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Hyundeok Choi

Publications and source records attributed to Hyundeok Choi.

TPSAS-NF1676L-33993-DND

Large volcanic eruptions are the primary sources of aerosols in the stratosphere and play an important role in the global climate system. The transformation of sulfur dioxide emitted by volcanoes into sulfuric acid droplets leads to a global cooling effect at the surface by enhanced reflection of solar radiation to space and reduced the earth's radiative budget for months to years. In June 2019, the Raikoke volcano, Kuril Islands (153.24167 E, 48.29167 N) emitted 1.4 Tg of SO2 between June 21st and 22nd with plume injection height between 7 and 15 km based on several ultra-violet and infrared sensors as well as the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) space-based lidar. CALIPSO and the NASA Langley Trajectory Model (LaTM) with GEOS5 meteorological data are used to track dispersed volcanic ash plumes. The trajectory mapping technique will be used to re-construct the 3-dimension structure of volcanic ash and sulfate. Results will be compared with independent observations from the Stratospheric Aerosol and Gas Experiment and GEOS-Chem model outputs to understand the transport of the plume into the stratosphere and its lifetime.

Hyundeok Choi↗

Distribution and Sources of Tropospheric Aerosols Over the Western North Atlantic During ACTIVATE (February-March 2020)

The Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) is a five-year (2019-2023) NASA Earth-Venture Suborbital-3 (EVS-3) mission to robustly characterize aerosol-cloud-meteorology interactions during February-June, with a focus on marine boundary layer clouds. This characterization requires understanding of aerosol composition, distribution, transport pathways, and sources. Here we use the GEOS-Chem chemical transport model driven by the MERRA-2 reanalysis to simulate tropospheric carbon monoxide (CO) and aerosols over the western North Atlantic Ocean (WNAO) during the first field deployment of ACTIVATE (February-March 2020). CO is used as a tracer to diagnose transport pathways for continental pollution outflow to the WNAO. The aerosol simulation represents all major aerosols including sulfate-nitrate-ammonium (SNA), mineral dust, sea salt, black and organic carbon aerosols. Model-simulated mixing ratios of SNA and organic carbon are compared with aircraft observations. We show that intensive aerosol mass measurements in the lower troposphere over the North American outflow region during ACTIVATE provide strong constraints on model aerosol wet scavenging. Comparisons of model aerosol extinctions with the airborne High Spectral Resolution Lidar-2 (HSRL-2) measurements indicate that the model generally captures continental outflow of aerosols and enhanced extinctions associated with sea salt. Simulated aerosol optical depths (AODs) and extinction vertical profiles are also compared with satellite retrievals from MODIS/Aqua and CALIOP/CALIPSO, respectively. CALIOP sometimes observes enhanced aerosol extinction at altitudes between ~1.5km and ~2.0km south of 32°N. The model reproduces this enhancement and attributes it to coarse-mode sea salt associated with high relative humidity. The relative contributions of continental and oceanic sources to the aerosol loading, AOD, and their distributions over the study domain will also be discussed.

aerosols↗

Assessing the Radiative Impact of the 2019 – 2020 Australian Bushfires using Trajectory-Mapped CALIPSO and SAGE III/ISS Observations.

During the 2019/2020 fire season, Australian bushfires burned 46 million acres, killed 39 people and billions of animals, and became the costlier fire season in Australian history. Between the end of December and early January, a series of pyrocumulonimbus injected thick smoke layers in the upper troposphere and lower stratosphere which were observed over the Tasmanian Sea and New Zealand by the Ozone Mapping and Profiler Suite (OMPS) and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO). The smoke plume crossed the tropopause and was further dispersed across the Eastern Pacific Ocean rising up to 30 km height after two weeks. . In this study, we use CALIPSO and the NASA Langley Trajectory Model (LaTM), driven by Modern-Era Retrospective analysis for Research and Application, Version 2 (MERRA-2) meteorological data, to track the dispersion of Australian fire smoke plumes in both the troposphere and the stratosphere. Trajectory mapping is used to re-construct the 3-dimension structure of the smoke plumes. Results are compared with independent observations from the Stratospheric Aerosol and Gas Experiment (SAGE) III on the International Space Station (ISS) to understand the complex transport of the plume into the stratosphere and its lifetime. Using trajectory maps, the impact of the Australian bushfires on the Earth’s radiative energy budget is assessed with the Clouds and the Earth’s Radiant Energy System (CERES).

Australian bushfire↗