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Johnson, M. S.

Publications and source records attributed to Johnson, M. S..

The 40 Ar(d,p) 41 Ar cross section between 3–7 MeV

To determine the safety of using argon as a deuteron beam stopping material, the 40 Ar(d,p) 41 Ar cross section was measured at average deuteron energies of 3.6 MeV, 5.5 MeV, and 7.0 MeV using an activation method. A 16-MeV deuteron beam produced by Lawrence Berkeley National Laboratory’s 88-Inch Cyclotron was degraded to each energy by nickel foils and the front wall of an aluminum gas chamber. The reduced-energy deuterons were used to activate a sample of nat Ar gas. After each irradiation, the gas chamber’s 41 Ar activation was measured with a high-purity germanium detector. The cross sections measured were larger than a previous measurement by ~40%.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

s -wave scattering lengths for the 7 $\hbox{Be} +$ p system from an R -matrix analysis

The astrophysical S factor for the radiative proton capture reaction on Be 7 ( S 17 ) at low energies is affected by the s -wave scattering lengths. Herein, we report the measurement of elastic and inelastic scattering cross sections for the Be 7 + p system in the center-of-mass energy range 0.474–2.740 MeV and center-of-mass angular range 70 ° – 150 ° . A radioactive Be 7 beam produced at Oak Ridge National Laboratory's (ORNL) Holifield Radioactive Ion Beam Facility was accelerated and bombarded a thin polypropylene ( CH 2 ) n target. Scattered ions were detected in the segmented Silicon Detector Array. Using an R -matrix analysis of ORNL and Louvain-la-Neuve cross-section data, the s -wave scattering lengths for channel spins 1 and 2 were determined to be 17 . 34 – 1.33 + 1.11 and – 3 . 18 – 0.50 + 0.55 fm, respectively. The uncertainty in the s -wave scattering lengths reported in this work is smaller by a factor of 5–8 compared to the previous measurement, which may reduce the overall uncertainty in S 17 at zero energy. The level structure of B 8 is discussed based upon the results from this work. Evidence for the existence of 0 + and 2 + levels in B 8 at 1.9 and 2.21 MeV, respectively, is observed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fissile material detection using neutron time-correlations from photofission

The detection of special nuclear materials (SNM) in commercial cargoes is a major objective in the field of nuclear security. In this work we investigate the use of two-neutron time-correlations from photo-fission using the Prompt Neutrons from Photofission (PNPF) detectors in Passport Systems Inc.’s (PSI) Shielded Nuclear Alarm Resolution (SNAR) platform for the purpose of detecting ~5 kg quantities of fissionable materials in seconds. The goal of this effort was to extend the secondary scan mode of this system to differentiate fissile materials, such as highly enriched uranium, from fissionable materials, such as low enriched and depleted uranium (LEU and DU). Experiments were performed using a variety of material samples, and data were analyzed using the variance-over-mean technique referred to as Y 2F or Feynman-α. Results were compared to computational models to improve our ability to predict system performance for distinguishing fissile materials. Simulations were then combined with empirical formulas to generate receiver operating characteristics (ROC) curves for a variety of shielding scenarios. We show that a 10 second screening with a 200 μA 9 MeV X-ray beam is sufficient to differentiate kilogram quantities of HEU from DU in various shielding scenarios in a standard cargo container.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Implementing marine organic aerosols into the GEOS-Chem model

Marine-sourced organic aerosols (MOAs) have been shown to play an important role in tropospheric chemistry by impacting surface mass, cloud condensation nuclei, and ice nuclei concentrations over remote marine and coastal regions. In this work, an online marine primary organic aerosol emission parameterization, designed to be used for both global and regional models, was implemented into the GEOS-Chem (Global Earth Observing System Chemistry) model. The implemented emission scheme improved the large underprediction of organic aerosol concentrations in clean marine regions (normalized mean bias decreases from -79% when using the default settings to -12% when marine organic aerosols are added). Model predictions were also in good agreement (correlation coefficient of 0.62 and normalized mean bias of -36%) with hourly surface concentrations of MOAs observed during the summertime at an inland site near Paris, France. Our study shows that MOAs have weaker coastal-to-inland concentration gradients than sea-salt aerosols, leading to several inland European cities having >10% of their surface submicron organic aerosol mass concentration with a marine source. The addition of MOA tracers to GEOS-Chem enabled us to identify the regions with large contributions of freshly emitted or aged aerosol having distinct physicochemical properties, potentially indicating optimal locations for future field studies.

Gantt, B.↗

Atmospheric Dissolved Iron Depostiion to the Global Oceans: Effects of Oxalate-Promoted Fe Dissolution, Photochemical Redox Cycling, and Dust Mineralogy

Mineral dust deposition is suggested to be a significant atmospheric supply pathway of bioavailable iron (Fe) to Fe-depleted surface oceans. In this study, mineral dust and dissolved Fe (Fed) deposition rates are predicted for March 2009 to February 2010 using the 3-D chemical transport model GEOS-Chem implemented with a comprehensive dust-Fe dissolution scheme. The model simulates Fed production during the atmospheric transport of mineral dust taking into account inorganic and organic (oxalate)-promoted Fe dissolution processes, photochemical redox cycling between ferric (Fe(III)) and ferrous (Fe(II)) forms of Fe, dissolution of three different Fe-containing minerals (hematite, goethite, and aluminosilicates), and detailed mineralogy of windblown dust from the major desert regions. Our calculations suggest that during the yearlong simulation is approximately 0.26 Tg (1 Tg = 1012 g) of Fed was deposited to global oceanic regions. Compared to simulations only taking into account proton-promoted Fe dissolution, the addition of oxalate to the dust-Fe mobilization scheme increased total annual model-predicted Fed deposition to global oceanic regions by approximately 75%. The implementation of Fe(II)/Fe(III) photochemical redox cycling in the model allows for the distinction between different oxidation states of deposited Fed. Our calculations suggest that during the daytime, large fractions of Fed deposited to the global oceans is likely to be in Fe(II) form, while nocturnal fluxes of Fed are largely in Fe(III) form. Model simulations also show that atmospheric fluxes of Fed can be strongly influenced by the mineralogy of Fe-containing compounds. This study shows that Fed deposition to the oceans is controlled by total dust-Fe mass concentrations, mineralogy, the surface area of dust particles, atmospheric chemical composition, cloud processing, and meteorological parameters and exhibits complex and spatiotemporally variable patterns. Our study suggests that the explicit model representation of individual processes leading to Fed production within mineral dust are needed to improve the understanding of the atmospheric Fe cycle, and quantify the effect of dust-Fe on ocean biological productivity, carbon cycle, and climate.

Johnson, M. S.↗

Single Event Upset Effects on the Clementine Solid State Data Recorder

The sensitivity of the Clementine 2.1 Gbit Solid State Data Recorder (SSDR) to single event upsets was characterized in ground tests. Subsequent in-situ measurements of the ambient radiation environment by experiments on-board Clementine permitted evaluation of the ability of models of the single event phenomenon in the SSDR to be tested using actual data. Initial results from the analysis reveal a nearly constant background upset rate of ~71 bit flips/day for the SSDR. There is no obvious correlation with a solar proton event recorded by Clementine and several other spacecraft on 20-21 February 1994, indicating that the SSDR was not sensitive to protons. The constant rate is thus interpreted as being a function of the Galactic Cosmic Ray heavy ion environment. A pronounced lunar orbit altitude dependence has also been identified in the data though the cause has not yet been unambiguously identified.

Clementine↗

Space flight operations

Space flight operations - launch site, deep space instrumentation facility, operations complex, launch site, communications facility, and checkout facility

SPACE FLIGHT↗