Airborne lidar measurements of atmospheric CO 2 column concentrations to cloud tops made during the 2017 ASCENDS/ABoVE campaign
We measured the column-averaged atmospheric CO 2 mixing ratio (XCO 2 ) to a variety of cloud tops with an airborne pulsed multi-wavelength integrated path differential absorption (IPDA) lidar during NASA's 2017 ASCENDS/ABoVE airborne campaign. Measurements of height-resolved atmospheric backscatter profiles allow this lidar to retrieve XCO 2 to cloud tops, as well as to the ground, with accurate knowledge of the photon path length. We validated these measurements with those from an onboard in situ CO 2 sensor during spiral-down maneuvers. These lidar measurements were 2–3 times better than those from previous airborne campaigns due to our using a wavelength step-locked laser transmitter and a high-efficiency detector for this campaign. Precisions of 0.6 parts per million (ppm) were achieved for 10 s average measurements to mid-level clouds and 0.9 ppm to low-level clouds at the top of the planetary boundary layer. This study demonstrates the lidar's capability to fill in XCO 2 measurement gaps in cloudy regions and to help resolve the vertical and horizontal distributions of atmospheric CO 2 . Future airborne campaigns and spaceborne missions with this capability can be used to improve atmospheric transport modeling, flux estimation and carbon data assimilation.