Comprehensive study of d + Li 6 via observing simultaneous outgoing neutrons, γ rays, and charged particles
Not Available
Paneru, S. N. (ORCID:000000017343158X)↗
Engineering topics
Kuvin, S. A.
Publications and source records attributed to Kuvin, S. A..
Innovative approaches to neutron beam optimization: A case study of FP14 at LANSCE
This paper describes an experimental method to acquire high resolution energy- and spatially- resolved neutron beam spots using the time-gated neutron imaging system with Teledyne Pi-MAX4 camera. These experimental data offer a unique opportunity for benchmarking beam spot simulations. High-quality simulations depend significantly on a high-fidelity geometry model, which can be challenging for legacy facilities. We informed our MCNPX geometry model by latest metrology survey employing Leica laser tracker ATS600. It gave us a high fidelity description of our facility geometry. Such a robust integration of novel tools and methods yields a previously unattainable level of accuracy in both predicting and capturing neutron beam spots, marking a notable advancement over traditional methods reliant on static image plates. Here, to demonstrate the practical application of these tools, we are showing a non-uniform beam spot challenge at our Flight Path 14 (FP14) at the Los Alamos Neutron Science Center (LANSCE). Our precise MCNPX prediction of beam spot shifting as function of neutron energy was confirmed by experimental beam spot measured with extremely high level of detail. Results of this research demonstrate a significant leap in neutron beam optimization at LANSCE and set a new benchmark in beam spot characterization. The advanced methods presented here have potential for adoption at similar research facilities worldwide, aiming at substantial improvement in neutron beam delivery for experiments.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Measurement of the 25 Al(𝑑,𝑛) 26 Si reaction and impact on the 25 Al(𝑝,𝛾) 26 Si reaction rate
The 25 Al(p,γ) 26 Si reaction plays a key role in nucleosynthesis pathways that influence the galactic abundance of 26 Al. A more precise determination of the proton strength of the lowest ℓ = 0 proton resonance in 26 Si is needed to improve reaction-rate calculations. This work measures the 25 Al(d,n) 26 Si proton-transfer reaction in inverse kinematics using a radioactive ion beam at RESOLUT, determining excitation energies and cross sections for the lowest ℓ = 0 resonance associated with the 3 + 3 state at 5.92(2) MeV. Coupled-reaction-channels calculations (FRESCO) are used to extract the ℓ = 0 spectroscopic factor and the corresponding proton width, yielding Γₚ = 2.19(45) eV and a (p,γ) resonance strength of 26(10) meV. This resonance is found to dominate the 25 Al(p,γ) 26 Si reaction rate above 0.2 GK.
20 ≤ A ≤ 38↗
Strong Evidence for N 9 and the Limits of Existence of Atomic Nuclei
The boundaries of the Chart of Nuclides contain exotic isotopes that possess extreme proton-to-neutron asymmetries. Here we report on strong evidence of 9 N, one of the most exotic proton-rich isotopes where more than one half of its constitute nucleons are unbound. With seven protons and two neutrons, this extremely proton-rich system would represent the first-known example of a ground-state five-proton emitter. Here, the invariant-mass spectrum of its decay products can be fit with two peaks whose energies are consistent with the theoretical predictions of an open-quantum-system approach, however we cannot rule out the possibility that only a single resonance-like peak is present in the spectrum.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
First direct measurement of the 13 $\mathrm{N(α, ρ)}$ 16 $\mathrm{O}$ reaction relevant for core-collapse supernovae nucleosynthesis
We report that understanding the explosion mechanism of a core-collapse supernova (CCSN) is important to accurately model CCSN scenarios for different progenitor stars using model-observation comparisons. The uncertainties of various nuclear reaction rates relevant for CCSN scenarios strongly affect the accuracy of these stellar models. Out of these reactions, the 13 N(α, p) 16 O reaction has been found to affect various stages of a CCSN at varying temperatures. This work presents the first direct measurement of the 13 N(α, p) 16 O reaction performed using a 34.6 MeV beam of radioactive 13 N ions and the active-target detector MUSIC (MUlti-Sampling Ionization Chamber) at Argonne National Laboratory. The resulting total 13 N(α, p) 16 O reaction cross sections from this measurement in the center-of-mass energy range of 3.26 - 6.02 MeV are presented and compared with calculations using the Hauser-Feshbach formalism. Uncertainties in the reaction rate have been dramatically reduced at CCSN temperatures.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Using spin alignment of inelastically excited nuclei in fast beams to assign spins: The spectroscopy of 13 O as a test case
Excited states in O 13 were investigated using inelastic scattering of an E / A = 69.5 MeV O 13 beam off of a Be 9 target. The excited states were identified in the invariant-mass spectra of the decay products. Both single-proton and sequential two-proton decays of the excited states were examined. Furthermore, for a number of the excited states, the protons were emitted with strong anisotropy where emissions transverse to the beam axis are favored. The measured proton-decay angular distributions were compared to predictions from distorted-wave Born-approximation calculations of the spin alignment which was shown to be largely independent of the excitation mechanism. The deduced O 13 level scheme is compared to ab initio no-core shell model with continuum predictions. The lowest-energy excited states decay isotropically consistent with predictions of strong proton 1 s 1 / 2 structure. Above these states in the level scheme, we observed a number of higher-spin states not predicted within the model. Possibly these are associated with rotational bands built on deformed cluster configurations predicted by antisymmetrized molecular dynamics calculations. The spin alignment mechanism is shown to be useful for making spin assignments and may have widespread use.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Indirect determination of the astrophysical S factor for the Li 6 ( p , γ ) Be 7 reaction using the asymptotic normalization coefficient method
The 6 Li(p,γ) 7 Be cross section influences a variety of astrophysical scenarios, including big-bang and stellar nucleosynthesis. In recent years, conflicting results of direct measurements have been published, reporting contradictory low-energy trends. To shed light on the contradiction between the existing data sets, the reaction was studied using the asymptotic normalization coefficient (ANC) technique which was up-to-now never used for this reaction. To derive the ANC, the 6 Li( 3 He,d) 7 Be transfer reaction, studied at the Department of Physics and Astronomy of the University of Catania and at the John. D. Fox Superconducting Accelerator Laboratory at Florida State University, was re-analyzed, focusing on the proton transfer mechanism [the α transfer process is discussed by Kiss et al. [Phys. Lett. B 807, 135606 (2020)]. Here, the energy of the 3 He beam impinging on a 6 Li target was E lab = 3 MeV and E lab = 5 MeV. The yield of the emitted deuterons was measured with high precision by using silicon ΔE – E telescopes.
6 ≤ A ≤ 19↗
Configuration mixing in 28 Mg and the 26 Mg (t,p) 28 Mg reaction
We have studied the 26 Mg(t,p) 28 Mg reaction. The nucleus 28 Mg lies between 24 Mg and 32 Mg, the latter of which is central to the “island of inversion” characterized by low-lying neutron fp-shell configurations. The present results show that the second-excited 0 + state in 28 Mg contains large fp-shell occupation for the neutrons. The experiment was performed in inverse kinematics using the HELIcal Orbit Spectrometer (HELIOS) at Argonne National Laboratory. Shell-model calculations using the SDPF-MU interaction yielded level energies and two-neutron transfer amplitudes that were used in one-step distorted-wave Furthermore, born approximation calculations to provide theoretical predictions of the proton angular distributions. In many, but not all cases, the data were in good agreement with theoretical predictions.
20 ≤ A ≤ 38↗
Observation of the Exotic Isotope 13 F Located Four Neutrons beyond the Proton Drip Line
A 13 F resonance was observed following a charge-exchange reaction between a fast 13 O beam and a 9 Be target. The resonance was found in the invariant-mass distribution of 3p+ 10 C events and probably corresponds to a 5/2 + excited state. The ground state was also expected to be populated, but was not resolved from the background. The observed level decays via initial proton emissions to both the ground and first 2 + state of 12 O, which subsequently undergo 2p decay. In addition there may also be a significant proton decay branch to the second 2+ level in 12 O. The wavefunction associated with the observed level may be collectivized due to coupling to the continuum as is it located just above the threshold for proton decay to the second $2^{+}_{2}$ state of 12 O.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Search for the 1/2 + intruder state in 35 P
The excitation energy of deformed intruder states (specifically the 2p2h bandhead) as a function of proton number Z along N = 20 is of interest both in terms of better understanding the evolution of nuclear structure between spherical Ca 40 and the Island of Inversion nuclei, and for benchmarking theoretical descriptions in this region. At the center of the N = 20 Island of Inversion, the n p n h (where n = 2 , 4 , 6 ) neutron excitations across a diminished N = 20 gap result in deformed and collective ground states, as observed in Mg 32 . In heavier isotones, n p n h excitations do not dominate in the ground states but are present in the relatively low-lying level schemes. With the aim of identifying the expected 2 p 2 h x s 1 / 2 + state in P 35 , the only N = 20 isotone for which the neutron 2p2h excitation bandhead has not yet been identified, the S 36 ( d , He 3 ) P 35 reaction has been revisited in inverse kinematics with the HELical Orbit Spectrometer (HELIOS) at the Argonne Tandem Linac Accelerator System (ATLAS). While a candidate state has not been located, an upper limit for the transfer reaction cross section to populate such a configuration within a 2.5 to 3.6 MeV energy range provides a stringent constraint on the wave function compositions in both S 36 and P 35 .
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Total kinetic energy release in the fast-neutron-induced fission of Np 237
The total kinetic energy (TKE) release in the fast neutron-induced fission of 237Np was measured for neutron energies from En = 2.6–100 MeV at the Los Alamos Neutron Science Center at the Weapons Neutron Research facility. The post-TKE release decreases nonlinearly with increasing incident neutron energy and can be represented as TKE(MeV) = (174.38 ± 0.72) – (5.11 ± 0.5821) log 10 E n for En > 1 MeV. Analysis of the fragment mass distributions indicates that the decrease in TKE with increasing E n is a consequence of the fading out of shell effects at high excitation energies (resulting in an increase of symmetric fission) and the decrease of the total kinetic energy associated with asymmetric fission with increasing E n .
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Total kinetic energy and mass yields from the fast neutron-induced fission of $^{239}\hbox {Pu}$
The total kinetic energy (TKE) release in fission is an important observable, constituting over 80% of the energy released in fission (E f ≈ 200MeV). While the TKE release in the 239 Pu(n,f) reaction was previously measured up to 50 MeV incident neutron energy (E n ), there were features in TKE release at the highest values of E n that were puzzling. There was a marked flattening of TKE release from E n = 30 to 50 MeV, in disagreement with the clearly decreasing TKE observed from E n = 0.5 to 30 MeV. To verify and clarify this trend, TKE measurements at higher values of E n were made. We present absolute measurements of TKE release in 239 Pu(n,f) from E n = 2.4 to 100 MeV. Here, we used silicon PIN detectors to measure the fragment energies and deduce mass-yield curves using the 2E-method. We also discuss fission asymmetry and the relationships between approx. fission fragment mass and distortion.
239Pu↗
Astrophysical S-factor for the 3 He(α,γ) 7 Be reaction via the asymptotic normalization coefficient (ANC) method
Not Available
97 MATHEMATICS AND COMPUTING↗
Invariant-mass spectrum of O 11
The invariant-mass distribution of O 11 fragments formed in two-neutron-knockout reactions with a O 13 projectile and Be 9 target has been also examined. Gating on events where the C 9 decay fragments produced following 2 p emission are recoiled transversely in the projectile's frame improves the overall invariant-mass resolution. The observed peak is now shown to have contributions from at least two O 11 levels, in contradiction with the suggestion of Fortune [ Phys. Rev. C 99 , 051302(R) (2019) ]. The data, yet, do not differentiate between the ground-state properties obtained by the Gamow coupled-channels calculation and the prompt 2 p -decay model of Fortune. The ground-state 2 p -decay energy is 4.25(6) MeV in a two-level fit to the data, but lower values are possible if more states contribute to the observed spectrum, as suggested in the previous analysis.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Experimental study of the low-lying negative-parity states in 11 Be using the 12 B( d , 3 He) 11 Be reaction
In this work, low-lying negative-parity states in 11 Be having dominant p-wave neutron configurations were studied using the 12 B(d, 3 He) 11 Be proton-removal reaction in inverse kinematics. The 1/2 $\overset{-}{1}$ state at 0.32 MeV, the 3/2 $\overset{-}{1}$ state at 2.56 MeV and one or both of the states including the 5/2 $\overset{-}{1}$ level at 3.89 MeV and the 3/2 $\overset{-}{2}$ level at 3.96 MeV were populated in the present reaction. Spectroscopic factors were determined from the differential cross sections using a distorted wave Born approximation method. The p-wave proton removal strengths were well described by the shell model calculations while the Nilsson model calculation underestimates the spectroscopic factors for the higher excited states. Results from both variational Monte Carlo and no-core shell model calculations were also compared with the experimental observations.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Particle decays of levels in N 11 , 12 and O 12 investigated with the invariant-mass method
Particle-decaying states of the light nuclei 11,12 N and 12 O were studied using the invariant-mass method. The decay energies and intrinsic widths of a number of states were measured, and the momentum correlations of three-body decaying states were considered. A second $2p$-decaying 2 + state of 12 O was observed for the first time, and a higher-energy 12 O state was observed in the 4$p$+2α decay channel. This 4$p$+2α channel also contains contributions from fissionlike decay paths, including 6 Beg.s.+6Be g.s. . Analogs to these states in 12 O were found in 12 N in the 2$p$+ 10 B and 2$p$+α+ 6 Li channels. The momentum correlations for the prompt 2$p$ decay of 12 O g.s. were found to be nearly identical to those of 16 Ne g.s. , and the correlations for the new 2 + state were found to be consistent with sequential decay through excited states in 11 N. The momentum correlations for the 2$^+_1$ state in 12 O provide a new value for the 11 N ground-state energy. Finally, the states in 12 N/ 12 O that belong to the A=12 isobaric sextet do not deviate from the quadratic isobaric multiplet mass equation form
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
First Observation of Unbound O 11 , the Mirror of the Halo Nucleus Li 11
The structure of the extremely proton-rich nucleus O 8 11 3 , the mirror of the two-neutron halo nucleus Li 3 11 8 , has been studied experimentally for the first time. Following two-neutron knockout reactions with a O 13 beam, the O 11 decay products were detected after two-proton emission and used to construct an invariant-mass spectrum. A broad peak of width ~ 3.4 MeV was determined. Within the Gamow coupled-channel approach, it was concluded that this peak is a multiplet with contributions from the four lowest O 11 resonant states: J π = 3 / 2 1 - , 3 / 2 2 - , 5 / 2 1 + , and 5 / 2 2 + . The widths and configurations of these states show strong, nonmonotonic dependencies on the depth of the p - C 9 potential. This unusual behavior is due to the presence of a broad threshold resonant state in N 10 , which is an analog of the virtual state in Li 10 in the presence of the Coulomb potential. After optimizing the model to the data, only a moderate isospin asymmetry between ground states of O 11 and Li 11 was discovered.
6 ≤ A ≤ 19↗
Proton decay of 108 I and its significance for the termination of the astrophysical rp -process
Employing the Argonne Fragment Mass Analyzer and the implantation-decay-decay correlation technique, a weak 0.50(21)% proton decay branch was identified in 108 I for the first time. Here the 108 I proton-decay width is consistent with a hindered l = 2 emission, suggesting a d 5/2 origin. Using the extracted 108 I proton-decay Q value of 597(13) keV, and the Q α values of the 108 I and 107 Te isotopes, a proton-decay Q value of 510(20) keV for 104 Sb was deduced. Similarly to the 112,113 Cs proton-emitter pair, the value is lower than that for the less-exotic neighbor 109 I, possibly due to enhanced proton-neutron interactions in N ≈ 2 nuclei. In contrast, the present is higher than that of 105 Sb, suggesting a weaker interaction energy.
104Sb↗