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Livingston, John M.

Publications and source records attributed to Livingston, John M..

31 records · Page 2

Clear-Sky Closure Studies of Lower Tropospheric Aerosol and Water Vapor During ACE-2 Using Airborne Sunphotometer, Airborne In-Situ, Space-Borne, and Ground-Based Measurements

We report on clear-sky column closure experiments (CLEARCOLUMN) performed in the Canary Islands during the second Aerosol Characterization Experiment (ACE-2) in June/July 1997. We present CLEARCOLUMN results obtained by combining airborne sunphotometer and in-situ (optical particle counter, nephelometer, and absorption photometer) measurements taken aboard the Pelican aircraft, space-borne NOAA/AVHRR data and ground-based lidar and sunphotometer measurements. During both days discussed here, vertical profiles flown in cloud-free air masses revealed 3 distinctly different layers: a marine boundary layer (MBL) with varying pollution levels, an elevated dust layer, and a very clean layer between the MBL and the dust layer. A key result of this study is the achievement of closure between extinction or layer aerosol optical depth (AOD) computed from continuous in-situ aerosol size-distributions and composition and those measured with the airborne sunphotometer. In the dust, the agreement in layer AOD (lambda = 380-1060 nm) is 3-8%. In the MBL there is a tendency for the in-situ results to be slightly lower than the sunphotometer measurements (10-17% at lambda = 525 nm), but these differences are within the combined error bars of the measurements and computations.

Schmid, Beat↗

Ground-Based Lidar Measurements of Aerosols During ACE-2: Instrument Description, Results, and Comparisons with Other Ground-Based and Airborne Measurements

A micro-pulse lidar system (MPL) was used to measure the vertical and horizontal distribution of aerosols during the Aerosol Characterization Experiment 2 (ACE-2) in June and July of 1997. The MPL measurements were made at the Izana observatory (IZO), a weather station located on a mountain ridge (28 deg 18 min N, 16 deg 30 min W, 2367 m asl) near the center of the island of Tenerife, Canary Islands. The MPL was used to acquire aerosol backscatter, extinction, and optical depth profiles for normal background periods and periods influenced by Saharan dust from North Africa. System tests and calibration procedures are discussed, and an analysis of aerosol optical profiles acquired during ACE-2 is presented. MPL data taken during normal IZO conditions (no dust) showed that upslope aerosols appeared during the day and dissipated at night and that the layers were mostly confined to altitudes a few hundred meters above IZO. MPL data taken during a Saharan dust episode on 17 July showed that peak aerosol extinction values were an order of magnitude greater than molecular scattering over IZO, and that the dust layers extended to 5 km asl. The value of the dust backscatter-extinction ratio was determined to be 0.027 +/- 0.007 sr(exp -1). Comparisons of the MPL data with data from other collocated instruments showed good agreement during the dust episode.

Welton, Ellsworth J.↗

Shipboard Sunphotometer Measurements of Aerosol Optical Depth Spectra and Columnar Water Vapor During ACE-2, and Comparison with Selected Land, Ship, Aircraft, and Satellite Measurements

Analyses of aerosol optical depth (AOD) and columnar water vapor (CWV) measurements acquired with NASA Ames Research Center's six-channel Airborne Tracking Sunphotometer (AATS-6) operated aboard the R/V (research vehicle) Professor Vodyanitskiy during the second Aerosol Characterization Experiment (ACE-2) are discussed. Data are compared with various in situ and remote measurements for selected cases. The focus is on 10 July, when the Pelican airplane flew within 70 km of the ship near the time of a NOAA (National Oceanographic and Atmospheric Administration)-14/AVHRR (Advanced Very High Resolution Radiometer) satellite overpass and AOD measurements with the 14-channel Ames Airborne Tracking Sunphotometer (AATS-14) above the marine boundary layer (MBL) permitted calculation of AOD within the MBL from the AATS-6 measurements. A detailed column closure test is performed for MBL AOD on 10 July by comparing the AATS-6 MBL AODs with corresponding values calculated by combining shipboard particle size distribution measurements with models of hygroscopic growth and radiosonde humidity profiles (plus assumptions on the vertical profile of the dry particle size distribution and composition). Large differences (30-80% in the mid-visible) between measured and reconstructed AODs are obtained, in large part because of the high sensitivity of the closure methodology to hygroscopic growth models, which vary considerably and have not been validated over the necessary range of particle size/composition distributions. The wavelength dependence of AATS-6 AODs is compared with the corresponding dependence of aerosol extinction calculated from shipboard measurements of aerosol size distribution and of total scattering measured by a shipboard integrating nephelometer for several days. Results are highly variable, illustrating further the great difficulty of deriving column values from point measurements. AATS-6 CWV values are shown to agree well with corresponding values derived from radiosonde measurements during eight soundings on seven days and also with values calculated from measurements taken on 10 July with the AATS-14 and the University of Washington Passive Humidigraph aboard the Pelican.

Livingston, John M.↗

Characterization of Atmospheric Aerosol Behavior and Climatic Effects by Analysis of SAGE 2 and Other Space, Air, and Ground Measurements

This report documents the research performed under NASA Ames Cooperative Agreement NCC 2-991, which covered the period 1 April 1997 through 31 March 1999. Previously, an interim technical report (Technical Report No. 1, 20 March 1998) summarized the work completed during the period 1 April 1997 through 31 March 1998. The objective of the proposed research was to advance our understanding of atmospheric aerosol behavior, aerosol-induced climatic effects, and the remote measurement and retrieval capabilities of spaceborne sensors such as SAGE II by combining and comparing data from these instruments and from airborne and ground-based instruments.

Livingston, John M.↗

LASE measurements of aerosols and water vapor during TARFOX

The TARFOX (Tropospheric Aerosol Radiative Forcing Observational Experiment) intensive field campaign was designed to reduce uncertainties in estimates of the effects of anthropogenic aerosols on climate by measuring direct radiative effects and the optical, physical, and chemical properties of aerosols [1]. TARFOX was conducted off the East Coast of the United States between July 10-31, 1996. Ground, aircraft, and satellite-based sensors measured the sensitivity of radiative fields at various atmospheric levels to aerosol optical properties (i.e., optical thickness, phase function, single-scattering albedo) and to the vertical profile of aerosols. The LASE (Lidar Atmospheric Sensing Experiment) instrument, which was flown on the NASA ER-2 aircraft, measured vertical profiles of total scattering ratio and water vapor during a series of 9 flights. These profiles were used in real-time to help direct the other aircraft to the appropriate altitudes for intensive sampling of aerosol layers. We have subsequently used the LASE aerosol data to derive aerosol backscattering and extinction profiles. Using these aerosol extinction profiles, we derived estimates of aerosol optical thickness (AOT) and compared these with measurements of AOT from both ground and airborne sun photometers and derived from the ATSR-2 (Along Track and Scanning Radiometer 2) sensor on ERS-2 (European Remote Sensing Satellite-2). We also used the water vapor mixing ratio profiles measured simultaneously by LASE to derive precipitable water vapor and compare these to ground based measurements.

Ferrare, Richard A.↗

Measurement and Analysis of Atmospheric Spectral Optical Depths with NASA Ames Airborne Sunphotometers During TARFOX and ACE-2

In accordance with the scope of work of this contract, the following tasks were undertaken and completed during the course of the contract: (1) Participation in the design and development of the 14-channel Ames Airborne Tracking Sunphotometer (AATS-14), including the development and implementation of Visual Basic software for real-time data processing and display and post-acquisition data reduction and analysis. (2) Operation of the six-channel Ames Airborne Tracking Sunphotometer (AATS-6) aboard the University of Washington C-131A during TARFOX and in-field analysis and presentation of data acquired with the AATS-6. (3) Post-mission analysis of data acquired during TARFOX with the AATS-6 and the AATS-14. (4) Pre-TARFOX calibration of the AATS-6 at Mauna Loa Observatory in May 1996, and post-TARFOX calibration of the AATS-6 and AATS- 14 at Zugspitze, Germany in October 1996, including analyses of all data sets. (5) Analysis of AATS-14 airborne calibration data acquired on 17 November 1996 during a late afternoon Pelican flight over the central California coast. (6) Operational training, instrument preparation, field coordination, and analysis of shipboard measurements of aerosol optical depth with the AATS-6 during ACE-2. (7) Coordination of data acquisition with the AATS-14 aboard the Pelican during ACE-2 and in-field preliminary data analysis and presentation. (8) Calibration of the AATS-6 and AATS-14 in April/May 1997 at Mauna Loa prior to ACE-2, and post-mission calibration of the AATS-6 at Mauna Loa in August 1997.

Livingston, John M.↗

Airborne lidar mapping of vertical ozone distributions in support of the 1990 Clean Air Act Amendments

The 1990 Clean Air Act Amendments mandated attainment of the ozone standard established by the U.S. Environmental Protection Agency. Improved photochemical models validated by experimental data are needed to develop strategies for reducing near surface ozone concentrations downwind of urban and industrial centers. For more than 10 years, lidar has been used on large aircraft to provide unique information on ozone distributions in the atmosphere. However, compact airborne lidar systems are needed for operation on small aircraft of the type typically used on regional air quality investigations to collect data with which to develop and validate air quality models. Data presented in this paper will consist of a comparison between airborne differential absorption lidar (DIAL) and airborne in-situ ozone measurements. Also discussed are future plans to improve the airborne ultraviolet-DIAL for ozone and other gas observations and addition of a Fourier Transform Infrared (FTIR) emission spectrometer to investigate the effects of other gas species on vertical ozone distribution.

Uthe, Edward E.↗

SAGE II aerosol validation - Selected altitude measurements, including particle micromeasurements

The validity of particulate extinction coefficients derived from limb path solar radiance measurements obtained during the Stratospheric Aerosol and Gas Experiment (SAGE) II is tested. The SAGE II measurements are compared with correlative aerosol measurements taken during January 1985, August 1985, and July 1986 with impactors, laser spectrometers, and filter samplers on a U-2 aircraft, an upward pointing lidar on a P-3 aircraft, and balloon-borne optical particle counters. The data for July 29, 1986 are discussed in detail. The aerosol measurements taken on this day at an altitude of 20.5 km produce particulate extinction values which validate the SAGE II values for similar wavelengths.

Oberbeck, Verne R.↗

Retrieval of aerosol size distribution moments from multiwavelength particulate extinction measurements

Two methods for inferring aerosol size distribution moments from multiwavelength particulate extinction measurements are studied. The methods are an eigenvalue technique that approximates an appropriate moment-weighting function by a linear combination of kernel functions and a conversion ratio approach that uses the ratio of the particulate extinction measurements at two wavelengths to choose a model moment-to-extinction conversion ratio. The techniques are applied to infer the third moment, or volume, of the aerosol size distribution from actual particulate extinction measurements taken as part of the Stratospheric Aerosol and Gas Experiment II during a correlative measurement experiment in Brazil in April 1985.

Livingston, John M.↗

Comparison of satellite-inferred (SAGE II) aerosol optical depths with corresponding airborne sunphotometer optical depths

Solar radiation measurements were made with an airborne multiwavelength autotracking sunphotometer detector off the northeastern coast of Brazil on April 6, 1985. These measurements are used to validate solar radiation measurements from the Stratospheric Aerosol and Gas Experiment (SAGE II). The SAGE II data below 17.5 km are dominated by attenuation due to thunderstorm-generated cirrus clouds. When integrated above 17.5 km, however, the aerosol extinction profiles from SAGE II yield aerosol optical depths that are consistent with the corresponding sunphotometer values above 10.1 km.

Livingston, John M.↗

Observations of aerosol optical depth during the First ISLSCP Field Experiment (FIFE)

Solar radiation measurements were made with a multiwavelength airborne tracking sunphotometer during the First International Satellite Land Surface Climatology Project Field Experiment (FIFE). Data from June 6, and October 11, 1987 are analyzed. Atmospheric optical properties were derived from the data, including total optical depth, aerosol optical depth, aerosol size distribution, aerosol phase function, and aerosol single scattering albedo. The aerosol optical depths for June 6 exhibited a spectral dependence that peaked at short wavelengths, whereas those for October 11 decreased monotonically with wavelength and closely followed an Angstrom wavelength dependence. Also, a unimodal aerosol size distribution was found for the June 6 data, while the October 11 data exhibited a power law size distribution. It is suggested that these differences indicate the need for simultaneous sunphotometer measurements and remotely sensed data.

Spanner, Michael A.↗

The relationship of satellite-inferred stratospheric aerosol extinction to the position of the 50-mb north polar jet stream

The relationship between stratospheric aerosols and the location of the north polar night stratospheric jet stream was investigated for selected periods of four successive winters (1979-1982), using measurements from SAM II (Stratospheric Aerosol Measurement II) and SAGE I (Stratospheric Aerosol and Gas Experiment I) satellite-borne sun photometers and corresponding meteorological observations. Each period investigated included a polar stratospheric warming during which major dynamic meteorological changes are known to have perturbed the structure of the polar vortex. The analysis of variations in aerosol extinction mixing ratio patterns among winters and during major stratospheric warming events within separate winters showed a well-defined positive gradient in extinction mixing ratio and temperature across the jet stream from the cyclonic side to the anticyclonic side at altitudes between 20 and 30 km during each winter period. Estimates of extinction mixing ratio profiles measured near the center of the polar vortex suggest that a gradual subsidence took place within the polar vortex during at least three of the four winter periods.

Livingston, John M.↗