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Haas, Derek A.

Publications and source records attributed to Haas, Derek A..

At least 19 records

Seismic DAS observations of a large underground chemical explosion in dry tuff

On 18 October 2023 a 16.3-ton TNT equivalent chemical explosion was detonated underground at the Nevada National Security Site, generating a seismic event with a magnitude of 1.7 (Meyers et al., 2024). The associated seismic wavefield was measured on a Distributed Acoustic Sensing (DAS) array with slant range distances from 27 m – 1123 m. The first arriving phase traveled at an apparent velocity of about 2640 m s -1 from 27 m to 420 m slant range and about 2470 m s -1 from 505 m to 1123 m slant range according to the first arrival moveouts on the DAS data. The first arrival from the explosion temporarily saturated the cable from a slant range of 27 m – 186 m and 0.009 s to 0.084 s post detonation. From 186 m slant range to 420 m slant range, peak strain rates of 5.6 x 10 6 nm m -1 s -1 were observed for the first arrival phase. For the first arrival from 505 m slant range to 1123 m slant range, peak strain rates reduced to 8.0 x 104 nm m -1 s -1 . A comparison of the scaled accelerations computed from DAS, the geophone pairs, and the measurements of co-located accelerometer pairs show common agreement at the scaled ranges of the single point sensors. This study adds to the body of work reporting near-source DAS observations of the seismic wavefields generated by underground chemical explosions. These results indicate that near-source DAS observations can refine interpretations of phase identification from single-point sensor observations. Phase identification could be one mechanism that contributes scatter to single point seismic measurements which would confound the performance of empirical relationships for small explosions. Removing that mechanism may therefore reduce interstation variability and increase empirical relationship performance for small explosions.

58 GEOSCIENCES↗

Low Yield Nuclear Monitoring Physics Experiment 1 – Integrated Data Acquisition System Design and Initial Observations

The report documents the design of the Integrated Data AcQuisition (IDAQ) system and observations recorded during the first in a series of underground chemical explosions conducted on the Nevada National Security Site (NNSS) in southern Nevada. Experiments are funded as part of Low Yield Nuclear Monitoring (LYNM) research and development within the United States National Nuclear Security Administration NA-22 nuclear non-proliferation program. The series is part of the broader Physical Experiment 1 (PE1) being conducted in and around the P-tunnel facility on the NNSS. Each explosive experiment utilizes several tons of comp-B to generate signals recorded by a broad suite of instrumentation. The IDAQ serves as the backbone for all subsurface instrumentation providing precise time synchronization, remote control, data exfiltration and backup, along with recording several sensing modalities throughout the underground complex that includes ground motion, environmental conditions, and electromagnetic signals.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

In the nuclear explosion monitoring context, what is an anomaly?

Abstract In the early years of nuclear explosion monitoring, experts used downwind detections with meaningful ratios of radioactive species to identify an explosion. Today’s reality is sparse networks of radionuclide monitoring stations looking for weak signals. Analysts need to discriminate between industrial background radioactivity and nuclear explosion signals, even using the detection of one isotope. Aerosol and xenon measurements potentially related to nuclear tests in 2006 and 2013 announced by the Democratic People’s Republic of Korea and from worldwide civilian background radioactivity are considered when defining radionuclide detection anomalies to objectively guide the use of limited analyst resources and reduce the possibility of not detecting nuclear explosions.

Miley, Harry S.↗

Cryogenic tracer irradiation facility at the university of Texas at Austin

We report on a cryogenic gas irradiation facility in the 1.1 MW TRIGA reactor at The University of Texas at Austin. The system was designed to produce radioactive xenon and argon for environmental studies, and it can be applied to produce other gaseous radiotracers. The system design includes modeling accident scenarios to ensure operation does not risk damage to the reactor and minimizes risk of release of radioactive material. In conclusion, the SCALE code was used to model a 30-day irradiation of one liter of Xe-126 and the predicted activity is 0.9 Ci of Xe-127 at irradiation end.

Ar-37↗

Modeling the use of mobile modular gas samplers in near-field detection

The Wireless Independent Noble Gas Sampler (WINGS) is a mobile, modular gas sampling system designed for use in low infrastructure environments. In the case of a suspected underground nuclear explosion (UNE), WINGS units could be deployed to detect noble gases emanating from the suspected explosion site or identify gases originating from another source entering the local area from offsite. In conclusion, this work uses the atmospheric transport modeling tool inline WRF-HYSPLIT to test the effectiveness of WINGS units around a suspected UNE site as a function of sampler density and distance from the emission point of gases from a UNE.

Air sampling↗

Survey of Additive Manufacturing Signatures for the Prevention of Nuclear Proliferation

Improvements in additive manufacturing technologies will enable multiple-material and advanced material capabilities, creating opportunities to improve and expand the nuclear fuel fabrication process. Additive manufacturing can allow fuel to have complex geometries and contain composites of materials that would otherwise be difficult or impossible to make with traditional manufacturing methods. This opportunity also has implications for nuclear proliferation, as nuclear parts may be printed and more easily acquired. Here, we present a survey of additive manufacturing technologies and relevant signatures that could be used to identify processes, materials, or part properties.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Adsorption of Tracer Gases in Geological Media: Experimental Benchmarking

The interaction of xenon with containment barriers can play a crucial role in the detection of underground nuclear explosions. Independent field experiments and laboratory-derived models have observed depressed surface level xenon concentrations and subsequently predicted geological capture rates. This work sought to experimentally verify those predictions by analyzing xenon transport though a two-bulb diffusion apparatus adapted for the study of geologic media. Novel to this work is the timescale over which these experiments were carried out, allowing the system to reach equilibrium, rather than relying on numerical models to treat the equilibrium concentration of each gas as a fit coefficient.

Byers, Maggie↗

Study of Shadowing in Beta-Gamma Coincidence Plots for Radioxenon

This document describes a study of the cause of shadowing observed in certain beta-gamma plots produced with beta-gamma coincidence detectors for detection of radioxenon. Beta-gamma detectors must possess adequate resolution to allow for the metastable isotopes 131m Xe and 133m Xe to be distinguished from each other and from 133 Xe. One effect that can minimize the ability to distinguish the metastables from 133 Xe is the shadowing effect, in which a band of high-energy signal is present in addition to the primary signal. A study was performed to determine the cause of the shadowing, and how to minimize the effect of the shadowing on an individual beta cell. Through this study, it is determined that the shadowing results from a difference in light transmission between the dome and end-cap portions of the beta cell. Consequently, it is not possible to remove the shadowing during the beta cell manufacturing process. The shadowing must be minimized by preferentially matching the light output from the end-cap and dome portion prior to the manufacturing process.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Requirements for Xenon International (Rev. 2)

This document defines the requirements for the new Xenon International radioxenon system. The output of this project will be a Pacific Northwest National Laboratory (PNNL) developed prototype and a manufacturer-developed production prototype. The two prototypes are intended to be as close to matching as possible; this will be facilitated by overlapping development cycles and open communication between PNNL and the manufacturer.

61 RADIATION PROTECTION AND DOSIMETRY↗

Adsorptive Transport of Noble Gas Tracers in Porous Media

The transport of noble gas radionuclides in porous media is relevant to the detection of underground nuclear detonations as well as the sequestration of reprocessing off-gases. However, in field tests releasing radioxenon underground, the quantity of radioxenon observed at the surface has fallen well below expectations1. This study examined the diffusivity of noble gases (Kr and Xe) and the inert molecular gas sulfur hexafluoride (SF6) in porous media to observe any unexpected behavior. To replicate the transport of radiogenic noble gases in underground media, a two-bulb gaseous diffusion apparatus was constructed. The two bulbs are connected with a column of 10-30 Ottawa sand and ordinary atmosphere filled both the bulbs and pore spaces. The tracer gases were diluted in an isolated bulb to approximately 1000 ppm. Once released, the gases were allowed to diffuse through the column. Aliquots were withdrawn at regular time intervals from both bulbs and concentrations were quantified using a Shimadzu QP2010 SE gas chromatograph-mass spectrometer. The effective diffusivity was then calculated using a maximum likelihood estimate on the quasi-steady state model.

Paul, Matthew R.↗

Improved performance comparisons of radioxenon systems for low level releases in nuclear explosion monitoring

The Comprehensive Nuclear-Test-Ban Treaty bans all nuclear tests and mandates development of verification measures to detect treaty violations. One verification measure is detection of radioactive xenon isotopes produced in the fission of actinides. The International Monitoring System (IMS) currently deploys automated radioxenon systems that can detect four radioxenon isotopes. Radioxenon systems with lower detection limits are currently in development. Historically, the sensitivity of radioxenon systems was measured by the minimum detectable concentration for each isotope. In this paper we analyze the response of radioxenon systems using rigorous metrics in conjunction with hypothetical representative releases indicative of an underground nuclear explosion instead of using only minimum detectable concentrations. Our analyses incorporate the impact of potential spectral interferences on detection limits and the importance of measuring isotopic ratios of the relevant radioxenon isotopes in order to improve discrimination from background sources particularly for low-level releases. To provide a sufficient data set for analysis, hypothetical representative releases are simulated every day from the same location for an entire year. The performance of three types of samplers are evaluated assuming they are located at 15 IMS radionuclide stations in the region of the release point. The performance of two IMS-deployed samplers and a next-generation system is compared with proposed metrics for detection and discrimination using representative releases from the nuclear test site used by the Democratic People’s Republic of Korea.

Haas, Derek A.↗

Development of a Low-Level Ar-37 Calibration Standard

Argon-37 is an important environmental signature of an underground nuclear explosion. Producing and quantifying low-level 37Ar standards is an important step in the development of sensitive field measurement instruments for use during an On-Site Inspection, a key provision of the Comprehensive Nuclear-Test-Ban Treaty. This paper describes progress at Pacific Northwest National Laboratory (PNNL) in the development of a process to generate and quantify low-level 37Ar standard material, which can then be used to calibrate sensitive field systems at activities consistent with soil background levels. The 37Ar used for our work was generated using a laboratory-scale, high-energy neutron source to irradiate powdered samples of calcium carbonate. Small aliquots of 37Ar were then extracted from the head space of the irradiated samples. The specific activity of the head space samples, mixed with P10 (90% stable argon:10% methane by mole fraction) count gas, is then derived using the accepted Length-Compensated Internal-Source Proportional Counting method. Due to the low activity of the samples, a set of three Ultra-Low Background Proportional-Counters designed and fabricated at PNNL from radio-pure electroformed copper was used to make the measurements in PNNL’s shallow underground counting laboratory. Very low background levels (<10 counts/day) have been observed in the spectral region near the 37Ar emission feature at 2.8 keV. Two separate samples from the same irradiation were measured. The first sample was counted for 12 days beginning 28 days after irradiation, the second sample was counted for 24 days beginning 70 days after irradiation (the half-life of 37Ar is 35.0 days). Both sets of measurements were analyzed and yielded very similar results for the starting activity (~0.1 Bq) and activity concentration (0.15 mBq/ccSTP argon) after P10 count gas was added. A detailed uncertainty model was developed based on the ISO Guide to the Expression of Uncertainty in Measurement. This paper presents a discussion of the measurement analysis, along with assumptions and uncertainty estimates.

Absolute radiation measurement↗

Noble Gas Migration Experiment to Support the Detection of Underground Nuclear Explosions

A Noble Gas Migration Experiment (NGME) funded by the National Center for Nuclear Security and conducted at the Nevada National Security Site (NNSS) in collaboration with Lawrence Livermore national Laboratory and National Security Technology provided critical on-site inspection (OSI) information related to the detection of an underground nuclear explosion (UNE) event using noble gas signatures.

Underground nuclear explosion, Explosion cavity, O↗

Radioxenon detector calibration spike production and delivery systems

Abstract Beta-Gamma coincidence radioxenon detectors must be calibrated for each of the four-radioxenon isotopes (135Xe, 133Xe, 133mXe, and 131mXe). Without a proper calibration, there is potential for the misidentification of the amount of each isotope detected. It is important to accurately determine the amount of each radioxenon isotope, as the ratios can be used to distinguish between an anthropogenic source and a nuclear explosion. We have developed a xenon calibration system (XeCalS) that produces calibration spikes of known activity and pressure for field calibration of detectors. The activity concentrations of these calibration spikes are measured using a beta-gamma coincidence detector and a high purity germanium (HPGe) detector. We will present the results from the development and commissioning of XeCalS, along with the future plans for a portable spike implementation system.

beta-gamma coincidence detector↗

Requirements for Xenon International

This document defines the requirements for the new Xenon International radioxenon system. The output of this project will be a Pacific Northwest National Laboratory (PNNL) developed prototype and a manufacturer-developed production prototype. The two prototypes are intended to be as close to matching as possible; this will be facilitated by overlapping development cycles and open communication between PNNL and the manufacturer.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗