attenuation and compaction on the measurement, compared to intrinsic sensing techniques. The measurement range of these sensors is based on the stiffness of the diaphragm that deflects under pressure. This allows for a suite of fiber based sensors to be developed by interchanging this diaphragm for the requirements of each application. Key material and design considerations have been identified for the development of a Fabry-Perot interferometry pressure measurement for nuclear applications. These include high temperature bonding between the glass fiber optic and metal housing, identifying diaphragm materials & geometry, and minimizing cross sensitivity to temperature or implementing compensation techniques found in literature. Overcoming these challenges will develop a pathway for a fiber optic based pressure sensor for nuclear applications, and additionally can be leveraged for other sensing application based on Fabry-Perot interferometers, such as temperature, strain (creep & deformation), vibration, and index of refraction.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Upcoming irradiation of ultrasonic and fiber optic sensors in the MITR - 361

Fiber optic and ultrasonic technologies offer the potential for high accuracy and resolution in-pile measurement of a range of parameters, including geometry changes, temperature, crack initiation and growth, gas pressure and composition, and microstructural changes. These technologies, which have performed successfully in out-of-pile tests, have not been well qualified in a test reactor environment. The uncertainty of successful operation of instruments at this level of development has typically been a significant barrier to in-core deployment. Many Department of Energy-Office of Nuclear Energy (DOE-NE) programs are exploring the use of these technologies to provide enhanced sensors for irradiation testing. For example, the ability of small diameter ultrasonic thermometers (UTs) to provide a temperature profile in candidate metallic and oxide fuel would provide much needed data for validating new fuel performance models. The National Scientific User Facility (NSUF) is sponsoring a project to evaluate the performance of promising temperature sensors based on ultrasound and on fiber optics during an upcoming irradiation test in the Massachusetts Institute of Technology Research Reactor (MITR). Several types of thin-wire metallic waveguide ultrasonic thermometers will be tested along with fiber optic temperature sensors using regenerated Fiber-Bragg Grating technology. Additionally, samples of several new optical materials which are potentially much more radiation tolerant than commonly used fiber materials, such as silica, will be included and analyzed post-irradiation. The irradiation is a collaborative effort between researchers from Idaho National Laboratory, the French Alternative Energies and Atomic Energy Commission, the University of Pittsburgh, the Massachusetts Institute of Technology, and AFO Research, Inc. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Upcoming Irradiation of Ultrasonic and Fiber Optic Sensors in the MITR

Fiber optic and ultrasonic technologies offer the potential for high accuracy and resolution in-pile measurement of a range of parameters, including geometry changes, temperature, crack initiation and growth, gas pressure and composition, and microstructural changes. These technologies, which have performed successfully in out-of-pile tests, have not been well qualified in a test reactor environment. The uncertainty of successful operation of instruments at this level of development has typically been a significant barrier to in-core deployment. Many Department of Energy-Office of Nuclear Energy (DOE-NE) programs are exploring the use of these technologies to provide enhanced sensors for irradiation testing. For example, the ability of small diameter ultrasonic thermometers (UTs) to provide a temperature profile in candidate metallic and oxide fuel would provide much needed data for validating new fuel performance models. The National Scientific User Facility (NSUF) is sponsoring a project to evaluate the performance of promising temperature sensors based on ultrasound and on fiber optics during an upcoming irradiation test in the Massachusetts Institute of Technology Research Reactor (MITR). Several types of thin-wire metallic waveguide ultrasonic thermometers will be tested along with fiber optic temperature sensors using regenerated Fiber-Bragg Grating technology. Additionally, samples of several new optical materials which are potentially much more radiation tolerant than commonly used materials, such as silica, will be included and analyzed post-irradiation. The irradiation is a collaborative effort between researchers from Idaho National Laboratory, the French Alternative Energies and Atomic Energy Commission, the University of Pittsburgh, the Massachusetts Institute of Technology, and AFO Research, Inc.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Updated Results of Ultrasonic Transducer Irradiation Test

Ultrasonic technologies offer the potential for high accuracy and resolution in-pile measurement of a range of parameters, including geometry changes, temperature, crack initiation and growth, gas pressure and composition, and microstructural changes. Many Department of Energy-Office of Nuclear Energy (DOE-NE) programs are exploring the use of ultrasonic technologies to provide enhanced sensors for in-pile instrumentation during irradiation testing. For example, the ability of small diameter ultrasonic thermometers (UTs) to provide a temperature profile in candidate metallic and oxide fuel would provide much needed data for validating new fuel performance models. These efforts are limited by the lack of identified ultrasonic transducer materials capable of long term performance under irradiation test conditions. To address this need, the Pennsylvania State University (PSU) was awarded an Advanced Test Reactor National Scientific User Facility (ATR NSUF) project to evaluate the performance of promising magnetostrictive and piezoelectric transducers in the Massachusetts Institute of Technology Research Reactor (MITR) up to a fast fluence of at least 10{sup 21} n/cm{sup 2}. A multi-National Laboratory collaboration funded by the Nuclear Energy Enabling Technologies Advanced Sensors and Instrumentation (NEET-ASI) program also provided initial support for this effort. This irradiation, which started in February 2014, is an instrumented lead test and real-time transducer performance data are collected along with temperature and neutron and gamma flux data. The irradiation is ongoing and will continue to approximately mid-2015. To date, very encouraging results have been attained as several transducers continue to operate under irradiation. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗