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Fleming, Eric L.

Publications and source records attributed to Fleming, Eric L..

At least 37 records · Page 2

An Intercomparison of 2-D Models Within a Common Framework

A model intercomparison among the Atmospheric and Environmental Research (AER) 2-D model, the Goddard Space Flight Center (GSFC) 2-D model, and the Lawrence Livermore National Laboratory 2-D model allows us to separate differences due to model transport from those due to the model's chemical formulation. This is accomplished by constructing two hybrid models incorporating the transport parameters of the GSFC and LLNL models within the AER model framework. By comparing the results from the native models (AER and e.g. GSFC) with those from the hybrid model (e.g. AER chemistry with GSFC transport), differences due to chemistry and transport can be identified. For the analysis, we examined an inert tracer whose emission pattern is based on emission from a High Speed Civil Transport (HSCT) fleet; distributions of trace species in the 2015 atmosphere; and the response of stratospheric ozone to an HSCT fleet. Differences in NO(y) in the upper stratosphere are found between models with identical transport, implying different model representations of atmospheric chemical processes. The response of O3 concentration to HSCT aircraft emissions differs in the models from both transport-dominated differences in the HSCT-induced perturbations of H2O and NO(y) as well as from differences in the model represent at ions of O3 chemical processes. The model formulations of cold polar processes are found to be the most significant factor in creating large differences in the calculated ozone perturbations

Weisenstein, Debra K.↗

The Effect of Solar Proton Events on Ozone and Other Constituents in the Middle Atmosphere

Solar proton events (SPEs) can result in increases in both HO(x) (H, OH, HO2) and NO(x) (N, NO, NO2) constituents in the middle atmosphere polar region (>60 degrees geomagnetic). FlO(x) constituents produced by SPEs caused decreases in mesospheric and upper stratospheric ozone observed during several events. Recent SPEs in July and November of 2000 caused ozone decreases of over 30 percent during the event as measured by UARS HALOE and NOAA 14 SBUV/2. These HO(x)-driven ozone depletions last only during the SPEs (several hours to a few days) because of the short lifetimes of HO(x) constituents in the atmosphere. The NO(x) species feed into the entire odd nitrogen family NO(y) (N, NO, NO2, NO3, N2O5, HNO,14NO4, CIONO2, BrONO2) over a period of hours to weeks. The NO(y) family lasts several months or more in the stratosphere with low sun conditions. The two largest SPEs in the past 30 years, October 1989 and August 1972, caused polar stratospheric ozone depletions >10 percent for weeks past the events. The SPE in July 2000, third largest in 30 years, was measured by NOAA 14 SBUV/2 to decrease ozone by several percent for days past the event. Enhancements in mesospheric NO(x) of over 50 ppbv were also measured by UARS HALOE during this event. A review of the influence of SPEs on ozone and other constituents in the middle atmosphere will be given in this talk.

Jackman, Charles H.↗

Two-Dimensional Model Simulations of Interannual Variability in the Tropical Stratosphere

Meteorological data from the United Kingdom Meteorological Office (UKMO) and constituent data from the Upper Atmospheric Research Satellite (UARS) are used to construct yearly zonal mean dynamical fields for the 1990s for use in the GSFC 2-D chemistry and transport model. This allows for interannual dynamical variability to be included in the model constituent simulations. In this study, we focus on the tropical stratosphere. We find that the phase of quasi-biennial oscillation (QBO) signals in equatorial CH4, and profile and total column 03 data is resolved quite well using this empirically- based 2-D model transport framework. However. the QBO amplitudes in the model constituents are systematically underestimated relative to the observations at most levels. This deficiency is probably due in part to the limited vertical resolutions of the 2-D model and the UKMO and UARS input data sets. We find that using different heating rate calculations in the model affects the interannual and QBO amplitudes in the constituent fields, but has little impact on the phase. Sensitivity tests reveal that the QBO in transport dominates the ozone interannual variability in the lower stratosphere. with the effect of the temperature QBO being dominant in the tipper stratosphere via the strong temperature dependence of the ozone loss reaction rates. We also find that the QBO in odd nitrogen radicals, which is caused by the QBO modulated transport of NOy, plays a significant but not dominant role in determining the ozone QBO variability in the middle stratosphere. The model mean age of air is in good overall agreement with that determined from tropical lower,middle stratospheric OMS balloon observations of SF6 and CO2. The interannual variability of tile equatorial mean age in the model increases with altitude and maximizes near 40 km, with a range, of 4-5 years over the 1993-2000 time period.

Fleming, Eric L.↗

Satellite Measured Solar Protons from 1963-1993 and Their Influence on Ozone in a Changing Stratosphere

The fluxes of solar protons have been measured by a series of Interplanetary Monitoring Platform (IMP) satellites since 1963. Eight IMP satellites have been launched since 1963 providing excellent coverage of solar protons with energies from a few MeV to several hundred MeV. IMP 8, launched in October 1973, continues to provide proton measurements, twenty-six and a half (26 1/2) years after launch. These high energy solar protons rain down on the earth's polar atmosphere sporadically, primarily during solar proton events (SPEs) which typically last a few days. Solar protons with energies of 30 MeV or greater are capable of reaching the stratosphere and causing increases in odd nitrogen (NO(y)) constituents at polar latitudes ($>$ 60 degrees geomagnetic) which last for several months to years past the events. These enhanced NO(y) species can lead to significant upper stratospheric ozone depletions $ greater than $10\% during the gigantic SPEs that occurred in August 1972 and October 1989. We studied the effects of SPEs on the stratosphere from 1963 to the mid 1990s. During this time period, the stratospheric chlorine levels changed from relatively small in 1963 ($\sim$ 1 ppbv) to fairly substantial amounts in the mid-1990s ($\sim$ 3.3 ppbv). Our recently improved two-dimensional chemistry and transport atmospheric model was used to compute the effects of SPEs in this changing stratosphere. The long-lived SPE-produced NO(y) constituents were transported to lower stratospheric levels during winter after the events and caused impacts in the middle and lower stratosphere. Generally, the SPEs resulted in a decrease in ozone. However, during periods of high halogen loading these impacts resulted in interference with the chlorine and bromine loss cycles for ozone destruction. This interference actually led to a predicted total ozone increase that was especially notable in the time period 1992-4, a few years after the October 1989 SPE.

Jackman, Charles H.↗

Interannual Variability in the Equatorial Stratosphere: Comparison of 2D Model Simulations with Satellite Constituent Data

Satellite observations from UARS and TOMS have provided unique data sets for studying seasonal and interannual stratospheric constituent variability during the 1990's. The corresponding meteorological variability is also well represented by the partly satellite-based UKMO assimilation winds and temperatures. In this study, we use the UKMO meteorological fields to derive zonal mean transport components (residual circulation, horizontal eddy diffusion) for each year, 1992-1998. These fields are then used in our GSFC two-dimensional chemistry and transport model to simulate the year to year changes in ozone and long lived tracers in the equatorial stratosphere due to interannual dynamical variability. The resulting model simulation of ozone and CH4 compares reasonably well with UARS data in reproducing a dominant QBO signal in the lower stratosphere, and a dominant semiannual signature in the upper stratosphere which appears to be modulated by the lower stratospheric QBO. The model also compares well with TOMS data in simulating the phase of the QBO in total ozone, although the model QBO amplitude is somewhat underestimated relative to TOMS. These comparisons illustrate that the general zonal mean transport characteristics in the equatorial stratosphere can be reasonably well simulated using an empirically-based residual circulation.

Fleming, Eric L.↗

Multi-Satellite Measurements and Model Predictions of Mesospheric and Upper Stratospheric Influences from the Very Large July 14-16, 2000, Solar Proton Event

A large solar flare with an associated coronal mass ejection occurred in mid-July and caused a very large solar proton event at the earth in the time period July 14-16, 2000. So far this is the largest solar storm of solar cycle 23. The solar proton fluxes were measured by instruments aboard the GOES-10 satellite and used in our proton energy deposition model to help quantify the energy input to the middle atmosphere during this large solar event. Using this computed energy deposition in the GSFC 2D atmospheric model resulted in a prediction of $>$ 20\% increases in HO$-(x)$ (H, OH, HO$-(2)$) and $>$ 100\% increases in NO$-(x)$ (N, NO, NO$-(2)$) constituents in the mesosphere and upper stratosphere at polar latitudes ($>$ 60 degrees geomagnetic). Both the HO$-(x)$ and NO$_fx)$ increases impacted ozone. Large atmospheric impacts have been measured with the NOAA 14 SBUV/2 instrument (0$_(3)$), the UARS HALOE instrument (NO, NO$-(2)$, 0$-(3)$), and the POAM III instrument (0$_{3}$, NO$-(2)$). Preliminary analysis indicates that measured (SBUV/2) and modelled 0$_{3}$ decreases from this solar event are generally in agreement in the Northern Hemisphere. Short-term ozone changes (during the event) indicate $\sim$ 15% reduction at 2 hPa ($\sim$ 45 km) up to $\sim$ 40% reduction at 0.5 hPa ($\sim$ 55 km). A longer-term ozone depletion of $\sim$ 5% is indicated between 4 and 2 hPa ($\sim$ 40-45 km). The middle atmospheric changes caused by this solar event were very large and occurred fairly quickly ($\sim$ 1-2 days). Such a significant natural perturbation provides a good test of our understanding of the middle atmosphere. The measured and modelled impacts of this solar event will be compared and discussed in this paper.

Jackman, Charles H.↗

Simulation of Ozone and Long Lived Tracers in the GSFC Two-Dimensional Model

The GSFC two-dimensional transport and chemistry model has been used for a wide variety of scientific and assessment studies of stratospheric ozone. Transport is a key element in the ozone simulations, and we have recently upgraded our model transport formulation to include much of the information about atmospheric transport processes available from existing data sets. To properly evaluate the model transport, it is desirable to examine the effects of transport and photochemistry separately. Recently, high quality observations of several long lived stratospheric tracers have become available from aircraft, balloon, and satellite measurement systems. This data provides a means to do a detailed model transport evaluation, as has been done in the recent Models and Measurements Intercomparison Project II. In this paper, we will discuss the GSFC 2D model simulations of ozone together with model-data comparisons of long lived tracers such as methane and the age of air transport diagnostic. We will show that the model can reproduce many of the transport-sensitive features observed in the stratosphere, and can compare reasonably well with measurements of both total ozone and long lived tracers simultaneously. We will also discuss the model deficiencies in simulating some of the detailed aspects of the observations.

Fleming, Eric L.↗

The Influence of Extremely Large Solar Proton Events in a Changing Stratosphere. Stratospheric Influence of Solar Proton Events

Two periods of extremely large solar proton events (SPEs) occurred in the past thirty years, which forced significant long-term polar stratospheric changes. The August 2-10, 1972 and October 19-27, 1989 SPEs happened in stratospheres that were quite different chemically. The stratospheric chlorine levels were relatively small in 1972 (approximately 1.2 ppbv) and were fairly substantial in 1989 at about (approximately 3 ppbv). Although these SPEs produced both HO(x) and NO(y) constituents in the mesosphere and stratosphere, only the NO(y) constituents had lifetimes long enough to affect ozone for several months to years past the events. Our recently improved two-dimensional chemistry and transport atmospheric model was used to compute the effects of these gigantic SPEs in a changing stratosphere. Significant upper stratospheric ozone depletions > 10% are computed to last for a few months past these SPEs. The long-lived SPE-produced NO(y) constituents were transported to lower levels during winter after these huge SPEs and caused impacts in the middle and lower stratosphere. During periods of high halogen loading these impacts resulted in interference with the chlorine and bromine loss cycles for ozone destruction. The chemical state of the atmosphere, including the stratospheric sulfate aerosol density, substantially affected the predicted stratospheric influence of these extremely large SPEs.

Jackman, Charles H.↗

Influence of Transport on Two-Dimensional Model Simulation. Tracer Sensitivity to 2-D Model Transport: Long Lived Tracers - 1

In this study, we examine the sensitivity of long lived tracers to changes in the base transport components in our 2-D model. Changes to the strength of the residual circulation in the upper troposphere and stratosphere and changes to the lower stratospheric K(sub zz) had similar effects in that increasing the transport rates decreased the overall stratospheric mean age, and increased the rate of removal of material from the stratosphere. Increasing the stratospheric K(sub yy) increased the mean age due to the greater recycling of air parcels through the middle atmosphere, via the residual circulation, before returning to the troposphere. However, increasing K(sub yy) along with self-consistent increases in the corresponding planetary wave drive, which leads to a stronger residual circulation, more than compensates for the K(sub yy)-effect, and produces significantly younger ages throughout the stratosphere. Simulations with very small tropical stratospheric K(sub yy) decreased the globally averaged age of air by as much as 25% in the middle and upper stratosphere, and resulted in substantially weaker vertical age gradients above 20 km in the extratropics. We found only very small stratospheric tracer sensitivity to the magnitude of the horizontal mixing across the tropopause, and to the strength of the mesospheric gravity wave drag and diffusion used in the model. We also investigated the transport influence on chemically active tracers and found a strong age-tracer correlation, both in concentration and calculated lifetimes. The base model transport gives the most favorable overall comparison with a variety of inert tracer observations, and provides a significant improvement over our previous 1995 model transport. Moderate changes to the base transport were found to provide modest agreement with some of the measurements. Transport scenarios with residence times ranging from moderately shorter to slightly longer relative to the base case simulated N2O lifetimes that were within the observational estimates of Volk et al. [1997]. However, only scenarios with rather fast transport rates were comparable with the Volk et al. estimates of CFCl3 lifetimes. This is inconsistent with model-measurement comparisons of mean age in which the base model or slightly slower transport rates compared the most favorably with balloon SF6 data. For all comparisons shown, large transport changes away from the base case resulted in simulations that were outside the range of measurements, and in many cases, far outside this range.

Fleming, Eric L.↗

Effects of Solar Proton Events on the Middle Atmosphere

Solar proton events (SPEs) can result in increases in both HOx (H, OH, HO2) and NOx (N, NO, NO2) constituents in the polar middle atmosphere. Decreases in mesospheric and upper stratospheric ozone caused by HOx constituents produced by SPEs have been observed during several events, however, ozone levels generally recover within a few hours after the end of these events because of the short lifetime of the HOx species. The NOx species feed into the more inclusive odd nitrogen family, NOy (N, NO, NO2, NO3, N2O5, HNO3, HNO4, ClONO2), over a period of hours to weeks. In low sun and lower altitude conditions, the NOy family lasts several months or more in the stratosphere causing prolonged ozone changes over these longer periods. Observations of mesospheric winds during and after SPEs have also indicated some variations as a result of these atmospheric perturbations. An overview of the influence of SPEs on the polar neutral middle atmosphere will be presented in this paper.

Jackman, Charles H.↗

Influence of Transport on Two-Dimensional Model Simulation: 2. Stratospheric Aircraft Perturbations: Stratospheric Aircraft Perturbations - 2

We have adopted the transport scenarios used in Part 1 to examine the sensitivity of stratospheric aircraft perturbations to transport changes in our 2-D model. Changes to the strength of the residual circulation in the upper troposphere and stratosphere and changes to the lower stratospheric K(sub zz) had similar effects in that increasing the transport rates decreased the overall stratospheric residence time and reduced the magnitude of the negative perturbation response in total ozone. Increasing the stratospheric K(sub yy) increased the residence time and enhanced the global scale negative total ozone response. However, increasing K(sub yy) along with self-consistent increases in the corresponding planetary wave drive, which leads to a stronger residual circulation, more than compensates for the K(sub yy)-effect, and results in a significantly weaker perturbation response, relative to the base case, throughout the stratosphere. We found a relatively minor model perturbation response sensitivity to the magnitude of K(sub yy) in the tropical stratosphere, and only a very small sensitivity to the magnitude of the horizontal mixing across the tropopause and to the strength of the mesospheric gravity wave drag and diffusion. These transport simulations also revealed a generally strong correlation between passive NO(sub y) accumulation and age of air throughout the stratosphere, such that faster transport rates resulted in a younger mean age and a smaller NO(y) mass accumulation. However, specific variations in K(sub yy) and mesospheric gravity wave strength exhibited very little NO(sub y)-age correlation in the lower stratosphere, similar to 3-D model simulations performed in the recent NASA "Models and Measurements" II analysis. The base model transport, which gives the most favorable overall comparison with inert tracer observations, simulated a global/annual mean total ozone response of -0.59%, with only a slightly larger response in the northern compared to the southern hemisphere. For transport scenarios which gave tracer simulations within some agreement with measurements, the annual/globally averaged total ozone response ranged from -0.45% to -0.70%. Our previous 1995 model exhibited overly fast transport rates, resulting in a global/annually averaged perturbation total ozone response of -0.25%, which is significantly weaker compared to the 1999 model. This illustrates how transport deficiencies can bias model simulations of stratospheric aircraft.

Fleming, Eric L.↗

Simulation of Long Lived Tracers Using an Improved Empirically-Based Two-Dimensional Model Transport Algorithm

We have developed a new empirically-based transport algorithm for use in our GSFC two-dimensional transport and chemistry assessment model. The new algorithm contains planetary wave statistics, and parameterizations to account for the effects due to gravity waves and equatorial Kelvin waves. We will present an overview of the new algorithm, and show various model-data comparisons of long-lived tracers as part of the model validation. We will also show how the new algorithm gives substantially better agreement with observations compared to our previous model transport. The new model captures much of the qualitative structure and seasonal variability observed methane, water vapor, and total ozone. These include: isolation of the tropics and winter polar vortex, the well mixed surf-zone region of the winter sub-tropics and mid-latitudes, and the propagation of seasonal signals in the tropical lower stratosphere. Model simulations of carbon-14 and strontium-90 compare fairly well with observations in reproducing the peak in mixing ratio at 20-25 km, and the decrease with altitude in mixing ratio above 25 km. We also ran time dependent simulations of SF6 from which the model mean age of air values were derived. The oldest air (5.5 to 6 years) occurred in the high latitude upper stratosphere during fall and early winter of both hemispheres, and in the southern hemisphere lower stratosphere during late winter and early spring. The latitudinal gradient of the mean ages also compare well with ER-2 aircraft observations in the lower stratosphere.

Fleming, Eric L.↗

Recent trends in ozone in the upper stratosphere: Implications for chlorine chemistry

We have studied the implications of recent trends in the annual mean and the amplitude of the annual harmonic of ozone in the upper stratosphere from the 15 years of the combined data from the Nimbus-7 SBUV and the NOAA-11 SBUV/2 instruments. This was done in the context of the GSFC 2D model predictions of these trends which are based on plausible scenarios of anthropogenic Cly increase in the atmosphere. The comparison of the observed and model-estimated annual mean ozone trends show some similarity in their latitude and altitude characteristics. Both the model and data show a maximum ozone decrease of -6 to -10 % per decade at high latitudes in the upper stratosphere. However, there are also significant differences between the observed and computed trends which may be related to both the model uncertainty and the uncertainty in correcting for the long term instrument drift. The observations also suggest a decrease of 10-25 % per decade in the annual amplitude of ozone at 2 mb between 40 deg - 60 deg in both hemispheres, with a relatively larger interannual variability in the northern hemisphere. These values are in general agreement with the model predictions and thus provide additional support in favor of the chlorine induced changes in ozone in the upper stratosphere.

Chandra, Sushil↗

The middle atmospheric response to short and long term solar UV variations: analysis of observations and 2D model results

We have investigated the middle atmospheric response to the 27-day and 11-yr solar UV flux variations at low to middle latitudes using a two-dimensional photochemical model. The model reproduced most features of the observed 27-day sensitivity and phase lag of the profile ozone response in the upper stratosphere and lower mesosphere, with a maximum sensitivity of +0.51% per 1% change in 205 nm flux. The model also reproduced the observed transition to a negative phase lag above 2 mb, reflecting the increasing importance with height of the solar modulated HO(x) chemistry on the ozone response above 45 km. The model revealed the general anti-correlation of ozone and solar UV at 65-75 km, and simulated strong UV responses of water vapor and HO(x) species in the mesosphere. Consistent with previous 1D model studies, the observed upper mesospheric positive ozone response averaged over +/- 40 was simulated only when the model water vapor concentrations above 75 km were significantly reduced relative to current observations. In agreement with observations, the model computed a low to middle latitude total ozone phase lag of +3 days and a sensitivity of +0.077% per 1% change in 205 nm flux for the 27-day solar variation, and a total ozone sensitivity of +0.27% for the 11-yr solar cycle. This factor of 3 sensitivity difference is indicative of the photochemical time constant for ozone in the lower stratosphere which is comparable to the 27-day solar rotation period but is much shorter than the 11-yr solar cycle.

Fleming, Eric L.↗

Chlorine catalyzed destruction of ozone - Implications for ozone variability in the upper stratosphere

The annual mean and the annual amplitude of ozone have been derived from ozone measurements from the SBUV and SBUV/2 spectrometers on board the Nimbus-7 and NOAA-11 satellites. These values differ significantly from values calculated using a two-dimensional model of stratospheric photochemistry and dynamics with standard chemistry. We have found that the differences between the calculated and data-derived values are considerably improved by changing the partitioning in the Cly family to create a larger reservoir of HCl and reducing ClO. This is accomplished by including a channel for the products HCl + O2 from the reaction ClO + OH in addition to the products Cl + HO2. This partitioning also improves the agreement between the calculated and measured values of ClO/HCl ratio.

Chandra, Sushil↗

Monthly mean global climatology of temperature, wind, geopotential height and pressure for 0-120 km

This paper presents a monthly mean climatology of zonal mean temperature, zonal wind, and geopotential height with nearly pole-to-pole coverage (80 deg S-80 deg N) for 0-120 km which can be used as a function of altitude and pressure. This climatology reproduces most of the characteristic features of the atmosphere such as the lowering and cooling of the mesopause and the lowering and warming of the stratopause during the summer months at high latitudes. A series of zonal wind profiles is also presented comparing this climatological wind with monthly mean climatological direct wind measurements in the upper mesosphere and lower thermosphere. The two data sets compare well below 80 km, with some general seasonal trend agreement observed above 80 km. The zonal wind at the equator presented here simulates the observed features of the semiannual oscillation in the upper stratosphere and mesosphere.

Chandra, Sushil↗

Zonal mean temperature, pressure, zonal wind and geopotential height as functions of latitude

The new zonal mean COSPAR International Reference Atmosphere (CIRA-86) of temperature, zonal wind, and geopotential/geometric height is presented. This data can be used as a function of altitude or pressure and has nearly pole-to-pole coverage (80 deg S - 80 deg N) extending from the ground to approximately 120 km. Data sources and methods of computation are described; in general, hydrostatic and thermal wind balance are maintained at all levels and latitudes. As shown by a series of cross sectional plots, the new CIRA accurately reproduces most of the characteristic features of the atmosphere such as the equatorial wind and the general structure of the tropopause, stratopause, and mesopause.

Fleming, Eric L.↗

Equatorial zonal wind in the middle atmosphere derived from geopotential height and temperature data

This paper examines the feasibility of deriving the zonal wind at the equator using mean temperature and geopotential height data from satellite and radiosonde/rocketsonde measurements. Using climatological data of the stratosphere and mesosphere based on monthly mean Nimbus 5 Selective Chopper Radiometer and Nimbus 6 Pressure Modulator Radiometer measurements, and stratospheric monthly mean data from the National Meteorological Center for 1979-1986, meridional cross sections and time profiles of the zonal wind in the tropical middle atmosphere are presented. The derived zonal wind at the equator reproduces the mean climatology of the tropical middle atmosphere as well as the general characteristics of the equatorial quasi-biennial (QBO) and semiannual oscillations (SAO) observed in monthly mean radiosonde and rocketsonde data. Although the amplitude of the derived wind QBO is for the most part underestimated relative to direct-wind measurements, the amplitude of the derived wind SAO compares fairly well with rocketsonde observations.

Fleming, Eric L.↗