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Henderson, Brian S.

Publications and source records attributed to Henderson, Brian S..

Multiple monoenergetic gamma radiography (MMGR) with a compact superconducting cyclotron

Smuggling of special nuclear materials and nuclear devices through borders and ports of entry constitutes a major risk to global security. Technologies are needed to reliably screen the flow of commerce for the presence of high-Z materials such as uranium and plutonium. Here, we present an experimental proof-of-concept of a technique that uses inelastic (p,p') nuclear reactions to generate monoenergetic photons, which provide means to measure the areal density and the effective-Z (Z eff ) of an object with an accuracy surpassing that achieved by current methods. We use an ION-12 SC superconducting 12 MeV proton cyclotron to produce 4.4, 6.1, 6.9, and 7.1 MeV photons from a variety of nuclear reactions. Using these photons in a transmission mode, we show that we are able to accurately reconstruct the areal densities and Zeff of a test object. This methodology could enable mobile applications to screen commercial cargoes with high material specificity, providing a means of distinguishing common cargo materials from high-Z materials that include uranium and plutonium.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Validation of Geant4’s G4NRF module against nuclear resonance fluorescence data from 238 U and 27 Al

G4NRF (Jordan and Warren, 2007; Vavrek et al., 2018a,b) is a simulation module for modeling nuclear resonance fluorescence (NRF) interactions in the Geant4 framework (Allison et al., 2016). In this work, we validate G4NRF against both absolute and relative measurements of three NRF interactions near 2.2 MeV in 238 U and 27 Al using the transmission NRF data from the experiments described in Jayson et al. (2018). Agreement between the absolute NRF count rates observed in the data and predicted by extensive Geant4+G4NRF modeling validate the combined Geant4+G4NRF to approximately 15–20% in the 238 U NRF transitions and 10% in 27 Al, for an average 14% discrepancy across the entire study. The difference between simulation and experiment in relative NRF rates, as expressed as ratios of count rates in various NRF lines, is found at the level of ≲3%, and is statistically identical to zero. Finally, inverting the analysis, approximate values of the absolute level widths and branching ratios for 238 U and 27 Al are also obtained.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

High-accuracy Geant4 simulation and semi-analytical modeling of nuclear resonance fluorescence

Nuclear resonance fluorescence (NRF) is a photonuclear interaction that enables highly isotope-specific measurements in both pure and applied physics scenarios. High-accuracy design and analysis of NRF measurements in complex geometries is aided by Monte Carlo simulations of photon physics and transport, motivating Jordan and Warren (2007) to develop the G4NRF codebase for NRF simulation in Geant4. In this work, we enhance the physics accuracy of the G4NRF code and perform improved benchmarking simulations. The NRF cross section calculation in G4NRF, previously a Gaussian approximation, has been replaced with a full numerical integration for improved accuracy in thick-target scenarios. A high-accuracy semi-analytical model of expected NRF count rates in a typical NRF measurement is then constructed and compared against G4NRF simulations for both simple homogeneous and more complex heterogeneous geometries. Furthermore, agreement between rates predicted by the semi-analytical model and G4NRF simulation is found at a level of ~1% in simple test cases and ~3% in more realistic scenarios, improving upon the ~20% level of the initial benchmarking study and establishing a highly-accurate NRF framework for Geant4.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗