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Friedl, R.

Publications and source records attributed to Friedl, R..

Development of a thermal gradient cloud condensation nucleus spectrometer

Droplet clouds are one of the most important factors controlling the albedo and hence the temperature of out planet. Anthropogenic aerosols, such as black carbon (BC) organic carbon (OC) and sulfate, have a strong influence on cloud albedo. IPCC (2001) has estimated the global mean forcing from aerosols to be potentially as large as that of green house gases but opposite in sign. However, the uncertainties associated with the indirect aerosol forcing preclude a quantitative estimate. An additional impact on the indirect aerosol forcing, not quantified by IPCC, arises from recently identified chemical factors, for examples, interactions of atmospheric soluble gases, slightly soluble solutes, and organic substance with aerosols, which may influence the formation of cloud droplets. Recent studies suggest that inclusion of chemical effects on aerosol droplets. We plan to conduct several critical laboratory experiments that will reduce the uncertainty associated with indirect radiative forcing due to chemical modification of sulfate and BC aerosols by ambient gases.

organic carbon↗

Measurements of Aged Aircraft Exhaust in the ACCENT Mission

The Atmospheric Chemistry of Combustion Emissions Near the Tropopause (ACCENT) mission is a multi-agency sponsored effort to evaluate the roles of aircraft and rocket exhaust in perturbing ozone chemistry and modifying aerosols and clouds.

Atmosphere Chemistry Aviation Impacts↗

Unraveling Aircraft Impacts

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atmospheric chemistry aircraft emissions ozone che↗

The Production of NO subscript 2 from the Photolysis of Peroxyacetyl Nitrate

PAN vapor was photolyzed at 248 nm and the NO subscript 2 photoproduct was detected by laser induced fluorescence (LIF). By comparison to the NO subscript 2 production from the photolysis of HNO subscript 3 under identical experimental conditions, we have obtained a relative quantum yield for the production of NO subscript 2. The implications of these results for atmospheric PAN chemistry will be discussed.

Peroxyacetyl nitrate fluorescence↗