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Harris, S. E.

Publications and source records attributed to Harris, S. E..

At least 19 records

Spontaneous Raman scattering as a high-resolution XUV radiation source

A type of high resolution XUV radiation source is described which is based upon spontaneous anti-Stokes scattering of tunable incident laser radiation from atoms excited to metastable levels. The theory of the source is summarized and two sets of experiments using He (1s2s)(1)S atoms, produced in a CW hollow cathode and in a pulsed high power microwave discharge, are discussed. The radiation source is used to examine transitions originating from the 3p(6) shell of potassium. The observed features include four previously unreported absorption lines and several sharp interferences of closely spaced autoionizing lines. A source linewidth of about 1.9 cm(-1) at 185,000 cm(-1) is demonstrated. Previously announced in STAR as N83-18422

Rothenberg, J. E.

Studies on lasers and laser devices

The goal of this grant was to study lasers, laser devices, and uses of lasers for investigating physical phenomena are studied. The active projects included the development of a tunable, narrowband XUV light source and its application to the spectroscopy of core excited atomic states, and the development of a technique for picosecond time resolution spectroscopy of fast photophysical processes.

Harris, S. E.

Spontaneous Raman scattering as a high resolution XUV radiation source

A type of high resolution XUV radiation source is described which is based upon spontaneous anti-Stokes scattering of tunable incident laser radiation from atoms excited to metastable levels. The theory of the source is summarized and two sets of experiments using He (1s2s)(1)S atoms, produced in a cw hollow cathode and in a pulsed high power microwave discharge, are discussed. The radiation source is used to examine transitions originating from the 3p(6) shell of potassium. The observed features include four previously unreported absorption lines and several sharp interferences of closely spaced autoionizing lines. A source linewidth of about 1.9 cm(-1) at 185,000 cm(-1) is demonstrated.

Rothenberg, J. E.

Measurement of the line-of-sight velocity of high-altitude barium clouds A technique

It is demonstrated that for maximizing the scientific output of future ionospheric and magnetospheric ion cloud release experiments a new type of instrument is required which will measure the line-of-sight velocity of the ion cloud by the Doppler technique. A simple instrument was constructed using a 5-cm diam solid Fabry-Perot etalon coupled to a low-light-level integrating TV camera. It was demonstrated that the system has both the sensitivity and spectral resolution for detection of ion clouds and measurement of their line-of-sight Doppler velocity. The tests consisted of (1) a field experiment using a rocket barium cloud release to check sensitivity, and (2) laboratory experiments to show the spectral resolving capabilities of the system. The instrument was found to be operational if the source was brighter than approximately 1 kR, and it had a wavelength resolution much better than 0.2 A, which corresponds to approximately 12 km/sec or in the case of barium ion an acceleration potential of 100 V. The instrument is rugged and, therefore, simple to use in field experiments or on flight instruments. The sensitivity limit of the instrument can be increased by increasing the size of the etalon.

Mende, S. B.

Laser techniques for spectroscopy of core-excited atomic levels

We discuss three techniques which allow the use of tunable lasers for high resolution and picosecond time scale spectroscopy of core-excited atomic levels. These are: anti-Stokes absorption spectroscopy, laser induced emission from metastable levels, and laser designation of selected core-excited levels.

Harris, S. E.

High-resolution extreme-ultraviolet spectroscopy of potassium using anti-Stokes radiation

The use of a new extreme-ultraviolet radiation source based on spontaneous anti-Stokes scattering for high-resolution absorption spectroscopy of transition originating from the 3p6 shell of potassium is reported. The region from 546.6 to 536.8 A is scanned at a resolution of about 1.2 Kayser. Within this region, four previously unreported lines are observed.

Rothenberg, J. E.

Anti-Stokes scattering as an XUV radiation source

Harris (1977) has shown that laser induced scattering from atoms stored in a metastable level may be used to produce an XUV radiation source with several unique properties, including narrow linewidth, tunability, linear polarization, picosecond pulsewidth, and relatively high peak spectral brightness. The present investigation provides a summary concerning the progress made on the use of this radiation source as a unique instrument for XUV spectroscopy, and as a possible flashlamp for a 200 A laser. Zych et al. (1978) demonstrated that the maximum spectral brightness of the source is that of a blackbody with a temperature of the metastable storage level. The peak count rate and peak spectral brightness of the anti-Stokes emission at 569 A are 17 times and 139 times greater than those of the 584 A resonance line. The anti-Stokes process was employed as an external source of radiation for high resolution spectroscopy of the 3p6 shell of potassium. Attention is also given to emission spectroscopy of lithium, metastable levels which are appropriate for storage, and a hollow cathode discharge.

Harris, S. E.

Studies of laser and laser devices

The generation of tunable, infrared, and ultraviolet light, and the control of this light by mode-locking and modulation techniques are discussed. Particular emphasis is given to energy storage and extraction using atomic levels, the development of a tunable narrowband vacuum ultraviolet light source, and to the generation and applications of ultrashort optical pulses.

Harris, S. E.

Laser-induced two-photon blackbody radiation in the vacuum ultraviolet

Experimental measurements of a new type of vacuum-ultraviolet radiation source are reported. It is shown that the maximum source brightness, within its narrow linewidth, is that of a blackbody at the temperature of a metastable storage level. The laser-induced emission at 569 A from a He glow discharge corresponded to a metastable temperature of 22,700 K and was over 100 times brighter than the 584-A He resonance line.

Zych, L. J.

Rapid laser induced energy transfer in atomic systems

Analytical and experimental studies of the rapid transfer of stored populations from metastable states to selected target states of a different species are reported. Both laser-induced or laser-switched collision and laser-induced two-photon spontaneous emission are described. It is shown that the laser-induced collision method is particularly useful in the visible and UV spectral regions. It has applications in photochemistry, gas-phase kinetics, and in high-power, high-energy gas-phase lasers. The anti-Stokes source is useful in the VUV and soft X-ray spectral regions.

Harris, S. E.

Mixed metal vapor phase matching for third-harmonic generation

Phase matching for frequency tripling of 1.06 microns is demonstrated in a homogeneous mixture of sodium and magnesium vapor. The ratio of Mg to Na vapor pressures required for phase matching is 2:1. This ratio is about 1/75 of that required to phase match Na with Xe.

Bloom, D. M.

Third harmonic generation in phase-matched alkali metal vapors

We report improvements in conversion efficiency for third harmonic generation in sodium and rubidium vapor. 30-psec pulses of radiation at 1.064 micron have been converted to 0.3547 micron with an energy conversion efficiency of 10%. Factors limiting conversion efficiency are discussed.

Bloom, D. M.

Investigation of laser dynamics, modulation and control by means of intra-cavity time varying perturbation

The generation of tunable visible, infrared, and ultraviolet light is examined, along with the control of this light by means of novel mode-locking and modulation techniques. Transient mode-locking of the Nd:YAG laser and generation of short tunable pulses in the visible and the alkali metal inert gas excimer laser systems were investigated. Techniques for frequency conversion of high power and high energy laser radiation are discussed, along with high average power blue and UV laser light sources.

Harris, S. E.

Generation of ultraviolet and vacuum ultraviolet radiation

The paper describes nonlinear optical techniques that use phase-matched mixtures of metal vapors and inert gases, or, in certain cases, only inert gases for the generation of ultraviolet radiation. These systems are transparent where nonlinear crystals are opaque and their high ionization permits optical power densities of 10 to the 10 or 10 to the 11 W/sq cm to be utilized. An experiment designed to convert incident 1.064 micron radiation to 3547 A radiation is described as are experiments designed to generate vacuum ultraviolet at 1773, 1520, 1182 and 887 A. Theoretical considerations on the use of this nonlinear optical technique for the generation of soft X-rays are presented and the construction of a vacuum ultraviolet holographic grating with a fringe spacing of 836 A is reported on.

Harris, S. E.

Vacuum ultraviolet holography

We report the first demonstration of holographic techniques in the vacuum ultraviolet spectral region. Holograms were produced with coherent 1182-A radiation. The holograms were recorded in polymethyl methacrylate and examined with an electron microscope. A holographic grating with a fringe spacing of 386 A was produced and far-field Fraunhofer holograms of submicron particles were recorded.

Bjorklund, G. C.

Vacuum ultraviolet holography

The authors report the first demonstration of holographic techniques in the vacuum ultraviolet spectral region. Holograms were produced with coherent 1182 A radiation. The holograms were recorded in polymethyl methacrylate and read out with an electron microscope. A holographic grating with a fringe spacing of 836 A was produced and far-field Fraunhofer holograms of sub-micron particles were recorded.

Bjorklund, G. C.

Infrared up-conversion with resonantly two-photon pumped metal vapors

Observation of efficient up-conversion of low-level IR radiation near 10 microns to the near ultraviolet. Radiation at 9.26 micron is converted to 3305 A with a photon conversion efficiency of 58% and a corresponding power gain of 16.2. The process employs resonant two-photon pumping of the nonallowed 3s-3d transition in Na.

Bloom, D. M.

Resonantly two-photon pumped frequency converter

This letter describes a resonantly two-photon pumped frequency converter with application to the generation of tunable ultraviolet and vacuum ultraviolet radiation and also to infrared-to-visible up-conversion and imaging. Calculations show that up-conversion power efficiencies in excess of 100% should be obtained with tunable dye lasers having peak powers in the hundred watt to kilowatt range.

Harris, S. E.