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Kurz, N.

Publications and source records attributed to Kurz, N..

17 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

New insight into knockout reactions from the two-proton halo nucleus 17 Ne

The unexplained disagreement in the dependence of spectroscopic factors (𝐶2⁢𝑆 exp ) on the binding energy obtained by nucleon knockout using different targets is still a puzzle that needs to be addressed. To find an explanation of this riddle through exclusive measurements using different targets. The exclusive measurements were performed by using a 17 Ne beam with an energy of 500 MeV/u incident on C and CH 2 targets. Through the standard theoretical approach, 𝐶 2⁢ 𝑆 exp were derived from the analysis of the experimental data on proton ejection from the proton halo in 17 Ne as well as from its core 15 O. For the C target, proton ejection from the proton halo gave 𝐶 2 ⁢𝑆 exp about 37% smaller than for the H target. But when protons are ejected from the core of 17 Ne, 𝐶 2 ⁢𝑆 exp are identical within statistical uncertainties. An explanation for the difference in 𝐶 2 ⁢𝑆 exp could be the removal of both halo protons, a more important reaction pathway for the C target. The 𝐶 2 ⁢𝑆 exp values obtained by analyzing the proton ejection from the core indicate that it is not affected by the interaction with the halo protons.

6 ≤ A ≤ 19↗
DOE OSTI2023

First spectroscopic study of odd-odd Cu 78

Nuclei in the vicinity of 78 Ni are important benchmarks for nuclear structure, which can reveal changes in the shell structure far from stability. Spectroscopy of the odd-odd isotope 78 CU was performed for the first time in an experiment with the EURICA setup at the Radioactive Isotope Beam Factory at RIKEN Nishina Center. Excited states in the neutron-rich isotope were populated following the β decay of 78 Ni produced by in-flight fission and separated by the BigRIPS separator. A level scheme based on the analysis of $\gamma$-$\gamma$ coincidences is presented. Tentative spin and parity assignments were made when possible based on the β -decay feeding intensities and $\gamma$-decay properties of the excited states. Time correlations between β and $\gamma$ decay show clear indications of an isomeric state with a half-life of 3.8(4) ms. Large-scale Monte Carlo shell-model calculations were performed using the A3DA-m interaction and a valence space comprising the full f p shell and the 1⁢g 9/2 and 2⁢d 5/2 orbitals for both protons and neutrons. The comparison of the experimental results with the shell-model calculations allows interpreting the excited states in terms of spin multiplets arising from the proton-neutron interaction. In conclusion, the results provide further insight into the evolution of the proton single-particle orbitals as a function of neutron number, and quantitative information about the proton-neutron interaction outside the doubly magic 78 Ni core.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

On the adsorption and reactivity of element 114, flerovium

Flerovium (Fl, element 114) is the heaviest element chemically studied so far. To date, its interaction with gold was investigated in two gas-solid chromatography experiments, which reported two different types of interaction, however, each based on the level of a few registered atoms only. Whereas noble-gas-like properties were suggested from the first experiment, the second one pointed at a volatile-metal-like character. Here, we present further experimental data on adsorption studies of Fl on silicon oxide and gold surfaces, accounting for the inhomogeneous nature of the surface, as it was used in the experiment and analyzed as part of the reported studies. We confirm that Fl is highly volatile and the least reactive member of group 14. Our experimental observations suggest that Fl exhibits lower reactivity towards Au than the volatile metal Hg, but higher reactivity than the noble gas Rn.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2022

Unveiling the two-proton halo character of 17 Ne: Exclusive measurement of quasi-free proton-knockout reactions

The proton drip-line nucleus 17 Ne is investigated experimentally in order to determine its two-proton halo character. A fully exclusive measurement of the 17 Ne (p, 2p) 16 F* 15 O+p quasi-free one-proton knockout reaction has been performed at GSI at around 500 MeV/nucleon beam energy. All particles resulting from the scattering process have been detected. The relevant reconstructed quantities are the angles of the two protons scattered in quasi-elastic kinematics, the decay of 16 F into 15 O (including γ decays from excited states) and a proton, as well as the 15 O+p relative-energy spectrum and the 16 F momentum distributions. The latter two quantities allow an independent and consistent determination of the fractions of l = 0 and l = 2 motion of the valence protons in 17 Ne. With a resulting relatively small l = 0 component of only around 35(3)%, it is concluded that 17 Ne exhibits a rather modest halo character only. The quantitative agreement of the two values deduced from the energy spectrum and the momentum distributions supports the theoretical treatment of the calculation of momentum distributions after quasi-free knockout reactions at high energies by taking into account distortions based on the Glauber theory. Moreover, the experimental data allow the separation of valence-proton knockout and knockout from the 15O core. The latter process contributes with 11.8(3.1) mb around 40% to the total proton-knockout cross section of 30.3(2.3) mb, which explains previously reported contradicting conclusions derived from inclusive cross sections.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Persistence of the Z = 28 shell gap in A = 75 isobars: Identification of a possible ( 1 / 2 – ) μ s isomer in Co 75 and β decay to Ni 75

Here, the evolution of shell structure around doubly magic exotic nuclei is of great interest in nuclear physics and astrophysics. In the ‘southwest’ region of 78 Ni, the development of deformation might trigger a major shift in our understanding of explosive nucleosynthesis. To this end, new spectroscopic information on key close-lying nuclei is very valuable. We intend to measure the isomeric and β decay of 75 Co, with one-proton and two-neutron holes relative to 78Ni, to access new nuclear structure information in 75 Co and its β-decay daughters 75 Ni and 74 Ni. The nucleus 75 Co is produced in relativistic in-flight fission reactions of 238 U at the Radioactive Ion Beam Factory in the RIKEN Nishina Center. Its isomeric and β decay are studied exploiting the BigRIPS and EURICA setups. We obtain partial β-decay spectra for 75 Ni and 74 Ni, and report a new isomeric transition in 75 Co. The energy [E γ = 1914(2)keV] and half-life [t 1/2 = 13(6) μs] of the delayed γ ray lend support for the existence of a J π = (1/2 – ) isomeric state at 1914(2) keV. A comparison with PFSDG-U shell-model calculations provides a good account for the observed states in 75 Ni, but the first calculated 1/2 – level in 75 Co, a prolate K = 1/2 state, is predicted about 1 MeV below the observed (1/2 – ) level. The spherical-like structure of the lowest-lying excited states in 75 Ni is proved. In the case of 75 Co, the results suggest that the dominance of the spherical configurations over the deformed ones might be stronger than expected below 78 Ni. Further experimental efforts to discern the nature of the J π = (1/2 – ) isomer are necessary.

59 ≤ A ≤ 89↗
DOE OSTI2020

Search for elements 119 and 120

In this work, a search for production of the superheavy elements with atomic numbers 119 and 120 was performed in the 50 Ti + 249 Bk and 50 Ti + 249 Cf fusion-evaporation reactions, respectively, at the gas-filled recoil separator TASCA at GSI Darmstadt, Germany. Over four months of irradiation, the 249 Bk target partially decayed into 249 Cf, which allowed for a simultaneous search for both elements. Neither was detected at cross-section sensitivity levels of 65 and 200 fb for the 50 Ti + 249 Bk and 50 Ti + 249 Cf reactions, respectively, at a midtarget beam energy of E lab = 281.5 MeV. The nonobservation of elements 119 and 120 is discussed within the concept of fusion-evaporation reactions including various theoretical predictions on the fission-barrier heights of superheavy nuclei in the region of the island of stability.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2020

Isomeric and beta-decay spectroscopy of 173,174 Ho

β-decay spectroscopy of 173,174 Ho (Z = 67, N = 106,107) was conducted at Radioactive Isotope Beam Factory at RIKEN by using in-flight fission of a 345-MeV/u 238 U primary beam. A previously unreported isomeric state at 405 keV with half-life of 3.7(12) μs and a spin and parity of (3/2 + ) is identified in 173 Ho. Moreover, a new state with a spin and parity of 9 - was discovered in 174 Er. The experimental log ft values of 5.84(20) and 5.25(18) suggest an allowed-hindered β decay from the ground state of 174 Ho to the K π = 8 - isomeric state in 174 Er. Configuration-constrained potential energy surface (PES) calculations were performed and the predictions are in reasonable agreement with the experimental results.

150 ≤ A ≤ 189↗