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Edward Winstead

Publications and source records attributed to Edward Winstead.

Seasonal Updraft Speeds Change Cloud Droplet Number Concentrations in Low Level Clouds Over the Western North Atlantic

To determine the impact of dynamic and aerosol processes on marine low clouds, we examine the seasonal impact of updraft speed w and cloud condensation nuclei concentration at 0.43 % supersaturation () on the cloud droplet number concentration (N(C)) of low-level clouds over the western North Atlantic Ocean. Aerosol and cloud properties were measured with instruments on board the NASA LaRC Falcon HU-25 during the ACTIVATE (Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment) mission in summer (August) and winter (February–March) 2020. The data are grouped into different loadings, and the density functions of NC and w near the cloud bases are compared. For low updrafts (w < 1.3 m s−1), NC in winter is mainly limited by the updraft speed and in summer additionally by aerosols. At larger updrafts (w > 3 m s−1), NC is impacted by the aerosol population, while at clean marine conditions cloud nucleation is aerosol-limited, and for high it is influenced by aerosols and updraft. The aerosol size distribution in winter shows a bimodal distribution in clean marine environments, which transforms to a unimodal distribution in high due to chemical and physical aerosol processes, whereas unimodal distributions prevail in summer, with a significant difference in their aerosol concentration and composition. The increase of is accompanied with an increase of organic aerosol and sulfate compounds in both seasons. We demonstrate that NC can be explained by cloud condensation nuclei activation through upwards processed air masses with varying fractions of activated aerosols. The activation highly depends on w and thus supersaturation between the different seasons, while the aerosol size distribution additionally affects NC within a season. Our results quantify the seasonal influence of w and on NC and can be used to improve the representation of low marine clouds in models.

Simon Kirschler↗

Polarimeter + Lidar–Derived Aerosol Particle Number Concentration

In this study, we propose a simple method to derive vertically resolved aerosol particle number concentration (Na) using combined polarimetric and lidar remote sensing observations. This method relies on accurate polarimeter retrievals of the fine-mode column-averaged aerosol particle extinction cross section and accurate lidar measurements of vertically resolved aerosol particle extinction coefficient such as those provided by multiwavelength high spectral resolution lidar. We compare the resulting lidar + polarimeter vertically resolved N(a) product to in situ N(a) data collected by airborne instruments during the NASA aerosol cloud meteorology interactions over the western Atlantic experiment (ACTIVATE). Based on all 35 joint ACTIVATE flights in 2020, we find a total of 32 collocated in situ and remote sensing profiles that occur on 11separate days, which contain a total of 322 cloud-free vertically resolved altitude bins of 150 m resolution. We demonstrate that the lidar + polarimeter N(a) agrees to within 106% for 90% of the 322 vertically resolved points. We also demonstrate similar agreement to within 121% for the polarimeter-derived column-averaged N(a). We find that the range-normalized mean absolute deviation (NMAD) for the polarimeter-derived column-averaged Na is 21%, and the NMAD for the lidar + polarimeter-derived vertically resolved Na is 16%. Taken together, these findings suggest that the error in the polarimeter-only column-averaged N(a) and the lidar + polarimeter vertically resolved N(a) are of similar magnitude and represent a significant improvement upon current remote sensing estimates of N(a).

RSP↗

TPSAS-NF1676L-30150-DND

Validation of science data products from the Stratospheric Aerosol and Gas Experiment (SAGE) III, installed on the International Space Station (ISS) in March 2017, requires intercomparison with validated data sources. The SAGE III/ISS mission is actively utilizing in-situ profile measurements from balloon packages, consisting of a standard meteorological radiosonde, ozonesonde, and frost-point hygrometer, that were launched coincident with SAGE III/ISS overpass opportunities. Some packages have included an aerosol sonde. This provides regional correlations of ozone, water vapor and aerosol extinction between the in-situ measurement data and the SAGE III/ISS profile products. In addition, ground-based LIDAR measurements and aircraft-based measurements of ozone, water vapor, aerosol extinction and nitrogen dioxide will provide additional validation data for correlation with the SAGE III/ISS data products. Initial results of the mission directed validation program will be presented. When possible, operation and launch times were modified to improve the temporal and spatial coincidence between the measurements. Results and progress utilizing LIDAR and balloon-borne aerosol observations are discussed herein, while intercomparisons that make use of ozone sondes is are presented in the companion poster by Kizer et al.

Travis Knepp↗

Biofuel Blending Reduces Aircraft Engine Particle Emissions at Cruise Conditions

Aviation aerosol emissions have a disproportionately large climatic impact because they are emitted high in the relatively pristine upper troposphere where they can form linear contrails and influence cirrus clouds. Research aircraft from NASA, DLR, and NRC Canada made airborne measurements of gaseous and aerosol composition and contrail microphysical properties behind the NASA DC-8 aircraft at cruise altitudes. The DC-8 CFM-56-2C engines burned traditional medium-sulfur Jet A fuel as well as a low-sulfur Jet A fuel and a 50:50 biofuel blend. Substantial, two-to-three-fold emissions reductions are found for both particle number and mass emissions across the range of cruise thrust operating conditions. These observations provide direct and compelling evidence for the beneficial impacts of biojet fuel blending under real-world conditions.

Richard H Moore↗

TPSAS-NF1676L-22701-DND

The next generation of aerosol satellite instruments will include multi-spectral polarimetric measurements to retrieval aerosol size distribution and refractive index (Hasekamp et al., 2011; NRC, 2007). Refractive index is the “only means of constraining aerosol chemical composition from space” for passive sensors (Mischenko et al., 2007). A number of methods have been developed to derive refractive index from combined optical and electrical mobility sizing instruments (e.g., the “Alignment Method” of Hand and Kreidenweis, 2002). In this work, we evaluate the sensitivity of two, commercially-available, high-resolution optical particle counters for determining the size-resolved refractive index of laboratory-generated aerosols when used with a modified form of the Alignment Method.

Stephen Zimmerman↗

Survey of microphysical properties of marine boundary-layer clouds in the Western North Atlantic

Oceanic low level clouds strongly affect the atmospheric radiation budget. Uncertainties in their microphysical properties and cover currently limit the accuracy of climate predictions. Further, studies quantifying the relative importance of aerosol and dynamics on cloud properties in specific meteorological regimes are poorly constrained by observations in the Western North Atlantic boundary layer. Low level clouds were measured during the Aerosol Cloud meTereology Interactions oVer the western ATlantic Experiment (ACTIVATE) campaign in winter and summer 2020. The two NASA LaRC research aircraft HU-25 Falcon and UC-12 B-200 King Air conducted 35 simultaneous flights to investigate aerosol-cloud interactions of maritime clouds and their impact on radiation. Number concentration, liquid water content, ice water content, and particle size distribution in the size range of 3 µm to 1460 µm in diameter were measured with the fast forward scattering cloud probe (FCDP) and 2-dimensional optical array imaging probe (2D-S) onboard the Falcon. Here, we present an overview of late winter (February-March) and late summer (August-September) oceanic cloud properties in the region 65°W to 80°W and 30°N to 40°N. We compare cloud properties in these two seasons and investigate their dependence on meteorological parameters and aerosol abundance. In a case study, we present cloud observations in a cold air outbreak event on 1 March 2020 with a specific focus on mixed-phase clouds.

microphysical properties↗

Polarimeter + Lidar Derived Aerosol Particle Number Concentration

In this study, we propose a simple method to derive vertically resolved aerosol particle number concentration (Na) using combined polarimetric and lidar remote sensing observations. This method relies on accurate polarimeter retrievals of the fine-mode column-averaged aerosol particle extinction cross section and accurate lidar measurements of vertically resolved aerosol particle extinction coefficient such as those provided by multiwavelength high spectral resolution lidar. We compare the resulting lidar + polarimeter vertically resolved Na product to in situ Na data collected by airborne instruments during the NASA aerosol cloud meteorology interactions over the western Atlantic experiment (ACTIVATE). Based on all 35 joint ACTIVATE flights in 2020, we find a total of 32 collocated in situ and remote sensing profiles that occur on 11 separate days, which contain a total of 322 cloud-free vertically resolved altitude bins of 150 m resolution. We demonstrate that the lidar + polarimeter Na agrees to within 106% for 90% of the 322 vertically resolved points. We also demonstrate similar agreement to within 121% for the polarimeter-derived column-averaged Na. We find that the range-normalized mean absolute deviation (NMAD) for the polarimeter-derived column-averaged Na is 21%, and the NMAD for the lidar + polarimeter-derived vertically resolved Na is 16%. Taken together, these findings suggest that the error in the polarimeter-only column-averaged Na and the lidar + polarimeter vertically resolved Na are of similar magnitude and represent a significant improvement upon current remote sensing estimates of Na.

Aerosol number concentration↗

Three Years of Airborne Observations During NASA Activate: A Statistical Summary of Chemical, Optical, and Microphysical Aerosol Properties Over the Western North Atlantic Ocean

Airborne observations are critical to understanding Earth’s climate system and surface-level air quality by providing both spatial and vertical information that is not possible through ground measurement networks or satellite observations. Airborne platforms allow assessments of long-range transport, vertical redistribution, boundary-layer dynamics, and cloud-aerosol-interactions that are critical to model evaluation and satellite validation. Still, the high cost and effort of aircraft operations can limit measurement campaigns to short, focused time periods. Multiple deployments are often necessary for seasonal comparisons, and results can be limited if target phenomenon are infrequent. Subsequent analyses typically focus on case studies, especially if deployment conditions are climatologically anomalous. The NASA ACTIVATE (Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment) mission was designed to overcome these limitations by operating semi-continuously over multiple months during multiple seasons. Flight plans were intentionally simple, repetitive, and systematic to provide a statistically robust dataset that could be utilized similarly to a ground-network. Here, we present an overview of three years (2020-2022) of aerosol measurements from the NASA HU-25 Falcon aircraft supporting the ACTIVATE mission. Data from 179 flights were considered, the majority of which were based at NASA Langley Research Center and flown locally over the Wester North Atlantic Ocean just east of Hampton, VA, USA. Airmass characteristics tended to transition from continental outflow near the coast to mostly marine over the open ocean. Seasonal, diurnal, spatial, and vertical trends in aerosol microphysical, optical, and chemical properties are discussed in the context of synoptic scale meteorology. Statistical benefits of the ACTIVATE sampling strategy are discussed with regard to future model evaluation.

Luke D Ziemba↗