ENDF/B-VIII.1: Triton Reaction Sublibrary
The tritons sublibrary aims to describe nuclear reactions between incident triton particles and different nuclei. For ENDF/B-VIII.1, compared to ENDF/B-VIII.0, there were only evaluation updates for 4 He.
Engineering topics
Publications and source records attributed to Kravvaris, K..
The tritons sublibrary aims to describe nuclear reactions between incident triton particles and different nuclei. For ENDF/B-VIII.1, compared to ENDF/B-VIII.0, there were only evaluation updates for 4 He.
The β-decay properties of nuclei near the second nuclear “island of inversion” around neutron rich nuclei with neutron number 40 are important tests of nuclear structure models and interactions. In particular, the β-delayed neutron emission branch (Ρ n ), is useful for investigating β-strength and neutron-γ competition above the neutron separation energies of the daughter nuclei. We report new constraints for Ρ n values for three nuclei in the region: 62 Cr (Ρ n <1%), 64 Mn (Ρ n = 1.5(6)%), and 65 Fe (Ρ n < 1%), measured with the Neutron Emission Ratio Observer (NERO) neutron long counter system and the Beta Counting Station (BCS) at the National Superconducting Cyclotron Laboratory (NSCL). Our results resolve the large discrepancy between previous direct and indirect measurements for 64 Mn and confirm the predictions of global theoretical models when a statistical treatment of the γ and neutron decays of the daughter states is included. Here we also obtain improved half-lives for 62 Cr [206(5) ms] and the short-lived isomer in the 62 Fe daughter [112(7) ms] from β-delayed γ emission data obtained in the same experiment with the Summing NaI (SuN) total absorption spectrometer. Finally, we use γ emission data to obtain a new upper limit for the 62 Cr β-decay population of the long-lived isomeric state in 62 Mn.
Observations of anomalies in the electron-positron angular correlations in high-energy decays in 4 He, 8 Be, and 12 C have been reported recently by the ATOMKI collaboration. These could be explained by the creation and subsequent decay of a new boson with a mass of ≈ 17MeV. Theoretical understanding of pair creation in the proton capture reactions used in these experiments is important for the interpretation of the anomalies. We apply the ab initio no-core shell model with continuum (NCSMC) to the proton capture on 7 Li. The NCSMC describes both bound and unbound states in light nuclei in a unified way with chiral two- and three-nucleon interactions as the only input. We investigate the structure of 8 Be, the p+ 7 Li elastic scattering, the 7 Li(p,y) 8 Be cross section, and the internal pair creation 7 Li (p,e + e - ) 8 Be. Here we discuss the impact of a proper treatment of the initial scattering state on the electron-positron angular correlation spectrum and compare our results to available ATOMKI data sets. Finally, we calculate 7 Li (p,X) 8 Be cross sections for several proposed models of the hypothetical X17 particle.
Indirect methods have become the predominant approach in experimental nuclear astrophysics for studying several low-energy nuclear reactions occurring in stars, as direct measurements of many of these relevant reactions are rendered infeasible due to their low reaction probability. Such indirect methods, however, require theoretical input that in turn can have significant poorly quantified uncertainties, which can then be propagated to the reaction rates and have a large effect on our quantitative understanding of stellar evolution and nucleosynthesis processes. Here we present two such examples involving α-induced reactions, 13 C (α,n) 16 O and 12 C (α,γ) 16 O, for which the low-energy cross sections have been constrained with ( 6 Li,d) transfer data. In this Letter, we discuss how a first-principle calculation of 6 Li leads to a 21% reduction of the 12 C(α,γ) 16 O cross sections with respect to a previous estimation. This calculation further resolves the discrepancy between recent measurements of the 13 C (α,n) 16 O reaction and points to the need for improved theoretical formulations of nuclear reactions.
The purpose of this report is to document the effects of including excited states of 239 Pu in the calculation of transmission coefficients that will serve as inputs to Hauser-Feshbach calculations of neutron-induced reactions.
Deuteron-induced nuclear reactions are an essential tool for probing the structure of nuclei as well as astrophysical information such as (n, γ) cross sections. The deuteron-nucleus system is typically described within a Faddeev three-body model consisting of a neutron (n), a proton (p), and the target nucleus (A) interacting through pairwise phenomenological potentials. While Faddeev techniques enable the exact description of the three-body dynamics, their predictive power is limited in part by the omission of irreducible neutron-proton-nucleus three-body force (n–p–A 3BF). Here, our goal is to quantify systematic uncertainties stemming from the reduction of deuteron-nucleus (d + A) dynamics to a picture of three pointlike nuclear clusters interacting via pairwise nucleon-nucleus forces, using as testing grounds d + α scattering and the 6 Li ground state. We particularly focus on quantifying uncertainties arising from the full antisymmetrization of the (A + 2)-body system with the target nucleus fixed in its ground state. We adopt the ab initio no-core shell model coupled with the resonating group method (NCSM/RGM) to compute microscopic n–α and p–α interactions, and use them in a three-body description of the d + α system by means of momentum-space Faddeev-type equations. Simultaneously, we also carry out ab initio calculations of d + α scattering and 6 Li ground state by means of six-body NCSM/RGM calculations to serve as a benchmark for the three-body model predictions given by the Faddeev calculations. By comparing the Faddeev and NCSM/RGM results, we show that the irreducible n–p–α 3BF has a non-negligible effect on bound state and scattering observables alike. Specifically, the Faddeev approach yields a 6 Li ground state that is approximately 600 keV shallower than the one obtained with the NCSM/RGM. Additionally, the Faddeev calculations for d + α scattering yield a 3 + resonance that is located approximately 400 keV higher in energy compared to the NCSM/RGM result. The shape of the d + α angular distributions computed using the two approaches also differ, owing to the discrepancy in the predictions of the 3 + resonance energy. The Faddeev three-body model predictions for d + α scattering and 6 Li using microscopic n–α and p–α potentials differ from those computed microscopically with the NCSM/RGM. These discrepancies are due to the n–p–α 3BF, which arises from two-nucleon exchange terms in the microscopic d–α interaction and are not accounted for in the three-body model Faddeev calculations. This study lays the foundation for future parametrizations of the 3BF due to Pauli exclusion principle effects in improved three-body calculations of deuteron-induced reactions.
This experimental study of high-spin structure near the N = Z = 20 region focuses on 41 K and also reports three newly observed γ transitions in 41 Ca from the same reaction. High-spin states were populated using the 26 Mg( 18 O, p2nγ) 41 K and 26 Mg( 18 O, 3nγ) 41 Ca reactions at a beam energy of 50 MeV at the Florida State University John D. Fox Superconducting Linear Accelerator Laboratory, employing the FSU high-purity germanium detector array. The level scheme of 41 K was extended to 12325 keV, possibly up to J π = 25/2 − or 27/2 + , by means of 25 new γ-ray transitions, and that of 41 Ca to 9916 keV. Linear polarization and angular-distribution measurements were used to provide spin and parity information for several states in the 41 K decay scheme. The results are compared with spsdpf cross-shell shell-model calculations using the FSU interaction. Configurations involving zero or one nucleon promoted from the sd to the fp shell reproduce the energies of many known states reasonably well, while multi-particle excitations reveal a more complex interplay of single-particle motion, collective pairing, and deformation, posing an interesting challenge for future theoretical work.
In this work, the exotic β -delayed proton emission is calculated in 11 Be from first principles using chiral two- and three-nucleon forces. To investigate the unexpectedly large branching ratio measured in Ayyad et al. [Phys. Rev. Lett. 123, 082501 (2019)], we calculate the proposed (1/2 + , 1/2) proton resonance in 11 B using the no-core shell model with continuum. This calculation helps to address whether this enhancement is caused by unknown dark decay modes or an unobserved proton resonance. We report a branching ratio of $b_p$ = (1.3 ± 0.5) × 10 –6 , suggesting that its unexpectedly large value is caused by an unobserved proton resonance in 11 B.
Excited states in O 13 were investigated using inelastic scattering of an E / A = 69.5 MeV O 13 beam off of a Be 9 target. The excited states were identified in the invariant-mass spectra of the decay products. Both single-proton and sequential two-proton decays of the excited states were examined. Furthermore, for a number of the excited states, the protons were emitted with strong anisotropy where emissions transverse to the beam axis are favored. The measured proton-decay angular distributions were compared to predictions from distorted-wave Born-approximation calculations of the spin alignment which was shown to be largely independent of the excitation mechanism. The deduced O 13 level scheme is compared to ab initio no-core shell model with continuum predictions. The lowest-energy excited states decay isotropically consistent with predictions of strong proton 1 s 1 / 2 structure. Above these states in the level scheme, we observed a number of higher-spin states not predicted within the model. Possibly these are associated with rotational bands built on deformed cluster configurations predicted by antisymmetrized molecular dynamics calculations. The spin alignment mechanism is shown to be useful for making spin assignments and may have widespread use.
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The higher-spin structure of 38 Cl ($N=21$) was investigated following the 26 Mg( 14 C, $pn$) reaction at 30 and 37 MeV beam energies. The outgoing protons were detected in an $E-ΔE$ Si telescope placed at 0° close to the target with a Ta beam stopper between the target and telescope. Multiple $γ$ rays were detected in time coincidence with the protons using an enhanced version of the FSU $γ$-detection array. The level scheme was extended up to 8420 keV with a likely spin of 10 $ℏ$. A new multishell interaction was developed guided by the experimental information. This FSU interaction was built by fitting to the energies of 270 experimental states from 13 C to 51 Ti. Calculations using the FSU interaction reproduce observed properties of 38 Cl rather well, including the spectroscopic factors. The interaction has been successfully used to interpret the 1p1h and 2p2h configurations in some nearby nuclei as well.
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$β^-$ decay of $T_z$ = +$\frac{11}{2}$ nuclei $\mathrm{^{37}Al}$ and $\mathrm{^{39}Si}$ was studied to obtain information about excited states in the daughter and granddaughter nuclei. New information on excited states has been obtained for $\mathrm{^{37,39}P}$ whereas level schemes for $\mathrm{^{37}Si}$ and $\mathrm{^{37,39}S}$ were confirmed and expanded on as compared to the most recent investigations. For the nuclei studied, the valence proton and neutron occupy different major shells with opposite parities, hence, the $β^-$ decay preferentially and primarily populates core-excited $1p1h$ intruder states with a parity opposite to the ground state of the daughter nucleus. These low-lying intruder states shed light on the $N = 20$ shell gap and its evolution with neutron number. The $β^-$ decay of very neutron-rich nuclei also illustrates how the Gamow-Teller (GT) strength distribution changes with neutron excess. Comparing $β^-$ decay of $\mathrm{^{37,39}Si}$ presented here with $\mathrm{^{38,40}Si}$ from a previous study, we clearly see an even-odd effect in the GT strength distribution with the decay from even-even nuclei showing strong low-lying strength whereas for the odd $A$ being very fragmented. Finally, configuration interaction shell-model calculations with the state-of-art SDPFSDG-MU effective interaction were performed to understand the structure of the $1p1h$ states and explore the GT strength distribution.
High-spin states in $\mathrm{^{39}Ar}$ were populated using the $\mathrm{^{27}Al(^{14}C,} pn)$ reaction at 25.6 MeV. The de-exciting $γ$ rays were measured with the FSU $γ$ detector array along with evaporation protons in a Si $E-ΔE$ telescope. The known high-spin level scheme was extended up to over 11 MeV with a dozen new levels above the neutron decay threshold. The decay pattern appears somewhat atypical for heavy-ion fusion-evaporation reactions. The structure of $\mathrm{^{39}Ar}$ is discussed in terms of the new FSU cross-shell $spsdpf$ interaction fitted to a wide range of nuclei. This interaction has proved quite successful in accounting for the level scheme of $\mathrm{^{39}Ar}$, including the previously suggested fully aligned $πf_{7/2} Ⓧ νf_{7/2}17/2^+$ state and previously discovered analogs of the lowest states in $\mathrm{^{39}Cl}$.
Here, excited states in the neutron-rich isotopes P 33 and P 34 were populated by the O 18 + O 18 fusion-evaporation reaction at E lab = 24 MeV. The Gammasphere array was used along with the Microball particle detector array to detect γ transitions in coincidence with the charged particles emitted from the compound nucleus S 36 . The use of Microball enabled the selection of the proton emission channel. It also helped in determining the exact position and energy of the emitted proton; this was later employed in kinematic Doppler corrections. 16 new transitions and 13 new states were observed in P 33 and 21 γ rays and 20 energy levels were observed in P 34 for the first time. The nearly 4 π geometry of Gammasphere allowed the measurement of γ -ray angular distributions leading to spin assignments for many states. The experimental observations for both isotopes were interpreted with the help of shell-model calculations using the (0+1) ℏ ω PSDPF interaction. The calculations accounted for both the 0p-0h and 1p-1h states reasonably well and indicated that 2p-2h excitations might dominate the higher-spin configurations in both P 33 and P 34 .
The Si-31 nucleus was produced through the O-18(18O, an) fusion-evaporation reaction at E-lab = 24 MeV. Evaporated a particles from the reaction were detected and identified in the Microball detector array for channel selection. Multiple gamma-ray coincidence events were detected in Gammasphere. The energy and angle information for the alpha particles was used to determine the Si-31 recoil kinematics on an event-by-event basis for a more accurate Doppler correction. A total of 22 new states and 52 new gamma transitions were observed, including 14 from states above the neutron separation energy. The positive-parity states predicted by the shell-model calculations in the sd model space agree well with experiment. The negative-parity states were compared with shell-model calculations in the psdpf model space with some variations in the N = 20 shell gap. The best agreement was found with a shell gap intermediate between that originally used for A approximate to 20 nuclei and that previously adapted for P-32,P-34. This variation suggests the need for a more universal cross-shell interaction.
We present techniques that allow for α-cluster channels with realistic α-particle wave functions from No Core Shell Model calculations to be constructed. We compare results of several clustering calculations with realistic α wave functions to those assuming a trivial (0s) 4 structure.
Low-lying excited states in P 38,40 have been identified in the β decay of T z =+5,+6, Si 38,40 . Based on the allowed nature of the Gamow-Teller (GT) decay observed, these states are assigned spin and parity of 1 + and are core-excited 1p1h intruder states with a parity opposite to the ground state. The occurrence of intruder states at low energies highlights the importance of pairing and quadrupole correlation energies in lowering the intruder states despite the N=20 shell gap. Configuration interaction shell model calculations with the state-of-art SDPF-MU effective interaction were performed to understand the structure of these 1p1h states in the even-A phosphorus isotopes. States in P 40 with N=25 were found to have very complex configurations involving all the fp orbitals leading to deformed states as seen in neutron-rich nuclei with N≈28. The calculated GT matrix elements for the β decay highlight the dominance of the decay of the core neutrons rather than the valence neutrons.