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Luo, Mingzhao

Publications and source records attributed to Luo, Mingzhao.

Quantifying Spatial and Seasonal Variability in Atmospheric Ammonia with In Situ and Space-Based Observations

Ammonia plays an important role in many biogeochemical processes, yet atmospheric mixing ratios are not well known. Recently, methods have been developed for retrieving NH3 from space-based observations, but they have not been compared to in situ measurements. We have conducted a field campaign combining co-located surface measurements and satellite special observations from the Tropospheric Emission Spectrometer (TES). Our study includes 25 surface monitoring sites spanning 350 km across eastern North Carolina, a region with large seasonal and spatial variability in NH3. From the TES spectra, we retrieve a NH3 representative volume mixing ratio (RVMR), and we restrict our analysis to times when the region of the atmosphere observed by TES is representative of the surface measurement. We find that the TES NH3 RVMR qualitatively captures the seasonal and spatial variability found in eastern North Carolina. Both surface measurements and TES NH3 show a strong correspondence with the number of livestock facilities within 10 km of the observation. Furthermore, we find that TES H3 RVMR captures the month-to-month variability present in the surface observations. The high correspondence with in situ measurements and vast spatial coverage make TES NH3 RVMR a valuable tool for understanding regional and global NH3 fluxes.

Pinder, Robert W.

First Satellite Observations of Lower Tropospheric Ammonia and Methanol

The Tropospheric Emission Spectrometer (TES) on the EOS Aura satellite makes global measurements of infrared radiances which are used to derive profiles of species such as O3, CO, H2O, HDO and CH4 as routine standard products. In addition, TES has a variety of special modes that provide denser spatial mapping over a limited geographical area. A continuous-coverage mode (called ''transect'', about 460 km long) has now been used to detect additional molecules indicative of regional air pollution. On 10 July 2007 at about 05:37 UTC (13:24 LMST) TES conducted such a transect observation over the Beijing area in northeast China. Examination of the residual spectral radiances following the retrieval of the TES standard products revealed surprisingly strong features attributable to enhanced concentrations of ammonia (NH3) and methanol (CH3OH), well above the normal background levels. This is the first time that these molecules have been detected in space-based nadir viewing measurements that penetrate into the lower atmosphere.

methanol

TES Level 1 Algorithms: Interferogram Processing, Geolocation, Radiometric, and Spectral Calibration

The Tropospheric Emission Spectrometer (TES) on the Earth Observing System (EOS) Aura satellite measures the infrared radiance emitted by the Earth's surface and atmosphere using Fourier transform spectrometry. The measured interferograms are converted into geolocated, calibrated radiance spectra by the L1 (Level 1) processing, and are the inputs to L2 (Level 2) retrievals of atmospheric parameters, such as vertical profiles of trace gas abundance. We describe the algorithmic components of TES Level 1 processing, giving examples of the intermediate results and diagnostics that are necessary for creating TES L1 products. An assessment of noise-equivalent spectral radiance levels and current systematic errors is provided. As an initial validation of our spectral radiances, TES data are compared to the Atmospheric Infrared Sounder (AIRS) (on EOS Aqua), after accounting for spectral resolution differences by applying the AIRS spectral response function to the TES spectra. For the TES L1 nadir data products currently available, the agreement with AIRS is 1 K or better.

infrared remote sensing

An analysis of the Antarctic Halogen Occultation Experiment trace gas observations

Analysis of the version 16 Halogen Occultation Experiment (HALOE) CH4 data shows that this long-lived trace gas is well correlated with potential vorticity (PV) computed from National Meteorological Center balanced winds. Analyzing late September and October 1992 data, we show that very low CH4 values are confined to the interior of a vortex edge defined by the maximum gradient in PV. The CH4 and HF time tendency is used to estimate the descent rate in the Antarctic vortex. After removing a component of the trend correlated with the HALOE sampling pattern, we compute the lower stratosphere vertical descent rates and net heaing rates in the spring Antarctic vortex. Our computations of the spring Antarctic vortex heating rates give -0.5 to -0.1 K/day. Over the winter season, the overall lower stratospheric descent rate averages about 1.8-1.5 km/month. These computations are in line with radiative transfer estimates of the heating and descent rate. The HALOE data thus appear to be consistent with the picture of an isolated lower stratospheric Antarctic vortex.

Schoeberl, Mark R.

Using the application visualization system to view HALOE three-dimensional satellite data

The Application Visualization System (AVS) is used to view a three-dimensional data field containing the volume mixing ratios of a chemical species in the middle atmosphere obtained by the Halogen Occultation Experiment (HALOE) aboard the Upper Atmosphere Research Satellite (UARS). Since launch in September 1991, HALOE has been collecting data on approximately 30 sunrise/sunset events in two narrow latitude bands each day. The vertical volume mixing ratio profiles are retrieved for eight species for each event. The accumulated data for approximately 30 days cover most of the globe (limited by sunlit latitudes), and this monthly data block can be described as the volume mixing ratio of a specific species in the atmosphere as a function of latitude, longitude, and height. The data were remapped using linear interpolation for pressure levels and Gaussian weighted binning from sampling locations to a three-dimensional grid. An AVS network is constructed that allows for viewing the three-dimensional field with rendered slices at constant latitudes, longitudes or pressure levels. Discussions are given on the advantages and some disadvantages learned about from experiences applying AVS to visualize HALOE three dimensional data.

Luo, Mingzhao

Analysis of selected nitric oxide observations in the lower thermosphere by HALOE on UARS

Measurements of nitric oxide mixing ratios have been made by the Halogen Occultation Experiment on the Upper Atmosphere Research Satellite over an altitude range extending from 15 to 130 km on every spacecraft sunrise and sunset event with the exception of about 8 percent downtime. Selected NO profiles from the first few months of observations were examined with emphasis on the relation between geomagnetic disturbances and enhanced NO in the lower thermosphere. During a large geomagnetic storm on November 8-9, 1991, HALOE obtained 15 NO sunrise profiles along about the 50 deg N latitude circle. A factor of three increase in NO mixing ratio above about 115 km at this latitude and a one to two day decay time were observed. The measured NO longitude/altitude cross section on this day shows a longitudinal asymmetry in the NO distribution with a maximum near the geomagnetic pole. From approximately one month's data, a latitude/altitude cross section of zonal mean NO mixing ratio was calculated. An example of such cross sections demonstrates a strong positive correlation between geomagnetic activity and thermospheric NO globally. This auroral forcing has a larger effect on increasing NO at high latitude than at low latitude.

Luo, Mingzhao

Image plane detector spectrophotometer - Application to O2 atmospheric band nightglow

A new variety of low resolution spectrometer is described. This device, an image plane detector spectrophotometer, has high sensitivity and modest resolution sufficient to determine the rotational temperature and brightness of molecular band emissions. It uses an interference filter as a dispersive element and a multichannel image plane detector as the photon collecting device. The data analysis technqiue used to recover the temperature of the emitter and the emission brightness is presented. The atmospheric band of molecular oxygen is used to illustrate the use of the device.

Luo, Mingzhao