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DeLand, Matthew

Publications and source records attributed to DeLand, Matthew.

Improvement of Stratospheric Aerosol Extinction Retrieval from OMPS/LP Using a New Aerosol Model

The Ozone Mapping and Profiler Suite Limb Profiler (OMPS/LP) has been flying on the Suomi National Polar-orbiting Partnership (S-NPP) satellite since October 2011. It is designed to produce ozone and aerosol vertical profiles at 2-kilometer vertical resolution over the entire sunlit globe. Aerosol extinction profiles are computed with Mie theory using radiances measured at 675 nanometers. The operational Version 1.0 (V1.0) aerosol extinction retrieval algorithm assumes a bimodal lognormal aerosol size distribution (ASD) whose parameters were derived by combining an in situ measurement of aerosol microphysics with the Stratospheric Aerosol and Gas Experiment (SAGE II) aerosol extinction climatology. Internal analysis indicates that this bimodal lognormal ASD does not sufficiently explain the spectral dependence of LP-measured radiances. In this paper we describe the derivation of an improved aerosol size distribution, designated Version 1.5 (V1.5), for the LP retrieval algorithm. The new ASD uses a gamma function distribution that is derived from Community Aerosol and Radiation Model for Atmospheres (CARMA)-calculated results. A cumulative distribution fit derived from the gamma function ASD gives better agreement with CARMA results at small particle radii than bimodal or unimodal functions. The new ASD also explains the spectral dependence of LP-measured radiances better than the V1.0 ASD. We find that the impact of our choice of ASD on the retrieved extinctions varies strongly with the underlying reflectivity of the scene. Initial comparisons with collocated extinction profiles retrieved at 676 nanometers from the SAGE III instrument on the International Space Station (ISS) show a significant improvement in agreement for the LP V1.5 retrievals. Zonal mean extinction profiles agree to within 10 percent between 19 and 29 kilometers, and regression fits of collocated samples show improved correlation and reduced scatter compared to the V1.0 product. This improved agreement will motivate development of more sophisticated ASDs from CARMA results that incorporate latitude, altitude and seasonal variations in aerosol properties.

Ozone Mapping Profiler Suite Limb Profiler (OMPS/L

Validation of Ozone Profile Retrievals Derived from the OMPS LP Version 2.5 Algorithm Against Correlative Satellite Measurements

The Limb Profiler (LP) is a part of the Ozone Mapping and Profiler Suite launched on board of the Suomi NPP satellite in October 2011. The LP measures solar radiation scattered from the atmospheric limb in ultraviolet and visible spectral ranges between the surface and 80 km. These measurements of scattered solar radiances allow for the retrieval of ozone profiles from cloud tops up to 55 km. The LP started operational observations in April 2012. In this study we evaluate more than 5.5 years of ozone profile measurements from the OMPS LP processed with the new NASA GSFC version 2.5 retrieval algorithm. We provide a brief description of the key changes that had been implemented in this new algorithm, including a pointing correction, new cloud height detection, explicit aerosol correction and a reduction of the number of wavelengths used in the retrievals. The OMPS LP ozone retrievals have been compared with independent satellite profile measurements obtained from the Aura Microwave Limb Sounder (MLS), Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) and Odin Optical Spectrograph and InfraRed Imaging System (OSIRIS). We document observed biases and seasonal differences and evaluate the stability of the version 2.5 ozone record over 5.5 years. Our analysis indicates that the mean differences between LP and correlative measurements are well within required +/- 10% between 18 and 42 km. In the upper stratosphere and lower mesosphere (>43 km) LP tends to have a negative bias. We find larger biases in the lower stratosphere and upper troposphere, but LP ozone retrievals have significantly improved in version 2.5 compared to version 2 due to the implemented aerosol correction. In the northern high latitudes we observe larger biases between 20 and 32 km due to the remaining thermal sensitivity issue. Our analysis shows that LP ozone retrievals agree well with the correlative satellite observations in characterizing vertical, spatial and temporal ozone distribution associated with natural processes, like the seasonal cycle and quasi-biennial oscillations. We found a small positive drift approx. 0.5%/yr in the LP ozone record against MLS and OSIRIS that is more pronounced at altitudes above 35 km. This pattern in the relative drift is consistent with a possible 100m drift in the LP sensor pointing detected by one of our altitude-resolving methods.

Ozone Mapping

The Ozone Monitoring Instrument: Overview of 14 Years in Space

This overview paper highlights the successes of the Ozone Monitoring Instrument (OMI) on board the Aura satellite spanning a period of nearly 14 years. Data from OMI has been used in a wide range of applications and research resulting in many new findings. Due to its unprecedented spatial resolution, in combination with daily global coverage, OMI plays a unique role in measuring trace gases important for the ozone layer, air quality, and climate change. With the operational very fast delivery (VFD; direct readout) and near real-time (NRT) availability of the data, OMI also plays an important role in the development of operational services in the atmospheric chemistry domain.

KNMI

A New Algorithm for Detecting Cloud Height using OMPS/LP Measurements

The Ozone Mapping and Profiler Suite Limb Profiler (OMPS/LP) ozone product requires the determination of cloud height for each event to establish the lower boundary of the profile for the retrieval algorithm. We have created a revised cloud detection algorithm for LP measurements that uses the spectral dependence of the vertical gradient in radiance between two wavelengths in the visible and near-IR spectral regions. This approach provides better discrimination between clouds and aerosols than results obtained using a single wavelength. Observed LP cloud height values show good agreement with coincident Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) measurements.

Chen, Zhong

The Solar Spectral Irradiance as a Function of the Mg II Index for Atmosphere and Climate Modelling

In this paper we present a new method to reconstruct the solar spectrum irradiance in the Ly alpha-400 nm region, and its variability, based on the Mg II index and neutron monitor. Measurements of the solar spectral irradiance available in the literature have been made with different instruments at different times and different spectral ranges. However, climate studies require harmonized data sets. This new approach has the advantage of being independent of the absolute calibration and aging of the instruments. First, the Mg II index is derived using solar spectra from Ly alpha (121 nm) to 410 nm measured from 1978 to 2010 by several space missions. The variability of the spectra with respect to a chosen reference spectrum as a function of time and wavelength is scaled to the derived Mg II index. The set of coefficients expressing the spectral variability can be applied to the chosen reference spectrum to reconstruct the solar spectra within a given time frame or Mg II index values. The accuracy of this method is estimated using two approaches: by direct comparison with particular cases where solar spectra are available from independent measurements, and by calculating the standard deviation between the measured spectra and their reconstruction. From direct comparisons with measurements we obtain an accuracy of about 1 to 2 %, which degrades towards Ly alpha. In a further step, we extend our solar spectral irradiance reconstruction back to the Maunder Minimum introducing the relationship between the Mg II index and the neutron monitor data. Consistent measurements of the Mg II index are not available prior to 1978. However, we observe that over the last three solar cycles, the Mg II index shows strong correlation with the modulation potential determined from the neutron monitor data. Assuming that this correlation can be applied to the past, we reconstruct the Mg II index from the modulation potential back to the Maunder Minimum, and obtain the corresponding solar spectral irradiance reconstruction back to that period. As there is no direct measurement of the spectral irradiance for this period we discuss this methodology in light of the other proposed approaches available in the literature. The use of the cosmogenic isotope data provides a major advantage: it provides information about the solar activity over several thousands years. Using technology of today we can calibrate the solar irradiance against the activity and thus reconstruct it for the times when cosmogenic isotope data are available. This calibration can be re-accessed at any time, if necessary.

Thuillier, Gerard