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Kossler, W. J.

Publications and source records attributed to Kossler, W. J..

Studies of superconducting materials with muon spin rotation

The muon spin rotation/relaxation technique was found to be an exceptionally effective means of measuring the magnetic properties of superconductors, including the new high temperature superconductor materials, at the microscopic level. The technique directly measures the magnetic penetration depth (type II superconductors (SC's)) and detects the presence of magnetic ordering (antiferromagnetism or spin-glass ordering were observed in some high temperature superconductor (HTSC's) and in many closely related compounds). Extensive studies of HTSC materials were conducted by the Virginia State University - College of William and Mary - Columbia University collaboration at Brookhaven National Laboratory and TRIUMF (Vancouver). A survey of LaSrCuO and YBaCaCuO systems shows an essentially linear relationship between the transition temperature T(sub c) and the relaxation rate. This appears to be a manifestation of the proportionality between T(sub c) and the Fermi energy, which suggests a high energy scale for the SC coupling, and which is not consistent with the weak coupling of phonon-mediated SC. Studies of LaCuO and YBaCuO parent compounds show clear evidence of antiferromagnetism. YBa2Cu(3-x)CO(x)O7 shows the simultaneous presence of spin-glass magnetic ordering and superconductivity. Three-dimensional SC, (Ba, K) BiO3, unlike the layered CuO-based compounds, shows no suggestion of magnetic ordering. Experimental techniques and theoretical implications are discussed.

Davis, Michael R.↗

Comparison between muon spin rotation and neutron scattering studies on the 3-dimensional magnetic ordering of La2CuO(4-y)

Muon spin rotation and neutron scattering studies on powder and single-crystal specimens of La2CuO(4-y) are compared. The apparent difference between the muon and neutron results for the ordered moment in the antiferromagnetic state is interpreted as the signature of increasingly short-ranged spatial spin correlations with increasing oxygen content.

Uemura, Y. J.↗

Coexisting static magnetic ordering and superconductivity in CeCu2.1Si2 found by muon spin relaxation

Zero- and longitudinal-field muon spin relaxation measurements on a heavy fermion system CeCu2.1 Si2 have revealed an onset of static magnetic ordering below T(M) approximately 0.8 K, which coexists with superconductivity below T(c) = 0.7 K. The line shapes of the observed muon spin depolarization functions suggest an ordering in either spin glass or incommensurate spin-density-wave state, with a small averaged static moment of the order of 0.1 micro-B per formula unit at T approaches 0.

Uemura, Y. J.↗

Static magnetic ordering of CeCu2.1Si2 found by muon spin relaxation

Zero- and longitudinal-field muon spin relaxation measurements on a polycrystal sample of a heavy fermion superconductor CeCu2.1 Si2 (T(c) = 0.7 K) have revealed an onset of static magnetic ordering below T approximately 0.8 K. The line shapes of the observed spectra in zero field indicate a wide distribution of static random local fields at muon sites, suggesting that the ordering is either spin glass or incommensurate spin-density-wave state. The observed width of the random local field at T = 0.05 K corresponds to a small averaged static moment of the order of 0.1 micro-B per formula unit.

Uemura, Y. J.↗

Muon motion in titanium hydride

Motional narrowing of the transverse-field muon spin rotation signal was observed in gamma-TiH(x) for x = 1.83, 1.97, and 1.99. An analysis of the data for TiH1.99 near room temperature indicates that the mechanism responsible for the motion of the muon out of the octahedral site is thermally activated diffusion with an attempt frequency comparable to the optical vibrations of the lattice. Monte Carlo calculations to simulate the effect of muon and proton motion upon the muon field-correlation time were used to interpret the motional narrowing in TiH1.97 near 500 K. The interpretation is dependent upon whether the Bloembergen, Purcell, and Pound (BPP) theory or an independent spin-pair relaxation model is used to obtain the vacancy jump rate from proton NMR T1 measurements. Use of BPP theory shows that the field-correction time can be obtained if the rate of motion of the muon with respect to the rate of the motion for the protons is decreased. An independent spin-pair relaxation model indicates that the field-correlation time can be obtained if the rate of motion for the nearest-neighbor protons is decreased.

Kempton, J. R.↗

Antiferromagnetism of La2CuO(4-y) studied by muon-spin rotation

Zero-field spin precession of positive muons has been observed in the antiferromagnetic state of La2CuO(4-y). Sharp onsets of the sublattice magnetization are found at temperatures close to those of the susceptibility maxima of different specimens. The long-lived precession signal indicates a microscopically homogeneous distribution of spin density at each Cu atom below the Neel temperature. A combination of the present results and neutron-scattering studies indicates the ordered moment per Cu atom to be significantly less than 1 mu(B).

Uemura, Y. J.↗

Magnetic field penetration depth of La(1.85)Sr(0.15)CuO4 measured by muon spin relaxation

Muon-spin-relaxation measurements have been performed on a high-Tc superconductor La(1.85)Sr(0.15)CuO4. In an external transverse magnetic field of 500 G, a magnetic field penetration depth of 2000 A at T = 10 K has been determined from the muon-spin-relaxation rate which increased with decreasing temperature below Tc. From this depth and the Pauli susceptibility, the superconducting carrier density is estimated at 3 x 10 to the 21st per cu cm. The zero-field relaxation rates above and below Tc were equal, which suggests that the superconducting state in this sample is not associated with detectable static magnetic ordering.

Kossler, W. J.↗

Uniaxial stress induced symmetry breaking for muon sites in Fe

Uniaxial stress was used on Fe single crystals to induce muon precession frequency shifts. The frequency shift for a nominally pure Fe sample at 302K was -0.34 + or - .023 MHz per 100 microstrain along the 100 magnetization axis. This corresponds to a change of magnetic field at the muon of 25.1 + to 1.6G/100 magnetic moment. For an Fe (3wt%Si) single crystal the shifts were -0.348 + or - .008 MHz/100 magnetic moment. The agreement between the shifts for Fe and Fe(3wt%Si) shows the effect to be intrinsic to iron and not strongly impurity sensitive. These shifts and their temperature dependence (1/T) are dominated by the effect of strain inducted population shifts between crystallographically equivalent, but mgnetically inequivalent sites. Their magnitudes are in good agreement ith previous theoretical predictions and by previous extrapolation from calculations on Nb and V especially if both 4T(0) and 1T sites contribute comparably.

Kossler, W. J.↗

Absence of J/pi/, T = 0/+/, 1 level excitations in residual nuclei from /pi /+ or -/,2N/ reactions

Gamma-ray spectra taken in prompt coincidence with incident 180-MeV pi/+/, 220-MeV pi/-/ and 0-MeV pi/-/ on the self-conjugate targets C-12 and S-32 reveal that the cross sections/yields are equal to or near zero for production of the J/pi/,T = 0/+/, 1 levels of the odd Z, odd N nuclei resulting from np removal. It is thought that the 0-MeV pi/-/ results can be explained by selection rules governing one-step quasi-free interactions but that the delta(1232) region results cannot. This indicates that there may be additional restrictions upon the pion absorption mechanism.

Stronach, C. E.↗

Muon hyperfine fields in iron and its dilute alloys

The temperature dependence of the interstitial magnetic field, B, as determined by the rotation of the spin of the muon, has been measured for dilute polycrystalline iron alloys with Mo, Ti, and Nb additions over a temperature range of 240 to 633 K. In all cases the behaviors differ from one another and from the Fe(Al) alloys previously studied. B, which is negative with respect to the magnetization, is increased in magnitude by Al and Mo, and decreased greatly by Ti. The addition of Nb creates a two-phase alloy from which the role of heterogeneity and/or strain on B in iron can be assessed. If the temperature dependence of the hyperfine field extracted from B for Fe(Mo) alloys is interpreted on the model previously used to discuss the Fe(Al) data, then the muon must be attracted to the Mo atom while repelled by the Al atoms as the temperature decreases.

Stronach, C. E.↗

Magnetic environment of hydrogen in Fe from muon precession measurements

Polarized positive muon radiation was stopped in an ellipsoidal iron target and its precession was observed in a transverse magnetic field. Results indicate that the conduction electron polarization in the 77 K-Fe Curie point region is less than expected, and that the relaxation time of the muon polarization is dominated by the static inhomogeneity to 900 K, at which point magnetization fluctuations become important.

Heiman, N.↗