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Krzysztof Wargan

Publications and source records attributed to Krzysztof Wargan.

46 records · Page 3

Tropospheric Ozone in the NASA GEOS Model: Effects of Satellite Data Assimilation and Improvements in Background NO x Chemistry

Tropospheric ozone is a major atmospheric oxidant, the primary source of the hydroxyl radical, and a greenhouse gas. In the troposphere, it is produced from the oxidation of carbon monoxide and volatile organic compounds in the presence of nitrogen oxides (NO x =NO+NO 2 ) or has its origins in the stratosphere. The tropospheric ozone burdens in global atmospheric chemistry models disagree by a factor of 1.5, indicating an incomplete understanding of ozone sources and sinks. Here we examine the tropospheric ozone simulation in NASA Global Modeling and Assimilation Office’s (GMAO’s) GEOS model with the GEOS-Chem chemistry mechanism (version 14.2), using observations from satellites, aircraft, ozonesondes, and surface sites. This modeling framework is used to produce GMAO’s GEOS Composition Forecasts (GEOS-CF), and it has been updated extensively with new emission inventories, improved model physics, satellite data assimilation capability, and an up-to-date chemical mechanism that includes tropospheric halogen chemistry and NOx recycling from particulate nitrate. Earlier versions of the model using GEOS-Chem version 12.0 showed an underestimate in tropospheric ozone in the northern hemisphere. We evaluate the ozone simulation in the updated model, focusing on the effects of assimilating satellite NO 2 data from the Ozone Monitoring Instrument (OMI), constraining stratospheric ozone to satellite data, and updates to the NOx chemistry. We will examine changes in the vertical profiles of tropospheric ozone over the US in support of the Tropospheric Emissions: Monitoring of Pollution (TEMPO), and discuss implications for the tropospheric ozone budget.

Viral Shah↗

Hunga Tonga-Hunga Ha’apai Water Vapour and Composition of the Stratospheric Polar Vortices

We investigate the impacts of water vapor from the Hunga Tonga-Hunga Ha'apai (HTHH) eruption on the Antarctic stratospheric vortices in 2022 and 2023 and the Arctic stratospheric vortex in 2022/2023. Trace gas abundances from the Aura Microwave Limb Sounder (MLS) and the Modern Era Retrospective-analysis for Research and Applications (MERRA-2) Stratospheric Composition REanalysis with Aura MLS (M2-SCREAM), along with meteorological fields from the longer MERRA-2 record, are used to detail the evolution of the stratospheric polar vortex and its composition during these winter/spring seasons. Through austral winter and spring 2022, HTHH water vapor was effectively excluded from the Antarctic vortex until it broke up. The 2022 Antarctic vortex itself was large, strong, and long-lived, but not exceptionally so. By austral fall 2023, HTHH stratospheric water vapor had spread globally, and Antarctic vortex values in the lower through middle stratosphere were over 2 ppmv higher than usual when the vortex formed; these record-shattering water vapor concentrations led to earlier polar stratospheric cloud formation and chlorine activation, especially at levels that are typically the highest altitudes for polar processing. In the 2022/2023 Arctic winter/spring, HTHH water vapor reached the Arctic vortex region after the vortex had formed and was largely excluded until a major sudden stratospheric warming in mid-February 2023 eroded the vortex and mixed midlatitude and vortex air throughout the hemisphere.

Gloria L Manney↗

Broadening Systematic Reanalysis lntercomparisons in the SPARC-Reanalysis lntercomparison Project Phase 2 (S-RIP2): Chemical Reanalyses & Air Quality, Tropospheric Circulation, Extreme Events, and More

Reanalysis datasets are widely used to understand numerous atmospheric processes. Different reanalyses may give very different results for the same diagnostics. The Stratosphere-troposphere Processes And their Role in Climate (SPARC) Reanalysis Intercomparison Project (S-RIP, https://s-rip.github.io/) is a coordinated activity to compare key diagnostics among available reanalyses, identify differences among reanalyses and their underlying causes, provide guidance on appropriate usage of reanalyses in scientific studies, and contribute to future improvements in the reanalysis products via collaborations with reanalysis centers and data users. S-RIP Phase 1 (completed in early 2022) focused primarily on the upper troposphere through the middle atmosphere and processes linking these regions to the troposphere and surface. We look forward to broadening our efforts in Phase 2 (S-RIP2), with new foci including studies of tropospheric circulation, extreme weather events, and their links to the stratosphere, and focusing on evaluation of chemical reanalyses, both those with a stratosphere / upper troposphere focus and those that focus on air quality applications. This presentation will provide a summary of Phase 1 results and discussion of future directions for S-RIP2, emphasizing applications to composition and chemistry studies as well as fostering capacity building for Early Career Scientists.

Sean M Davis↗

Relationships Between Variability in the Stratospheric Polar Vortex, Upper Tropospheric Jets, Tropopauses, and UTLS Ozone

The impacts of stratospheric polar vortex variations on upper troposphere / lower stratosphere (UTLS) circulation and composition are not well understood. We use stratospheric polar vortex geometry / strength diagnostics combined with characterisation of tropopauses and UTLS jets to show links between stratospheric polar vortex variability and regional variations in UTLS jet and tropopause characteristics. Polar vortex diagnostics are from Characterization and Analysis of Vortex Evolution using Algorithms for Region Tracking (CAVE-ART), while UTLS diagnostics are from JEt and Tropopause Products for Analysis and Characterization (JETPAC). We will present results showing UTLS jet and tropopause characteristics for strong and weak stratospheric vortex states (defined using vortex-focused metrics that are less dependent on geometry and position than commonly used diagnostics), as well as regional variations in correlations between CAVE-ART and JETPAC diagnostics. Furthermore, we will focus on preliminary results extending the stratospheric vortex, UTLS jet, and tropopause relationships to assess their impacts on regional ozone variations diagnosed from the M2-SCREAM (MERRA-2 Stratospheric Composition Reanalysis of Aura Microwave Limb Sounder) composition reanalysis.

Gloria Manney↗

Trends in Asian Summer Monsoon Anticyclone Dynamical Diagnostics in Reanalyses

The area of the Asian summer monsoon anticyclone (ASMA), as defined by contours of Montgomery stream function (MSF) on isentropic surfaces, has been increasing over at least the last four decades. Here we analyze the relationship of the trend in ASMA area to trends in dynamical diagnostics in the ASM region, both inside and outside the ASMA, for 1979 through 2020 in the MERRA-2, JRA-55, and ERA5 reanalyses. Trends in geopotential height (GPH) and temperature (from which MSF is calculated) indicate that MSF increases are dominated by increasing temperature (GPH) at levels that are primarily in the troposphere (stratosphere). Trends in MSF, GPH, and temperature are much less clear within the ASMA circulation than those for the entire ASM region, suggesting that other mechanisms, besides the direct effects of increasing tropospheric temperatures, are at play. To further explore these results, we present trends in lapse rate and dynamical tropopause altitudes, easterly and westerly windspeeds bounding the ASMA, and potential vorticity. Overall, weak or inconsistent trends inside the ASMA in most diagnostics likely arise from a complex interplay of mechanisms in this region (which spans tropospheric/stratospheric and tropical/midlatitude conditions), and suggest that the previously reported area trends do not necessarily indicate an increase in “intensity" of the ASMA. In regions both with and without robust trends in dynamical diagnostics, trend results are typically consistent between the three reanalyses studied even when there are biases in the magnitudes of those diagnostics. This generally good agreement indicates that these reanalyses are suitable for more detailed studies needed to fully understand the mechanisms for trends in the ASMA.

Gloria Manney↗

Broadening Systematic Reanalysis Intercomparisons in the SPARC-Reanalysis Intercomparison Project Phase 2 (S-RIP2): Chemical Reanalyses & Air Quality, Tropospheric Circulation, Extreme Events, and More

Reanalysis datasets are widely used to understand numerous atmospheric processes. Different reanalyses may give very different results for the same diagnostics. The Stratosphere-troposphere Processes And their Role in Climate (SPARC) Reanalysis Intercomparison Project (S-RIP, https://s-rip.github.io/) is a coordinated activity to compare key diagnostics among available reanalyses, identify differences among reanalyses and their underlying causes, provide guidance on appropriate usage of reanalyses in scientific studies, and contribute to future improvements in the reanalysis products via collaborations with reanalysis centers and data users. S-RIP Phase 1 (completed in early 2022) focused primarily on the upper troposphere through the middle atmosphere and processes linking these regions to the troposphere and surface. We look forward to broadening our efforts in Phase 2 (S-RIP2), with new foci including studies of tropospheric circulation, extreme weather events, and their links to the stratosphere, and focusing on evaluation of chemical reanalyses, both those with a stratosphere / upper troposphere focus and those that focus on air quality applications. This presentation will provide a summary of Phase 1 results and discussion of future directions for S-RIP2, emphasizing applications to composition and chemistry studies as well as fostering capacity building for Early Career Scientists.

Sean M Davis↗

Composition Reanalyses at NASA’s Global Modeling and Assimilation Office

Scientific Assessments of Ozone Depletion 2018 and 2022 report the recovery of Antarctic ozone, consistent with diminishing concentrations of halogens in the stratosphere. Both the size and the depth of the springtime ozone holes exhibit downward trends, particularly in September. Superimposed on the recovery trend are significant year-to-year fluctuations arising from dynamical variability potentially influenced by climate forcing and volcanic eruptions. Since 2018 the Antarctic stratosphere has experienced a wild parade of austral spring seasons with a sudden stratospheric warming and exceptionally high ozone in 2019 followed by large and long-lasting ozone holes in the following years, prompting questions about the speed and detectability of Antarctic ozone recovery and its potential connections to human-induced climate change. From the Australian New Years’ wildfires of 2020 to volcanic aerosols to the unprecedented injection of water vapor by the Hunga volcanic eruption, recent scientific literature on the subject investigates many factors that may or may not have contributed to this remarkable interannual variability. This presentation summarizes dynamical influences on springtime Antarctic stratospheric ozone in recent years and discusses these results in the context of long-term trends. In particular, this work seeks to isolate dynamical and chemical contributions to the Antarctic springs since 2019 using a consistent methodological framework. Our analysis uses constituent and meteorological fields from the MERRA-2 Stratospheric Composition Reanalysis of Aura MLS (M2-SCREAM) in combination with data from the Atmospheric Chemistry Experiment – Fourier Transform Spectrometer and from ozone sondes. Using the high spatial and temporal resolution of M2-SCREAM, we analyze the daily evolution of southern polar ozone, HCl, N2O, and water vapor in dynamical flow-following coordinates relative to the location, size, and shape of the polar vortex. For vertically integrated stratospheric ozone we emphasize the importance of the wave-influenced geometry of the polar vortex and its vertical alignment. The ultimate purpose of this project is to contribute to the quantification of the speed of the Antarctic ozone recovery and associated uncertainties.

Krzysztof Wargan↗

How Unusual Were the 2020-2023 Ozone Holes?

The Scientific Assessment of Ozone Depletion 2022 reports the recovery of Antarctic ozone, particularly evident in September, consistent with diminishing concentrations of halogens in the stratosphere. Superimposed on the recovery trend are significant year-to-year fluctuations arising from dynamical variability and potentially influenced by climate forcing and volcanic eruptions. Since 2018 the Antarctic stratosphere has experienced large swings in Antarctic springtime ozone metrics with a sudden stratospheric warming and exceptionally high ozone in 2019 followed by large and long-lasting ozone holes in the following years, prompting questions about the speed and detectability of Antarctic ozone recovery and its potential connections to human-induced climate change.

Krzysztof Wargan↗