Development of Nuclear Data Measurements Capabilities at the Spallation Neutron Source
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Engineering topics
Publications and source records attributed to Karriem, Zain.
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Alumina-forming austenitic (AFA) stainless steels have emerged as a candidate alloy because of their high-temperature strength, formability, cost, and compatibility with primary coolants for lead-cooled fast reactors (LFRs). This class of steels has exceptional high-temperature oxidation performance; however, a high concentration of Ni is required to stabilize the austenite phase and to provide sufficient creep strength. AFA stainless steels are also susceptible to liquid metal embrittlement (LME). Additionally, under neutron irradiation, Ni will enrich at grain boundaries due to radiation-induced segregation (RIS). Nickel RIS can increase the LME under these coupled effects. Oak Ridge National Laboratory (ORNL) and the NSUF program have leveraged its High Flux Isotope Reactor (HFIR) and experience with complex irradiation experiments to design experiment capsules that test the aforementioned coupled effects. These capsules are designed for insertion in the central flux trap, the highest flux region, of HFIR. The experiment capsules will be filled with Pb, designed to passively melt from the gamma heating in HFIR. The specimens were fabricated into miniature tensile specimens from two different alloys, GA05-25Ni and GA05-20Ni, varying Ni concentrations. The experiment capsules are designed to achieve target temperatures of 400 °C and 650 °C with accumulated dosage of 3 dpa. This report documents the specimen alloy characterization, experimental design, and expected performance of the capsules.
High-density uranium nitride (UN) is a fuel candidate for several advanced nuclear reactor designs currently under development. Because there are limited UN performance data relative to fuel fabrication impurity and density variation, an irradiation campaign has been developed as part of a collaborative effort among the University of Texas at San Antonio (UTSA), Westinghouse Electric Company, Oak Ridge National Laboratory (ORNL), and Los Alamos National Laboratory (LANL) under the Nuclear Science User Facilities program. This project, entitled ROADRUNNER, or Research On ADvancing the peRformance of UraNium Nitrides in Extreme enviRonments, aimsto support UN fuel qualification for advanced reactors by investigating the impact of density and impurity variations on UN performance as a function of irradiation temperature and burnup. The MiniFuel experiment vehicle developed by ORNL, which leverages the High Flux Isotope Reactor, was selected to perform this accelerated separate-effects irradiation testing. The experiment test matrix consists of six MiniFuel targets containing miniature UN fuel disks, and targets three distinct burnup levels (37.5, 60, and 75 MWd/kg U) and three distinct temperatures (600, 900, and 1200°C). Neutronics and thermal analyses were performed to determine the experimental parameters needed to meet the desired irradiation conditions and to predict the experiment components temperatures. UN pellets were fabricated at LANL with tightly controlled parameters to produce specimens with three distinct densities and three levels of carbon content. The pellets were then thinned down by UTSA to the experiment-required thickness. The pre-characterization of the specimens includes density measurements, carbon and oxygen contents, microstructure analysis, and x-ray computed tomography. The selected specimens will be assembled into the MiniFuel experiment, and the first ROADRUNNER MiniFuel targets are intended for HFIR insertion during the Fall of 2024. After irradiation, the targets will be shipped to ORNL’s hot cell facility for disassembly. The post-irradiation examination on the fuel specimens includes fission gas release measurements, visual inspection, fuel swelling measurements, gamma spectroscopy, and microstructure analysis. The data collected post-irradiation will be used to develop fuel performance models.
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The Sustaining and Enhancing Nuclear Science Initiative at Oak Ridge National Laboratory (ORNL) was created to explore potential enhancements to scientific capabilities in the High Flux Isotope Reactor as part of a reactor pressure vessel replacement project. One proposed scientific enhancement included creation of an epithermal and fast neutron radiography station on the HB-3 beam tube with the capability to image highly radioactive specimens such as irradiated nuclear fuel rods, isotope production targets, or spallation neutron target materials. This document summarizes findings and recommendations from a working group of ORNL staff tasked with conceptualizing such a facility and includes a background of similar instruments at other research facilities, technical specifications, and an estimate of procurement cost and schedule.
In-core irradiation experiment research, such as materials and fuels irradiation research and radioisotope production, is one of the primary missions of Oak Ridge National Laboratory’s (ORNL) versatile High Flux Isotope Reactor (HFIR). In support of the HFIR-Sustaining and Enhancing Neutron Science (SENSe) Initiative, a technically diverse group of ORNL irradiation research subject matter experts formed the Spectrum Tailoring Working Group, with the goal of developing a compendium of experiment facility concepts to enhance irradiation experiment conditions via neutron spectrum tailoring capabilities. The purpose of this report is to document the concepts developed in FY22 and the associated scientific justifications, identify potential facility sponsors, and estimate costs and schedules for each concept. This report documents the efforts performed in FY22, which may continue in FY23 or later pending the direction of the HFIR-SENSe Initiative and the interested sponsors.
Completion of the originally planned critical facility has been considered as part of the High Flux Isotope Reactor (HFIR) Sustaining and Enhancing Neutron Science Initiative at Oak Ridge National Laboratory (ORNL). A working group of ORNL staff members was formed to develop the idea and to recommend one or more configurations to best support future HFIR operations and scientific capacities. HFIR was designed with a critical pool in the reactor bay that was projected to be outfitted as a critical facility. The primary purpose of the planned critical facility was to measure the subcritical worth of fresh fuel elements to support startup requirements. However, the Y-12 National Security Complex already housed a critical facility that was used for this purpose. This report presents the working group’s efforts, including determination of the proposed critical facility’s high-impact benefits. A generic low-power critical facility would be employed for reactor physics measurements, code and data validation, reactor operator and staff training, and education. This facility would be instrumental in supporting current HFIR operations, conversion of HFIR to low-enriched uranium, existing light water reactor operations, and advanced reactor development and deployment.
As part of the Sustaining and Enhancing Nuclear Science (SENSe) initiative at Oak Ridge National Laboratory (ORNL), the prospect of adding new detection systems to support High Flux Isotope Reactor (HFIR) operations and to advance scientific research has prompted many ideas and discussions regarding potential features, configurations, locations, and applications. A working group of ORNL staff members was organized to further develop the concepts and recommending one or more configurations to best support future HFIR operations and scientific capacities and to provide order-of-magnitude cost estimates and timing. The areas of investigation included fast access detection systems, non-scattering beamline instruments, shielded detection instruments, and an ultracold neutron source. In each case, the focus was to develop world leading capabilities that would be unmatched by any other facility.
Niowave is seeking to develop a commercial medical isotope production process using a low-enriched uranium accelerator-driven subcritical reactor (ADSR) system to produce molybdenum-99. As part of the US Department of Energy national laboratory support to develop low enriched uranium molybdenum-99 production technologies, Oak Ridge National Laboratory is providing research and development resources to assist Niowave in the design and licensing process of its technology. The goals of this work under the radiation shielding task are to assist Niowave in developing a methodology and framework for efficient radiation shielding simulations of their Uranium Target Assembly 2 facility and to provide preliminary radiation shielding calculations and design recommendations for the facility.
This report presents the work that was performed to determine the neutron energy spectrum (spectrum) of the Multi-Mission Radioisotope Thermoelectric Generator (MMRTG) with a neutron Multi-Sphere Spectrometer (MSS). The spectrometer measurements were performed when the generator is in an INL Materials and Fuels Complex (MFC) laboratory. The measurements were used in a spectrum unfolding software to calculate the neutron spectrum. Based on initial testing of the MSS spectrometer and experience with the unfolding software, an MMRTG spectrum is reported and a justification for the spectrum is provided.