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Lein, Manfred

Publications and source records attributed to Lein, Manfred.

High-order harmonic generation in the presence of a resonance

We investigate high-order harmonic generation from laser-irradiated systems that support a shape resonance. From the numerical solution of the time-dependent Schroedinger equation, we calculate the harmonic spectra and the time-frequency analysis of the harmonic intensity and phase. The analysis reveals the separate contributions of the short and long trajectories as well as the resonance. A range of harmonics is strongly enhanced by the presence of the resonance irrespective of the pulse length. The signature of the resonance remains significant after coherent summation over intensities as a simple method to simulate macroscopic effects. The time-frequency analysis supports the recently proposed four-step mechanism of the enhanced harmonic generation process.

74 ATOMIC AND MOLECULAR PHYSICS↗

Interference in above-threshold-ionization electron distributions from molecules

We present quantum-mechanical studies on above-threshold ionization of molecular ions in two and three dimensions. The momentum distributions show signatures of interfering emissions from the molecular centers. These structures deviate from a simple double-slit model that ignores the electron-ion interaction, but they are reproduced by an eikonal model. Such distortions of the interference pattern are partly responsible for the absence of clear interference patterns in the angle-integrated electron energy spectra.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗