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Josephson, Alexander J.

Publications and source records attributed to Josephson, Alexander J..

Informed Multi‐Scale Approach Applied to the British Columbia Fires of Late Summer 2017

Abstract Pyrocumulonimbus (PyroCb) clouds have a complex origin dependent on fire dynamics and meteorological conditions. When a pyrocumulonimbus cloud develops and is maintained over a period of time, it can inject significant aerosol into the troposphere and lower stratosphere, resulting in a longer‐term (months to years) occurrence of aerosol in the stratosphere. In this work, we investigate the British Columbia wildfires on 12–13 August 2017 using a multi‐scale simulation framework. We use the output of a physics‐based wildfire model (FIRETEC) with parameterized energy, particle, and gas emissions to drive the upper atmospheric aerosol mass injection within a regional cloud resolving model (HIGRAD). We demonstrate that vertical motions produced by latent heat release of the condensation of ice and cloud particles within the PyroCbs induce another 5 km of lifting of the simulated aerosol plume. Primary black carbon and organic aerosols (OAs) alone may not be enough to explain the observed aerosol burden, thus we show that secondary OA produced via condensation of gases by the fires, ash, and possibly dust can enhance lofted aerosol mass. A simulation with all emission mechanisms active, driven by the observed fuel load and environmental conditions, reasonably reproduces an aerosol profile inferred from observational data.

54 ENVIRONMENTAL SCIENCES↗

Reduction of a detailed soot model for simulations of pyrolysing solid fuels

Here, we introduce a computationally inexpensive soot formation model for use in simulating large solid-complex fuel systems. The proposed model evaluates three variables: number density of tars, bulk mass density of soot particles, and particle number density. Each of these variables are influenced by soot formation phenomena, and this model evaluates the most common of these phenomena: soot nucleation, surface reactions, and coagulation. Two separate simulations were carried out using this model and results were compared against simulations using a more detailed and computationally expensive model. Findings are promising and show a meaningful reduction in model complexity and computational cost while still giving comparable results.

58 GEOSCIENCES↗

Modeling soot formation from solid complex fuels

A detailed model is proposed for predicting soot formation from complex solid fuels. The proposed model resolves two particle size distributions, one for soot precursors and another for soot particles. The precursor size distribution is represented with a sectional approach while the soot particle-size distribution is represented with the method of moments and an interpolative closure method is used to resolve fractional methods. Based on established mechanisms, this model includes submodels for precursor coagulation, growth, and consumption, as well as soot nucleation, surface growth, agglomeration, and consumption. The model is validated with comparisons to experimental data for two systems: coal combustion over a laminar flat-flame burner and biomass gasification. Results are presented for soot yield for three coals at three temperatures each, and for soot yield from three types of biomass at two temperatures each. These results represent a wide range of fuels and varying combustion environments, demonstrating the broad applicability of the model.

97 MATHEMATICS AND COMPUTING↗