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Jeffrey S Reid

Publications and source records attributed to Jeffrey S Reid.

Multi-Campaign Ship and Aircraft Observations of Marine Cloud Condensation Nuclei and Droplet Concentrations

In-situ marine cloud droplet number concentrations (CDNCs), cloud condensation nuclei (CCN), and CCN proxies, based on particle sizes and optical properties, are accumulated from seven field campaigns: ACTIVATE; NAAMES; CAMP2EX; ORACLES; SOCRATES; MARCUS; and CAPRICORN2. Each campaign involves aircraft measurements, ship-based measurements, or both. Measurements collected over the North and Central Atlantic, Indo-Pacific, and Southern Oceans, represent a range of clean to polluted conditions in various climate regimes. With the extensive range of environmental conditions sampled, this data collection is ideal for testing satellite remote detection methods of CDNC and CCN in marine environments. Remote measurement methods are vital to expanding the available data in these difficult-to-reach regions of the Earth and improving our understanding of aerosolcloud interactions. The data collection includes particle composition and continental tracers to identify potential contributing CCN sources. Several of these campaigns include High Spectral Resolution Lidar (HSRL) and polarimetric imaging measurements and retrievals that will be the basis for the next generation of space-based remote sensors and, thus, can be utilized as satellite surrogates.

Atmospheric chemistry↗

The Extreme Forest Fires in California/Oregon in 2020: Aerosol Optical and Physical Properties and Comparisons of Aged Versus Fresh Smoke

Wildfire activity in the western United States during August to October 2020 was exceptional in terms of the fire severity and area burned. Extremely dry biomass fuels from near historic multi-year drought conditions were further exacerbated with very hot and dry conditions in 2020. These conditions when coupled with strong offshore flow allowed many ignitions to grow into extremely large and severe wildfires. Long-term monitoring at a few AERONET sites in California showed that the number of days with high Aerosol Optical Depth at 440 nm (AOD 440 >1) in 2020 was greater than any other year going back to the beginning of the data records in 2002. A wide range of fine mode particle volume median radii were retrieved from AERONET data over the course of these fires suggesting significant variability in combustion conditions and aging processes. Additionally, the fine mode radii in some of these smoke plumes in 2020 were very large especially at high AOD (∼0.22–0.32 μm volume median radius), likely due to both coagulation and condensation occurring during aging at very high particulate concentrations. The largest fine mode particle radii combined with narrow distributions resulted in some very rare AOD spectra showing peak AOD at 500 nm and decreasing to lower AOD at both shorter and longer wavelengths. The most extreme retrieved size distributions and associated measured AOD spectra were principally observed in long-distance transported smoke plumes from these western United States fires at sites in Colorado, Maryland and Virginia, possibly due to further aging during transport. Additionally, strong absorption was sometimes observed at short wavelengths with much lower single scattering albedo at 440 nm compared to 675 nm in some plumes consistent with significant brown carbon (BrC) and/or coated black carbon (BC) absorption in biomass burning particles. This strong spectral absorption signature observed at some California sites and dates remained similarly strong in some smoke plumes observed at some east coast sites in Maryland and Virginia, thereby suggesting that the lifetime of these particular BrC and/or coated BC absorbing species was greater than 5 days.

Aerosol↗

A Coupled Evaluation of Operational MODIS and Model Aerosol Products for Maritime Environments Using Sun Photometry: Evaluation of the Fine and Coarse Mode

Although satellite retrievals and data assimilation have progressed to where there is a good skill for monitoring maritime Aerosol Optical Depth (AOD), there remains uncertainty in achieving further degrees of freedom, such as distinguishing fine and coarse mode dominated species in maritime environments (e.g., coarse mode sea salt and dust versus fine mode terrestrial anthropogenic emissions, biomass burning, and maritime secondary production). For the years 2016 through 2019, we performed an analysis of 550 nm total AOD550, fine mode AOD (FAOD550; also known as FM AOD in the literature), coarse mode AOD (CAOD550), and fine mode fraction (η550) between Moderate Resolution Spectral Imaging Radiometer (MODIS) V6.1 MOD/MYD04 dark target aerosol retrievals and the International Cooperative for Aerosol Prediction (ICAP) core four multi-model consensus (C4C) of analyses/short term forecasts that assimilate total MODIS AOD550. Differences were adjudicated by the global shipboard Maritime Aerosol Network (MAN) and selected island AERONET sun photometer observations with the application of the spectral deconvolution algorithm (SDA). Through a series of conditional and regional analyses, we found divergence included regions of terrestrial influence and latitudinal dependencies in the remote oceans. Notably, MODIS and the C4C and its members, while having good correlations overall, have a persistent +0.04 to +0.02 biases relative to MAN and AERONET for typical AOD550 values (84th% < 0.28), with the C4C underestimating significant events thereafter. Second, high biases in AOD550 are largely associated with the attribution of the fine mode in satellites and models alike. Thus, both MODIS and C4C members are systematically overestimating AOD550 and FAOD550 but perform better in characterizing the CAOD550. Third, for MODIS, findings are consistent with previous reports of a high bias in the retrieved Ångström Exponent, and we diagnosed both the optical model and cloud masking as likely causal factors for the AOD550 and FAOD550 high bias, whereas for the C4C, it is likely from secondary overproduction and perhaps numerical diffusion. Fourth, while there is no wind-speed-dependent bias for surface winds <12 m s−1, the C4C and MODIS AOD550s also overestimate CAOD550 and FAOD550, respectively, for wind speeds above 12 m/s. Finally, sampling bias inherent in MAN, as well as other circumstantial evidence, suggests biases in MODIS are likely MODIS and the C4C products have their own strengths and challenges for a given climate application and discuss needed research. even larger than what was diagnosed here. We conclude with a discussion on how

Aerosols↗

Above-Aircraft Cirrus Cloud and Aerosol Optical Depth From Hyperspectral Irradiances Measured By a Total-Diffuse Radiometer

This study develops the use of spectral total and diffuse irradiance measurements, made from a prototype hyperspectral total-diffuse sunshine pyranometer (SPN-S), to retrieve layer fine-mode aerosol (τ aer ) and total optical depths from airborne platforms. Additionally, we use spectral analysis in an attempt to partition the total optical depth into its τ aer and cirrus cloud optical depth (τ cld ) components in the absence of coarse-mode aerosols. Two retrieval methods are developed: one leveraging information in the diffuse irradiance and the other using spectral characteristics of the transmitted direct beam, with each approach best suited for specific cloud and aerosol conditions. The SPN-S has advantages over traditional sun photometer systems, including no moving parts and a low cost. However, a significant drawback of the instrument is that it is unable to measure the direct-beam irradiance as accurately as sun photometers. To compensate for the greater measurement uncertainty in the radiometric irradiances, these retrieval techniques employ ratioed inputs or spectral information to reduce output uncertainty. This analysis uses irradiance measurements from the SPN-S and the solar spectral flux radiometer (SSFR) aboard the National Aeronautics and Space Administration’s (NASA) P-3 aircraft during the 2018 deployment of the ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) campaign and the 2019 Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP 2 Ex) mission to quantify above-aircraft cirrus τ cld and derive vertical profiles of layer τ aer . Validation of the τ aer retrieval is accomplished by comparison with co-located measurements of direct solar irradiance made by the Sky-Scanning Sun-Tracking Atmospheric Research (4STAR) and in situ measurements of aerosol optical depth. For the aggregated 2018 ORACLES results, regression between the SPN-S-based method and sun photometer τ aer values yields a slope of 0.96 with an R 2 of 0.96, while the root mean square error (RMSE) is 3.0 x 10 -2 . When comparing the retrieved τ aer to profiles of integrated in situ measurements of optical extinction, the slope, R 2 , and RMSE values for ORACLES are 0.90, 0.96, and 3.4 x 10 -2 , and for CAMP 2 Ex they are 0.94, 0.97, and 3.4 x 10 -2 , respectively. This paper is a demonstration of methods for deriving cloud and aerosol optical properties in environments where both atmospheric constituents may be present. With improvements to the low-cost SPN-S radiometer instrument, it may be possible to extend these methods to a broader set of sampling applications, such as ground-based settings.

spectral instrument (SPN-S)↗

Detecting Layer Height of Smoke and Dust Aerosols Over Vegetated Land and Water Surfaces Via Oxygen Absorption Bands

We present an algorithm for retrieving aerosol layer height (ALH) and aerosol optical depth (AOD) for smoke and dust over vegetated land and water surfaces from measurements of the Earth Polychromatic Imaging Camera (EPIC) onboard the Deep Space Climate Observatory (DSCOVR). Our algorithm uses EPIC atmospheric window bands to determine AOD and then takes advantage of oxygen A and B bands to derive ALH. We applied this algorithm on several dust and smoke events. Validation shows our results are of high accuracy.

Jing Zeng↗

Detecting Nighttime Fire Combustion Phase by Hybrid Application of Visible and Infrared Radiation from Suomi NPP VIIRS

An accurate estimation of biomass burning emissions is 1 partially limited by the lack of knowledge of fire burning phase (smoldering vs. flaming). In recent years, several fire detection products have been developed to provide information of fire radiative power (FRP), location, size, and temperature of fire pixels, but no information regarding fire burning phase is retrieved. The Day-Night band (DNB) aboard Visible Infrared Imaging Radiometer Suite (VIIRS) is sensitive to visible light from flaming fires in nighttime scenes. In contrast, VIIRS 4 m moderate resolution band #13 (M13), though capable of detecting fires at all phases, has no direct sensitivity for discerning fire phase. However, the hybrid usage of VIIRS DNB and M-bands data is hampered by their different scanning technology and spatial resolution. In this study, we present a novel method to rapidly and accurately resample DNB pixel radiances to the footprint of M-band pixels, accounting for onboard detector aggregation schemes and bowtie effect removals. The visible energy fraction (VEF) is subsequently introduced as an indicator of fire burning phase VEF is calculated as the ratio of visible light power (VLP) to FRP for each fire pixel retrieved from the VIIRS 750 m active fire product. A global distribution of VEF values, and thereby the fire phase, is quantitatively obtained, showing smaller VEF values in regions with mostly smoldering wildfires, such as peatland fires in Indonesia, larger VEF values in regions with flaming wildfires over grasslands and savannas in the sub-Sahelian region, and the largest VEF values associated with gas flaring in the Middle East. Mean VEF for different land cover types or regions is highly correlated with modified combustion efficiency (MCE). These results, together with a case study of the 2018 California Camp Fire, show that the VEF has the potential to be an indicator of fire combustion phase for each fire pixel, appropriate for estimating emission factors at the satellite pixel level.

Jun Wang↗

Investigation of CATS Aerosol Products and Application Toward Global Diurnal Variation of Aerosols

We present a comparison of 1064 nm aerosol optical depth (AOD) and aerosol extinction profiles from the Cloud-Aerosol Transport System (CATS) level 2 aerosol product with collocated Aerosol Robotic Network (AERONET) AOD, Moderate Imaging Spectroradiometer (MODIS) Aqua and Terra Dark Target AOD and Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) AOD and extinction data for the period of March 2015–October 2017. Upon quality-assurance checks of CATS data, reasonable agreement is found between aerosol data from CATS and other sensors. Using quality-assured CATS aerosol data, for the first time, variations in AODs and aerosol extinction profiles are evaluated at 00:00, 06:00, 12:00 and 18:00 UTC (and/or 00:00, 06:00, 12:00 and 18:00 local time or LT) on both regional and global scales. This study suggests that marginal variations are found in AOD from a global mean perspective, with the minimum aerosol extinction values found at 18:00 LT near the surface layer for global oceans, for both the June–November and December–May seasons. Over land, below 500 m, the daily minimum and maximum aerosol extinction values are found at 12:00 and 00:00/06:00 LT, respectively. Strong diurnal variations are also found over north Africa, the Middle East and India for the December–May season, and over north Africa, south Africa, the Middle East and India for the June–November season.

Logan Lee↗

Characterization and Application of Artificial Light Sources for Nighttime Aerosol Optical Depth Retrievals using the Visible Infrared Imager Radiometer Suite Day/Night Band

Using nighttime observations from Visible Infrared Imager Radiometer Suite (VIIRS) Day/Night band (DNB), the characteristics of artificial light sources are evaluated as functions of observation conditions, and incremental improvements are documented on nighttime aerosol retrievals using VIIRS DNB data on a regional scale. We find that the standard deviation of instantaneous radiance for a given artificial light source is strongly dependent upon the satellite viewing angle but is weakly dependent on lunar fraction and lunar angle. Retrieval of nighttime aerosol optical thickness (AOT) based on the novel use of these artificial light sources is demonstrated for three selected regions (United States, Middle East and India) during 2015. Reason-able agreement is found between nighttime AOTs from the VIIRS DNB and temporally adjacent daytime AOTs from the AErosol RObotic NETwork (AERONET) as well as from coincident nighttime AOT retrievals from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), indicating the potential of this method to begin filling critical gaps in diurnal AOT information at both regional and global scales. Issues related to cloud, snow and ice contamination during the winter season, as well as data loss due to the misclassification of thick aerosol plumes as clouds, must be addressed to make the algorithm operationally robust.

Jianglong Zhang↗

TPSAS-NF1676L-35847-DND

Aerosols, especially particulate matter with aerodynamic diameters smaller than 2.5 ?m (PM2.5), contribute to air pollution and negatively impact human health. Past studies have estimated PM2.5 concentrations through the use of aerosol optical thickness (AOT) datasets from passive satellite sensors like MODIS and MISR. However, a major limitation of using passive AOTs for PM2.5 applications is that they are column-integrated, while PM2.5 is a surface measurement. In this study, we employ a bulk-mass-modeling-based method to directly derive PM2.5 concentrations over the contiguous United States (CONUS) using two years (2008-2009) of daytime and nighttime near-surface aerosol extinction retrievals from the NASA Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument, bulk mass extinction efficiencies, and model-based hygroscopicity. Results reveal that CALIOP-derived PM2.5 agrees reasonably well with ground-based PM2.5 observations from the U.S. Environmental Protection Agency (EPA), implying this method exhibits some merit in monitoring PM2.5 concentrations from CALIOP data. The newly developed method is then applied to CALIOP aerosol extinction retrievals using nearly the entire CALIOP data record (2007-2018), and an initial trend analysis is conducted. Results from various sensitivity studies are also shown, including those of surface layer height and assumed aerosol type.

Travis D Toth↗