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Gray, S. K.

Publications and source records attributed to Gray, S. K..

9 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Optical detection and storage of entanglement in plasmonically coupled quantum-dot qubits

Recent proposals and advances in quantum simulations, quantum cryptography, and quantum communications substantially rely on quantum entanglement formation. Contrary to the conventional wisdom that dissipation destroys quantum coherence, coupling with a dissipative environment can also generate entanglement. We consider a system composed of two quantum-dot qubits coupled with a common, damped surface plasmon mode; each quantum dot is also coupled to a separate photonic cavity mode. Cavity quantum electrodynamics calculations show that upon optical excitation by a femtosecond laser pulse, entanglement of the quantum-dot excitons occurs, and the time evolution of the g (2) pair correlation function of the cavity photons is an indicator of the entanglement. We also show that the degree of entanglement is conserved during the time evolution of the system. Furthermore, if coupling of the photonic cavity and quantum-dot modes is large enough, the quantum-dot entanglement can be transferred to the cavity modes to increase the overall entanglement lifetime. This latter phenomenon can be viewed as a signature of entangled, long-lived quantum-dot exciton-polariton formation. In conclusion, the preservation of total entanglement in the strong-coupling limit of the cavity-quantum-dot interactions suggests a novel means of entanglement storage and manipulation in high-quality optical cavities.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2017

Cooling a Mechanical Resonator with Nitrogen-Vacancy Centres Using a Room Temperature Excited State Spin-Strain Interaction

Cooling a mechanical resonator mode to a sub-thermal state has been a long-standing challenge in physics. This pursuit has recently found traction in the field of optomechanics in which a mechanical mode is coupled to an optical cavity. An alternate method is to couple the resonator to a well-controlled two-level system. Here we propose a protocol to dissipatively cool a room temperature mechanical resonator using a nitrogen-vacancy centre ensemble. The spin ensemble is coupled to the resonator through its orbitally-averaged excited state, which has a spin-strain interaction that has not been previously studied. We experimentally demonstrate that the spin-strain coupling in the excited state is 13.5 ± 0.5 times stronger than the ground state spin-strain coupling. Lastly, we then theoretically show that this interaction, combined with a high-density spin ensemble, enables the cooling of a mechanical resonator from room temperature to a fraction of its thermal phonon occupancy.

36 MATERIALS SCIENCE↗
DOE OSTI2016

Nano-optical imaging of WS e 2 waveguide modes revealing light-exciton interactions

We report on a nano-optical imaging study of WSe 2 thin flakes with scanning near-field optical microscopy (NSOM). The NSOM technique allows us to visualize in real space various waveguide photon modes inside WSe 2 . By tuning the excitation laser energy, we are able to map the entire dispersion of these waveguide modes both above and below the A exciton energy of WSe 2 . We found that all the modes interact strongly with WSe 2 excitons. The outcome of the interaction is that the observed waveguide modes shift to higher momenta right below the A exciton energy. At higher energies, on the other hand, these modes are strongly damped due to adjacent B excitons or band-edge absorptions. Lastly, the mode-shifting phenomena are consistent with polariton formation in WSe 2 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2012

Inhomogeneous dephasing masks coherence lifetimes in ensemble measurements

An open question at the forefront of modern physical sciences is what role, if any, quantum effects may play in biological sensing and energy transport mechanisms. One area of such research concerns the possibility of coherent energy transport in photosynthetic systems. Spectroscopic evidence of long-lived quantum coherence in photosynthetic light-harvesting pigment protein complexes (PPCs), along with theoretical modeling of PPCs, has indicated that coherent energy transport might boost efficiency of energy transport in photosynthesis. Accurate assessment of coherence lifetimes is crucial for modeling the extent to which quantum effects participate in this energy transfer, because such quantum effects can only contribute to mechanisms proceeding on timescales over which the coherences persist. While spectroscopy is a useful way to measure coherence lifetimes, inhomogeneity in the transition energies across the measured ensemble may lead to underestimation of coherence lifetimes from spectroscopic experiments. Theoretical models of antenna complexes generally model a single system, and direct comparison of single system models to ensemble averaged experimental data may lead to systematic underestimation of coherence lifetimes, distorting much of the current discussion. In this study, we use simulations of the Fenna-Matthews-Olson complex to model single complexes as well as averaged ensembles to demonstrate and roughly quantify the effect of averaging over an inhomogeneous ensemble on measured coherence lifetimes. We choose to model the Fenna-Matthews-Olson complex because that system has been a focus for much of the recent discussion of quantum effects in biology, and use an early version of the well known environment-assisted quantum transport model to facilitate straightforward comparison between the current model and past work. Although ensemble inhomogeneity is known to lead to shorter lifetimes of observed oscillations (simply inhomogeneous spectral broadening in the time domain), this important fact has been left out of recent discussions of spectroscopic measurements of energy transport in photosynthesis. In general, these discussions have compared single-system theoretical models to whole-ensemble laboratory measurements without addressing the effect of inhomogeneous dephasing. Our work addresses this distinction between single system and ensemble averaged observations, and shows that the ensemble averaging inherent in many experiments leads to an underestimation of coherence lifetimes in individual systems.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗