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De Rudder, Anne

Publications and source records attributed to De Rudder, Anne.

Ozone reduction in the 1980's - A model simulation of anthropogenic and solar perturbations

An interpretation of global ozone changes deduced from satellite data obtained since 1979 is presented, based on two-dimensional model simulations. The study shows that a depletion in total ozone of the order of 2 percent and a reduction in ozone density near 40 km of 7 to 12 percent over the 1979-1986 period are consistent with the observed increase in trace gas densities (chlorofluorocarbons, methane, nitrous oxide, carbon dioxide) and the simultaneous decrease in solar activity during this period. The model also suggests that ozone variations of solar and anthropogenic origins between 1979 and 1986 were of similar magnitude but that the ozone response to trace gas emissions increases substantially with latitude while the solar signal in ozone is present lower in the atmosphere and is nearly independent of latitude.

Brasseur, Guy↗

The potential impact on atmospheric ozone and temperature of increasing trace gas concentrations

The response of the atmosphere to emission of chlorofluorocarbons and other chlorocarbons and to increasing concentrations of other radiatively active trace gases is calculated using a coupled, one-dimensional, time-dependent chemical-radiative-transport model. The model predicts future changes in the ozone content and in the temperature based on several possible time-dependent scenarios of future atmospheric emissions. The sensitivity of the atmospheric responses to the values adopted for parameters such as the eddy diffusion coefficient for vertical transport and the atmospheric budget of nitrogen oxides is estimated and discussed.

Brasseur, Guy↗

Odd nitrogen during the MAP/GLOBUS 1983 campaign - Theoretical considerations

The paper reviews the chemical processes involved in the formation and destruction of active nitrogen in the stratosphere and indicates that transport processes play an important role in the behavior of these species. Vertical profiles measured during the MAP/GLOBUS 1983 campaign are compared to distributions calculated by a number of one-dimensional models. An intercomparison between six of these models shows that, if some quantitative differences attributed to different model input are noticeable, the same type of behavior is predicted for NO and NO2 by all models. Although the observed concentration of species belonging to the odd nitrogen family should be highly variable, as a result of dynamical disturbances, most data obtained during the campaign appear to be consistent with the chemical scheme currently used in photochemical models.

Brasseur, Guy↗