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Henderson, R. A.

Publications and source records attributed to Henderson, R. A..

Toward the Discovery of New Elements: Production of Livermorium (𝑍 = 116) with 50 Ti

The 244 Pu ⁢(50 Ti ,𝑥⁢𝑛)⁢ 294−𝑥 Lv reaction was investigated at Lawrence Berkeley National Laboratory’s 88-Inch Cyclotron. The experiment was aimed at the production of a superheavy element with 𝑍 ≥114 by irradiating an actinide target with a beam heavier than 48 Ca. Produced Lv ions were separated from the unwanted beam and nuclear reaction products using the Berkeley Gas-filled Separator and implanted into a newly commissioned focal-plane detector system. Two decay chains were observed and assigned to the decay of 290 Lv . The production cross section was measured to be 𝜎 prod = 0.44($^{+0.58}_{−0.28}$) pb at a center-of-target center-of-mass energy of 220(3) MeV. Furthermore, this represents the first published measurement of the production of a superheavy element near the “island of stability,” with a beam of 50 Ti and is an essential precursor in the pursuit of searching for new elements beyond 𝑍 =118.

36 MATERIALS SCIENCE↗

239 Pu Fission Spectrum Cumulative Fission Product Yield Measurement Using Godiva IV Critical Assembly

Precise integral measurement of fast neutron-induced fission product yields for various actinides is of high interest for applied nuclear science. The goal of this effort is to improve uncertainties in fission product yield values of 239 Pu. Fission was induced in a pure 239 Pu (>99%) target using the Godiva IV critical assembly in burst mode. Further, the irradiated sample was transferred to a high-resolution γ-ray detector within 45 minutes. γ-ray list mode data was collected from 45 minutes to 1 week after the irradiation. γ-ray spectroscopy was performed to analyze the time dependent γ-ray yields using an automated peak search algorithm to identify isotopes by their decay γ-ray energy and half-life. The initial activity for each isotope identified was used to calculate their fission product yield.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Quick Look Report of Godiva U233 shot March 2022 Data Collection Activities

This report discussing the March 2022 irradiation of U233 on the Godiva critical assembly using burst mode and subsequent analysis of the fission products starting at 65 minutes post irradiation, and ending 12 days later. The Short-Lived Fission Product Yield (SLFPY) project is one of many efforts under the Nuclear Physics Multi-Lab and related Venture Project. The objective of the SLFPY project is to provide improved measurements of fission product yields for select nuclides. The SLFPY project consists of measurement and analysis campaigns. To produce fission data, samples of actinide material are irradiated in a high-flux neutron environment. These samples are quickly placed in front of a detection system where both gamma singles and coincidence spectra are collected as a function of time. Gamma spectroscopy is performed on the irradiated material on site near the irradiation facility, starting as soon as feasible after the irradiation and continuing for 7 days or longer. Following the data collection, time-dependent fission yield analyses are performed using gamma-ray spectroscopy. This document summarizes the measurement campaign performed March 21 - April 4, 2022 where sub-gram quantities of 233 U nitrate (UO 2 (NO 3 ) 2 ) were irradiated in the Godiva reactor. The Godiva burst #2076 conducted under experiment IER 504 had a temperature change of +156 degrees Celsius, lasted 13.32 microseconds, and had a reactivity of $\$$1.089. The targets consisted of uranium oxide solution deposited in a quartz tube and packed with quartz wool. The flame-sealed quartz ampoules were used to contain the uranium samples for the irradiation and count activities. On March 22, 2022, at 10:27:00 a.m. the three uranium ampoules, along with a witness foil pack, were irradiated in the Godiva critical assembly using burst mode operations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Measurement of the 240 Pu(n,f) Prompt Fission Neutron Spectra with Chi-Nu

The DOE Nuclear Criticality Safety Program has funded a multi-year effort to measure the 240 Pu(n,f) Prompt Fission Neutron Spectrum at Chi-Nu. This project is a joint LANL-LLNL effort, involving the preparation of 12 240 Pu foils and construction of a Parallel-Plate Avalanche Counter at LLNL, with subsequent measurements of the 240 Pu(n,f) PFNS at the Chi-Nu beamline at the Los Alamos Neutron Science Center’s Weapons Neutron Research facility (LANSCE/WNR). We expect the PPAC to be ready in time to perform the measurements this run cycle.

240Pu Foils↗

Beta Radiation Hardness of GYGAG(Ce) Transparent Ceramic Scintillators

GYGAG(Ce) transparent ceramic garnet scintillators were irradiated with electrons from 0.5 to 2 MeV with fluences from 10 16 e – /cm 2 to 10 19 e – /cm 2 , corresponding to doses from 0.3 to 310 Gigarad. Absorption spectra were measured before and after irradiations. Light yields from alpha, beta, and gamma excitations were measured before and after irradiation and compared to preirradiation values to gain a deeper understanding of how electron irradiations can affect light yield, as well as defects generated in both the surface and bulk. Within experimental error, no degradation in light yield was observed for the electron-irradiated samples, as measured via beta or gamma excitation, with minimal degradation observed via alpha excitation. A small increase in optical absorption near the wavelength of emission was observed following the largest dose irradiation. These results suggest that GYGAG(Ce) is radiation hard to electron irradiation up to 10 19 e – /cm 2 and doses up to 310 Gigarad. Furthermore, this robustness to irradiation indicates that transparent ceramic garnets may prove useful for applications such as scintillation-based nuclear batteries by allowing for higher energy beta emitters, increased power densities, and enabling long service lifetimes.

36 MATERIALS SCIENCE↗

Selenium-iodide: A low melting point eutectic semiconductor

Inorganic liquid semiconductors are of interest in harsh radiological environments, flexible electronics, and for direct printing of semiconductor devices. Many elemental and compound liquid semiconductors exist, although the lowest melting point is observed for Se at 221 °C. Recently, reports of liquid Se-S systems have shown betavoltaic and alphavoltaic power generation as a liquid with a reduced melting point of 105 °C. Here in this paper, we show the ability to depress the melting point to 57 °C by using equal atomic fractions of selenium and iodine while maintaining semiconducting behavior. A heterojunction structure using ITO and n-GaN as the contacts was selected based on chemical compatibility and predicted band lineups. Electrical and optical measurements were used to deduce the electronic and transport properties of the mixture.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Prompt neutron emission in the neutron-induced fission of 239 Pu and the spontaneous fission of 252 Cf: an unfolding story

Prompt neutron emission is one of the major observables in fission and critical to a sustained chain reaction. The prompt neutron emission spectrum and its precision are essential for adequately modeling the chain reaction for any given application. Within this context, a joint program, called Chi-Nu, was initiated by LANL [1] with the objective to improve the precision of experimental measurements of prompt neutron emission for neutron-induced fission of 235 U and 239 Pu as well as the spontaneous fission of 252 Cf. The measurements were carried out at the Weapons Neutron Research Facility at Los Alamos Neutron Science Center using two scintillator arrays for neutron detection and a PPAC (parallel-plate avalanche counter) for fission-fragment detection.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Theoretical analysis of the electrical aspects of the basic electro-impulse problem in aircraft de-icing applications

A summary of modeling the electrical system aspects of a coil and metal target configuration resembling a practical electro-impulse deicing (EIDI) installation, and a simple circuit for providing energy to the coil, was presented. The model was developed in sufficient theoretical detail to allow the generation of computer algorithms for the current in the coil, the magnetic induction on both surfaces of the target, the force between the coil and target, and the impulse delivered to the target. These algorithms were applied to a specific prototype EIDI test system for which the current, magnetic fields near the target surfaces, and impulse were previously measured.

Henderson, R. A.↗