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Kulkarni, Gourihar

Publications and source records attributed to Kulkarni, Gourihar.

14 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Performance of pumped counterflow virtual impactors to study aerosol interactions with laboratory generated warm clouds

Pumped Counterflow Virtual Impactors (PCVI) are designed to separate aerosols based on aerodynamic diameter, which is particularly useful for isolating cloud droplets and ice crystals from smaller particles. However, the PCVI transmission efficiency (TE) values reported in the literature show considerable variability, and little information is available on the TEs for cloud liquid droplets. Here, we determined the optimal flow conditions for PCVI sampling for different activation ratios from the MTU Pi-cloud chamber, highlighting the conditions that maximize droplet residual sampling while minimizing interstitial transmission. Even for a lower limit cloud activation ratio = 1:10, an add flow of 1.5 LPM achieves a residual fraction greater than 0.80, with a droplet TE of ∼15% for typical Pi-Chamber droplets with diameters between 3.5 to 10 µm. This framework can be adapted for field cloud measurements based on the cloud conditions of interest. TE for cloud droplets under flow conditions at which ∼99% of the unactivated submicron particles were removed was substantially lower between 8 and 16% than for supermicron dry particles (∼30 to 40% for 3 µm polystyrene latex spheres). In addition, we conducted a comparison of the performances of three similar PCVI units to assess repeatability for dry aerosols and cloud droplets. All three PCVIs performed similarly in rejecting submicron particles smaller than the desired cutoff diameter. One of the units showed lower TEs due to a misalignment of the internal orifice. We discuss a procedure that improved alignment and performance.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Data associated with the manuscript “Radiative impact of record-breaking wildfires from integrated ground-based data” collected in Richland, Washington in September 2020

This data package is associated with the publication “Radiative impact of record-breaking wildfires from integrated ground-based data” submitted to Nature Scientific Reports (Kassianov et al., 2024). Data from ground-based measurements of shortwave and spectrally resolved irradiance and aerosol optical depth (AOD) in the visible and near-infrared spectral ranges were assessed to quantify the radiative impact of the September 2020 wildfires that occurred in the Western United States. Data were collected in September 2020 by several ground-based instruments at the Atmospheric Measurements Laboratory (AML) located in Richland, Washington (46.3451, -119.2792). These data include (1) Aerosol Optical Depth (AOD); (2) spectrally resolved and shortwave (SW) irradiances; (3) backscatter profiles; (4) total sky images; and (5) near-surface ambient air temperatures.The data package consists of five sub-directories: (1) “AML_Ceilometer_”; (2)” AML_CSPHOT_”; (3) “AML_MFRSR_irradiances_”; (4) “AML_SW_irradiances_and_Temp_”; (5) “AML_TSI_images_”; and 6 files stored at the directory level, including the readme, file-level metadata file, and data dictionary. The file-level metadata file (the file ending in “_flmd.csv”) lists all files contained in this data package and descriptions for each. The data dictionary (the file ending in “_dd.csv”) describes each tabular column header’s unit, definition, and structure. Below are descriptions of each sub-directory:“AML_Ceilometer_” includes ceilometer data collected at the AML. These files contain the corresponding narratives of data. Details related to the ceilometer data can be found in Morris (2016). “AML_CSPHOT_” includes ascii files with high-temporal resolution (about 10-15 min) AML CSPHOT data and their daily-averaged counterparts. These two files contain the corresponding narratives of data. Details related to the CSPHOT data can be found in Gregory (2011). “AML_MFRSR_irradiances_” includes ascii files with the AML MFRSR-measured diffuse, normal, and total spectrally resolved irradiance. Details related to the MFRSR data can be found in Hodges and Michalsky (2016) and Koontz et al. (2013). “AML_SW_irradiances_+_Temp_” includes near-surface ambient air temperature and SW irradiances, namely direct normal, diffuse hemispherical, and total hemispheric (global), measured at the AML. These files also incorporate the corresponding narratives of data. Details related to the SW irradiances can be found in Andreas et al. (2018). “AML_TSI_images_” includes Total Sky Images (TSIs) collected at the AML. Details related to the TSI data can be found in Morris (2005).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Retrieved Number Concentration of Cloud Condensation Nuclei (RNCCN) Profile Value-Added Product Report

The cloud condensation nuclei (CCN) concentration at cloud base is the most relevant measure of the aerosol that influences droplet formation in clouds. Since the CCN concentration depends on supersaturation, a more general measure of the CCN concentration is the CCN spectrum (values at multiple supersaturations). The CCN spectrum is now measured at the surface at several U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility observatories and by the ARM Mobile Facility (AMF) but is not measured at the cloud base. Rather than rely on expensive aircraft measurements for all studies of aerosol effects on clouds, a way to project CCN observations made at the surface to cloud base is needed. Remote sensing of aerosol extinction provides information about the vertical profile of the aerosol but cannot be directly related to the CCN concentration because the aerosol extinction is strongly influenced by humidification, particularly near cloud base. Ghan and Collins (2004) and Ghan et al. (2006) propose a method to remove the influence of humidification from the extinction profiles and tie the “dry extinction” retrieval to the surface CCN concentration, thus estimating the CCN profile. This methodology has been implemented as ARM’s Retrieved Number Concentration of CCN (RNCCN) Profile Value-Added Product (VAP).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Cloud Condensation Nuclei Hygroscopicity Value-Added Product Report

The purpose of the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility’s Cloud Condensation Nuclei Hygroscopicity Parameter (AOSCCNSMPSKAPPA and AOSCCNUHSASKAPPA) Value-Added Product (VAP) is to calculate the hygroscopicity parameter, kappa, to quantify the ability of aerosols to activate into cloud water droplets. The hygroscopicity parameter is often used to model the cloud condensation nuclei (CCN) activity of atmospheric aerosols of different sizes and compositions, providing additional insight on the influence of aerosols on climate. The AOSCCNUHSASKAPPA VAP was recently developed to provides kappa data for ARM sites where AOSCCNSMPSKAPPA was missing.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

aosccnuhsaskappa.c1

Hygroscopicity parameter kappa derived from CCN and UHSAS data sources

54 ENVIRONMENTAL SCIENCES↗