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McGee, T. J.

Publications and source records attributed to McGee, T. J..

A New Differential Absorption Lidar to Measure Sub-Hourly Fluctuation of Tropospheric Ozone Profiles in the Baltimore - Washington D.C. Region

Tropospheric ozone profiles have been retrieved from the new ground based National Aeronautics and Space Administration (NASA) Goddard Space Flight Center TROPospheric OZone DIfferential Absorption Lidar (GSFC TROPOZ DIAL) in Greenbelt, MD (38.99 N, 76.84 W, 57 meters ASL) from 400 m to 12 km AGL. Current atmospheric satellite instruments cannot peer through the optically thick stratospheric ozone layer to remotely sense boundary layer tropospheric ozone. In order to monitor this lower ozone more effectively, the Tropospheric Ozone Lidar Network (TOLNet) has been developed, which currently consists of five stations across the US. The GSFC TROPOZ DIAL is based on the Differential Absorption Lidar (DIAL) technique, which currently detects two wavelengths, 289 and 299 nm. Ozone is absorbed more strongly at 289 nm than at 299 nm. The DIAL technique exploits this difference between the returned backscatter signals to obtain the ozone number density as a function of altitude. The transmitted wavelengths are generated by focusing the output of a quadrupled Nd:YAG laser beam (266 nm) into a pair of Raman cells, filled with high pressure hydrogen and deuterium. Stimulated Raman Scattering (SRS) within the focus generates a significant fraction of the pump energy at the first Stokes shift. With the knowledge of the ozone absorption coefficient at these two wavelengths, the range resolved number density can be derived. An interesting atmospheric case study involving the Stratospheric-Tropospheric Exchange (STE) of ozone is shown to emphasize the regional importance of this instrument as well as assessing the validation and calibration of data. The retrieval yields an uncertainty of 16-19 percent from 0-1.5 km, 10-18 percent from 1.5-3 km, and 11-25 percent from 3 km to 12 km. There are currently surface ozone measurements hourly and ozonesonde launches occasionally, but this system will be the first to make routine tropospheric ozone profile measurements in the Baltimore-Washington DC area.

Stimulated Raman Scattering↗

STROZ Lidar Results at the MOHAVE III Campaign, October, 2009, Table Mountain, CA

During October, 2009 the GSFC STROZ Lidar participated in a campaign at the JPL Table Mountain Facility (Wrightwood, CA, 2285 m Elevation) to measure vertical profiles of water vapor from near the ground to the lower stratosphere. On eleven nights, water vapor, aerosol, temperature and ozone profiles were measured by the STROZ lidar, two other similar lidars, frost-point hygrometer sondes, and ground-based microwave instruments made measurements. Results from these measurements and an evaluation of the performance of the STROZ lidar during the campaign will be presented in this paper. The STROZ lidar was able to measure water vapor up to 13-14 km ASL during the campaign. We will present results from all the STROZ data products and comparisons with other instruments made. Implications for instrumental changes will be discussed.

McGee, T. J.↗

Optical-Microphysical Cirrus Model

A model is presented that permits the simulation of the optical properties of cirrus clouds as measured with depolarization Raman lidars. It comprises a one-dimensional cirrus model with explicit microphysics and an optical module that transforms the microphysical model output to cloud and particle optical properties. The optical model takes into account scattering by randomly oriented or horizontally aligned planar and columnar monocrystals and polycrystals. Key cloud properties such as the fraction of plate-like particles and the number of basic crystals per polycrystal are parameterized in terms of the ambient temperature, the nucleation temperature, or the mass of the particles. The optical-microphysical model is used to simulate the lidar measurement of a synoptically forced cirrostratus in a first case study. It turns out that a cirrus cloud consisting of only monocrystals in random orientation is too simple a model scenario to explain the observations. However, good agreement between simulation and observation is reached when the formation of polycrystals or the horizontal alignment of monocrystals is permitted. Moreover, the model results show that plate fraction and morphological complexity are best parameterized in terms of particle mass, or ambient temperature which indicates that the ambient conditions affect cirrus optical properties more than those during particle formation. Furthermore, the modeled profiles of particle shape and size are in excellent agreement with in situ and laboratory studies, i.e., (partly oriented) polycrystalline particles with mainly planar basic crystals in the cloud bottom layer, and monocrystals above, with the fraction of columns increasing and the shape and size of the particles changing from large thin plates and long columns to small, more isometric crystals from cloud center to top. The findings of this case study corroborate the microphysical interpretation of cirrus measurements with lidar as suggested previously.

Reichardt, J.↗

Chemical Observations of a Polar Vortex Intrusion

An intrusion of vortex edge air in D the interior of the Arctic polar vortex was observed on the January 31,2005 flight of the NASA DC-8 aircraft. This intrusion was identified as anomalously high values of ozone by the AROTAL and DIAL lidars. Our analysis shows that this intrusion formed when a blocking feature near Iceland collapsed, allowing edge air to sweep into the vortex interior. along the DC-8 flight track also shows the intrusion in both ozone and HNO3. Polar Stratospheric Clouds (PSCs) were observed by the DIAL lidar on the DC-8. The spatial variability of the PSCs can be explained using MLS HNO3 and H2O observations and meteorological analysis temperatures. We also estimate vortex denitrification using the relationship between N2O and HNO3. Reverse domain fill back trajectory calculations are used to focus on the features in the MLS data. The trajectory results improve the agreement between lidar measured ozone and MLS ozone and also improve the agreement between the HNO3 measurements PSC locations. The back trajectory calculations allow us to compute the local denitrification rate and reduction of HCl within the filament. We estimate a denitrification rate of about lO%/day after exposure to below PSC formation temperature. Analysis of Aura MLS observations made

Schoeberl, M. R.↗

Lidar system for investigation of aerosols and cirrus clouds near the equator

In the current environment of concern over global warming, climate change, and ozone depletion/recovery, measurements in the tropics, within 5 degrees of the equator are limited and/or sporadic. Clearly, routine observations in this region would be of great benefit to many programs including those dealing with atmospheric chemistry, dynamics and radiation, and validation of satellite instruments. Such observations represent the primary goals of the Network for the Detection of Stratospheric Change (NDSC).

atmosphere↗

Correlations among the Optical Properties of Cirrus-Cloud Particles: Microphysical Interpretation

Cirrus measurements obtained with a ground-based polarization Raman lidar at 67.9 deg N in January 1997 reveal a strong positive correlation between the particle optical properties, specifically depolarization ratio delta(sub par) and extinction- to-backscatter (lidar) ratio S, for delta(sub par) less than approximately 40%, and an anti-correlation for delta(sub par) greater than approximately 40%. Over the length of the measurements the particle properties vary systematically. Initially, delta (sub par) approximately equals 60% and S approximately equals 10sr are observed. Then, with decreasing delta(sub par), S first increases to approximately 27sr (delta(sub par) approximately equals 40%) before decreasing to values around 10sr again (delta(sub par) approximately equals 20%). The analysis of lidar humidity and radiosonde temperature data shows that the measured optical properties stem from scattering by dry solid ice particles, while scattering by supercooled droplets, or by wetted or subliming ice particles can be excluded. For the microphysical interpretation of the lidar measurements, ray-tracing computations of particle scattering properties have been used. The comparison with the theoretical data suggests that the observed cirrus data can be interpreted in terms of size, shape, and, under the assumption that the lidar measurements of consecutive cloud segments can be mapped on the temporal development of a single cloud parcel moving along its trajectory, growth of the cirrus particles: Near the cloud top in the early stage of cirrus development, light scattering by nearly isometric particles that have the optical characteristics of hexagonal columns (short, column-like particles) is dominant. Over time the ice particles grow, and as the cloud base height extends to lower altitudes characterized by warmer temperatures they become morphologically diverse. For large S and depolarization values of approximately 40%, the scattering contributions of column- and plate-like particles are roughly the same. In the lower ranges of the cirrus clouds, light scattering is predominantly by plate-like ice particles. This interpretation assumes random orientation of the cirrus particles. Simulations with a simple model suggest, however, that the positive correlation between S and delta(sub par) which is observed for depolarization ratios less than 40% mainly at low cloud altitudes, can be alternatively explained by horizontal alignment of a fraction of the cirrus particle population.

Reichardt, J.↗

Retrieval of Polar Stratospheric Cloud Microphysical Properties from Lidar Measurements: Dependence on Particle Shape Assumptions

A retrieval algorithm has been developed for the microphysical analysis of polar stratospheric cloud (PSC) optical data obtained using lidar instrumentation. The parameterization scheme of the PSC microphysical properties allows for coexistence of up to three different particle types with size-dependent shapes. The finite difference time domain (FDTD) method has been used to calculate optical properties of particles with maximum dimensions equal to or less than 2 mu m and with shapes that can be considered more representative of PSCs on the scale of individual crystals than the commonly assumed spheroids. Specifically. these are irregular and hexagonal crystals. Selection of the optical parameters that are input to the inversion algorithm is based on a potential data set such as that gathered by two of the lidars on board the NASA DC-8 during the Stratospheric Aerosol and Gas Experiment 0 p (SAGE) Ozone Loss Validation experiment (SOLVE) campaign in winter 1999/2000: the Airborne Raman Ozone and Temperature Lidar (AROTEL) and the NASA Langley Differential Absorption Lidar (DIAL). The 0 microphysical retrieval algorithm has been applied to study how particle shape assumptions affect the inversion of lidar data measured in leewave PSCs. The model simulations show that under the assumption of spheroidal particle shapes, PSC surface and volume density are systematically smaller than the FDTD-based values by, respectively, approximately 10-30% and approximately 5-23%.

Reichardt, J.↗

Correlation Between Cirrus Particle Optical Properties: Microphysics and Implications for Spaceborne Remote Sensing

Cirrus measurements obtained with a ground-based polarization Raman lidar at 67.9 deg N in arctic winter reveal a strong correlation between the particle optical properties, specifically depolarization ratio and extinction-to-backscatter ratio, for ambient cloud temperatures above approximately -45 C, and an anti-correlation for colder temperatures. Similar correlations are evident in a 2-year midlatitude (53.4 deg N) cirrus data set. Scattering calculations show that the observed dependences can be interpreted in terms of the shapes and sizes of the cirrus ice particles. These findings suggest a retrieval method for determining cirrus extinction profiles from spaceborne lidar polarization data.

Reichardt, Jens↗

Lidar temperature measurements at NY-Alesund (79N) during winter, 1998

During January and February, 1998, a measurements campaign was held at the Network for the Detection of Stratospheric Change (NDSC) Arctic site at Ny-Alesund (78.9N). Lidar measurements of ozone, temperature and aerosol parameters were made along with balloon sonde and microwave measurements of ozone. Atmospheric temperatures were measured between 10 and 70 km. During the time of the campaign an strong warming occurred at the stratopause, elevating the measured temperature by as much as 80 K. The height of the stratopause descended at this time to below 40 km.

McGee, T. J.↗

First results from the aerosol lidar and backscatter sonde intercomparison campaign STRAIT'1997 at table mountain facility during February-March 1997

First results of an intercomparison measurement campaign between three aerosol lidar instruments and in-situ backscatter sondes performed at Table Mountain Facility (34.4 deg N, 117.7 deg E, 2280 m asl) in February-March 1997 are presented. During the campaign a total of 414 hours of lidar data were acquired by the Aerosol-Temperature-Lidar (ATL, Goddard Space Flight Center) the Mobile-aerosol-Raman-Lidar (MARL, Alfred Wegener Institute), and the TMF-Aerosol-Lidar (TAL, Jet Propulsion Laboratory), and four backscatter sondes were launched. From the data set altitude profiles of backscatter ratio and volume depolarization of stratospheric background aerosols at altitudes between 15 and 25 km and optically thin high-altitude cirrus clouds at altitudes below 13 km are derived. On the basis of a sulfuric acid aerosol model color ratio profiles obtained from two wavelength lidar data are compared to the corresponding profiles derived from the sonde observations. We find an excellent agreement between the in-situ and ATL lidar data with respect to backscatter and color ratio. Cirrus clouds were present on 16 of 26 nights during the campaign. Lidar observations with 17 minute temporal and 120-300 m spatial resolution indicate high spatial and temporal variability of the cirrus layers. Qualitative agreement is found between concurrent lidar measurements of backscatter ratio and volume depolarization.

Beyerle, G.↗

Validation of UARS Microwave Limb Sounder Temperature and Pressure Measurements

The accuracy and precision of the Upper Atmosphere Research Satellite (UARS) Microwave Limb Sounder (MLS) atmospheric temperature and tangent-point pressure measurements are described. Temperatures and tangent- point pressure (atmospheric pressure at the tangent height of the field of view boresight) are retrieved from a 15-channel 63-GHz radiometer measuring O2 microwave emissions from the stratosphere and mesosphere. The Version 3 data (first public release) contains scientifically useful temperatures from 22 to 0.46 hPa. Accuracy estimates are based on instrument performance, spectroscopic uncertainty and retrieval numerics, and range from 2.1 K at 22 hPa to 4.8 K at 0.46 hPa for temperature and from 200 m (equivalent log pressure) at 10 hPa to 300 m at 0.1 hPa. Temperature accuracy is limited mainly by uncertainty in instrument characterization, and tangent-point pressure accuracy is limited mainly by the accuracy of spectroscopic parameters. Precisions are around 1 K and 100 m. Comparisons are presented among temperatures from MLS, the National Meteorological Center (NMC) stratospheric analysis and lidar stations at Table Mountain, California, Observatory of Haute Provence (OHP), France, and Goddard Spaceflight Center, Maryland. MLS temperatures tend to be 1-2 K lower than NMC and lidar, but MLS is often 5 - 10 K lower than NMC in the winter at high latitudes, especially within the northern hemisphere vortex. Winter MLS and OHP (44 deg N) lidar temperatures generally agree and tend to be lower than NMC. Problems with Version 3 MLS temperatures and tangent-point pressures are identified, but the high precision of MLS radiances will allow improvements with better algorithms planned for the future.

Fishbein, E. F.↗

Validation of UARS Microwave Limb Sounder Temperature and Pressure Measurements

The accuracy and precision of the Upper Atmosphere Research Satellite (UARS) Microwave Limb Sounder (MLS) atmospheric temperature and tangent-point pressure measurements are described. Temperatures and tangent-point pressure are retrieved from a 15-channel 63-GHz radiometer measuring O 2 microwave emissions from the stratosphere and mesosphere.

atmospheric↗

Stratospheric Ozone Intercomparison Campaign (STOIC) 1989: Overview

The NASA Upper Atmosphere Research Program organized a Stratospheric Ozone Intercomparison Campaign (STOIC) held in July-August 1989 at the Table Mountain Facility (TMF) of the Jet Propulsion Laboratory (JPL). The primary instruments participating in this campaign were several that had been developed by NASA for the Network for the Detection of Stratospheric Change: the JPL ozone lidar at TMF, the Goddard Space Flight Center trailer-mounted ozone lidar which was moved to TMF for this comparison, and the Millitech/LaRC microwave radiometer. To assess the performance of these new instruments, a validation/intercomparison campaign was undertaken using established techniques: balloon ozonesondes launched by personnel from the Wallops Flight Facility and from NOAA Geophysical Monitoring for Climate Change (GMCC) (now Climate Monitoring and Diagnostics Laboratory), a NOAA GMCC Dobson spectrophotometer, and a Brewer spectrometer from the Atmospheric Environment Service of Canada, both being used for column as well as Umkehr profile retrievals. All of these instruments were located at TMF and measurements were made as close together in time as possible to minimize atmospheric variability as a factor in the comparisons. Daytime rocket measurements of ozone were made by Wallops Flight Facility personnel using ROCOZ-A instruments launched from San Nicholas Island. The entire campaign was conducted as a blind intercomparison, with the investigators not seeing each others data until all data had been submitted to a referee and archived at the end of the 2-week period (July 20 to August 2, 1989). Satellite data were also obtained from the Stratospheric Aerosol and Gas Experiment (SAGE 2) aboard the Earth Radiation Budget Satellite and the Total Ozone Mapping Spectrometer (TOMS) aboard Nimbus 7. An examination of the data has found excellent agreement among the techniques, especially in the 20- to 40-km range. As expected, there was little atmospheric variability during the intercomparison, allowing for detailed statistical comparisons at a high level of precision. This overview paper summarizes the campaign and provides a 'road map' to subsequent papers in this issue by the individual instrument teams which will present more detailed analysis of the data and conclusions.

Margitan, J. J.↗