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Hering, Susanne

Publications and source records attributed to Hering, Susanne.

7 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Mapping the performance of a versatile water-based condensation particle counter (vWCPC) with numerical simulation and experimental study

Accurate airborne aerosol instrumentation is required to determine the spatial distribution of ambient aerosol particles, particularly when dealing with the complex vertical profiles and horizontal variations of atmospheric aerosols. A versatile water-based condensation particle counter (vWCPC) has been developed to provide aerosol concentration measurements under various environments with the advantage of reducing the health and safety concerns associated with using butanol or other chemicals as the working fluid. However, the airborne deployment of vWCPCs is relatively limited due to the lack of characterization of vWCPC performance at reduced pressures. Given the complex combinations of operating parameters in vWCPCs, modeling studies have advantages in mapping vWCPC performance. In this work, we thoroughly investigated the performance of a laminar-flow vWCPC using COMSOL Multiphysics® simulation coupled with MATLAB™. We compared it against a modified vWCPC (vWCPC model 3789, TSI, Shoreview, MN, USA). Our simulation determined the performance of particle activation and droplet growth in the vWCPC growth tube, including the supersaturation, $D$ p,kel,0 (smallest size of particle that can be activated), $D$ p,kel,50 (particle size activated with 50 % efficiency) profile, and final growth particle size D d under wide operating temperatures, inlet pressures $P$ (30–101 kPa), and growth tube geometry (diameter $D$ and initiator length $L$ ini ). The effect of inlet pressure and conditioner temperature on vWCPC 3789 performance was also examined and compared with laboratory experiments. The COMSOL simulation result showed that increasing the temperature difference (Δ$T$) between conditioner temperature $T$ con and initiator $T$ ini will reduce $D$ p,kel,0 and the cut-off size $D$ p,kel,50 of the vWCPC. In addition, lowering the temperature midpoint ($T$ mid = $\frac{T_{con}+T_{ini}}{2}$ increases the supersaturation and slightly decreases the $D$ p,kel . The droplet size at the end of the growth tube is not significantly dependent on raising or lowering the temperature midpoint but significantly decreases at reduced inlet pressure, which indirectly alters the vWCPC empirical cut-off size. Our study shows that the current simulated growth tube geometry ($D$=6.3 mm and $L$ ini =30 mm) is an optimized choice for current vWCPC flow and temperature settings. The current simulation can more realistically represent the $D$ p,kel for 7 nm vWCPC and also achieved good agreement with the 2 nm setting. Using the new simulation approach, we provide an optimized operation setting for the 7 nm setting. This study will guide further vWCPC performance optimization for applications requiring precise particle detection and atmospheric aerosol monitoring.

47 OTHER INSTRUMENTATION↗
DOE OSTI2021

Simulation-aided characterization of a versatile water-based condensation particle counter for atmospheric airborne research

Capturing the vertical profiles and horizontal variations of atmospheric aerosols often requires accurate airborne measurements. With the advantage of avoiding health and safety concerns related to the use of butanol or other chemicals, water-based condensation particle counters have emerged to provide measurements under various environments. However, airborne deployments are relatively rare due to the lack of instrument characterization under reduced pressure at flight altitudes. This study investigates the performance of a commercial “versatile” water-based condensation particle counter (vWCPC, model 3789, TSI, Shoreview, MN, USA) under various ambient pressure conditions (500–920 hPa) with a wide range of particle total number concentrations (1500–70 000 cm -3 ). The effect of conditioner temperature on vWCPC 3789 performance at low pressure is examined through numerical simulation and laboratory experiments. We show that the default instrument temperature setting of 30 °C for the conditioner is not suitable for airborne measurement and that the optimal conditioner temperature for low-pressure operation is 27°. Under the optimal conditioner temperature (27°), the 7 nm cut-off size is also maintained. Additionally, we show that insufficient droplet growth becomes more significant under the low-pressure operation. The counting efficiency of the vWCPC 3789 can vary up to 20 % for particles of different chemical compositions (e.g., ammonium sulfate and sucrose particles). However, such variation is independent of pressure.

54 ENVIRONMENTAL SCIENCES↗