Engineering topics

Kapaklis, Vassilios

Publications and source records attributed to Kapaklis, Vassilios.

4 records

DOE OSTI2024

Magnetic metamaterials by ion-implantation

We present a method for the additive fabrication of planar magnetic nanoarrays with minimal surface roughness. Synthesis is accomplished by combining electron-beam lithography, used to generate nanometric patterned masks, with ion implantation in thin films. By implanting 56 Fe + ions, we are able to introduce magnetic functionality in a controlled manner into continuous Pd thin films, achieving 3D spatial resolution down to a few tens of nanometers. Our results demonstrate the application of this technique in fabricating square artificial spin ice lattices, which exhibit well-defined magnetization textures and interactions among the patterned magnetic elements.

36 MATERIALS SCIENCE↗

DOE OSTI2018

Observation of the nonlinear Wood's anomaly on periodic arrays of nickel nanodimers

Linear and nonlinear magnetophotonic properties of periodic arrays of nickel nanodimers are governed by the interplay of the (local) optical response of individual nanoparticles and (nonlocal) diffraction phenomena. The redistribution of light intensity between diffracted beams when a diffraction order onsets or disappears is known as Wood's anomaly. Here in this paper, angular and magnetic-field-dependent near-infrared spectroscopic measurements, performed for different optical wavelengths and grating constants, discriminate between the linear and nonlinear excitation mechanisms of Wood's anomalies. In the nonlinear regime, evidenced by the magnetic second-harmonic generation, Wood's anomaly is characterized by an order-of-magnitude larger effect in intensity redistribution between the diffracted beams as compared to the linear case. Finally, the nonlinear Wood's anomaly manifests itself also in the nonlinear magnetic contrast highlighting the prospects of nonlinear magnetophotonics.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2018

Magnetic order and energy-scale hierarchy in artificial spin-ice structures

In order to explain and predict the properties of many physical systems, it is essential to understand the interplay of different energy scales. Here we present investigations of the magnetic order in thermalized artificial spin-ice structures, with different activation energies of the interacting Ising-like elements. We image the thermally equilibrated magnetic states of the nanostructures using synchrotron-based magnetic microscopy. By comparing results obtained from structures with one or two different activation energies, we demonstrate a clear impact on the resulting magnetic order. The differences are obtained by the analysis of the magnetic spin structure factors, in which the role of the activation energies is manifested by distinct short-range order. Furthermore, these results highlight the potential of artificial spin-ice structures to serve as model systems for designing various energy-scale hierarchies and investigating their impact on the collective dynamics and magnetic order.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

DOE OSTI2018

Interaction modifiers in artificial spin ices

The modification of geometry and interactions in two-dimensional magnetic nanosystems has enabled a range of studies addressing the magnetic order, collective low-energy dynamics and emergent magnetic properties in, for example, artificial spin-ice structures. The common denominator of all these investigations is the use of Ising-like mesospins as building blocks, in the form of elongated magnetic islands. Here, we introduce a new approach: single interaction modifiers, using slave mesospins in the form of discs, within which the mesospin is free to rotate in the disc plane1. We show that by placing these on the vertices of square artificial spin-ice arrays and varying their diameter, it is possible to tailor the strength and the ratio of the interaction energies. We demonstrate the existence of degenerate ice-rule-obeying states in square artificial spin-ice structures, enabling the exploration of thermal dynamics in a spin-liquid manifold. Furthermore, we even observe the emergence of flux lattices on larger length scales, when the energy landscape of the vertices is reversed. In conclusion, the work highlights the potential of a design strategy for two-dimensional magnetic nano-architectures, through which mixed dimensionality of mesospins can be used to promote thermally emergent mesoscale magnetic states.

77 NANOSCIENCE AND NANOTECHNOLOGY↗