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McGee, Thomas

Publications and source records attributed to McGee, Thomas.

Importance of a Priori Vertical Ozone Profiles for TEMPO Air Quality Retrievals

Ozone (O3) is a toxic pollutant which plays a major role in air quality. Typically, monitoring of surface air quality and O3 mixing ratios is conducted using in situ measurement networks. This is partially due to high-quality information related to air quality being limited from space-borne platforms due to coarse spatial resolution, limited temporal frequency, and minimal sensitivity to lower tropospheric and surface-level O3. The Tropospheric Emissions: Monitoring of Pollution (TEMPO) satellite is designed to address the limitations of current space-based platforms and to improve our ability to monitor North American air quality. TEMPO will provide hourly data of total column and vertical profiles of O3 with high spatial resolution to be used as a near-real-time air quality product. TEMPO O3 retrievals will apply the Smithsonian Astrophysical Observatory profile algorithm developed based on work from GOME (Global Ozone Monitoring Experiment), GOME-2, and OMI (Ozone Monitoring Instrument). This algorithm is suggested to use a priori O3 profile information from a climatological data-base developed from long-term ozone-sonde measurements (tropopause-based (TB-Clim) O3 climatology). This study evaluates the TB-Clim dataset and model simulated O3 profiles, which could potentially serve as a priori O3 profile information in TEMPO retrievals, from near-real-time data assimilation model products (NASA GMAO's (Global Modeling and Assimilation Office) operational GEOS-5 (Goddard Earth Observing System, Version 5) FP (Forecast Products) model and reanalysis data from MERRA2 (Modern-Era Retrospective analysis for Research and Applications, Version 2)) and a full chemical transport model (CTM), GEOS-Chem. In this study, vertical profile products are evaluated with surface (0-2 kilometers) and tropospheric (0-10 kilometers) TOLNet (Tropospheric Ozone Lidar Network) observations and the theoretical impact of individual a priori profile sources on the accuracy of TEMPO O3 retrievals in the troposphere and at the surface are presented. Results indicate that while the TB-Clim climatological dataset can replicate seasonally-averaged tropospheric O3 profiles, model-simulated profiles from a full CTM resulted in more accurate tropospheric and surface-level O3 retrievals from TEMPO when compared to hourly and daily-averaged TOLNet observations. Furthermore, it is shown that when large surface O3 mixing ratios are observed, TEMPO retrieval values at the surface are most accurate when applying CTM a priori profile information compared to all other data products.

Priori↗

Evaluating a Priori Ozone Profile Information Used in TEMPO Tropospheric Ozone Retrievals

Ozone (O3) is a greenhouse gas and toxic pollutant which plays a major role in air quality. Typically, monitoring of surface air quality and O3 mixing ratios is primarily conducted using in situ measurement networks. This is partially due to high-quality information related to air quality being limited from space-borne platforms due to coarse spatial resolution, limited temporal frequency, and minimal sensitivity to lower tropospheric and surface-level O3. The Tropospheric Emissions: Monitoring of Pollution (TEMPO) satellite is designed to address these limitations of current space-based platforms and to improve our ability to monitor North American air quality. TEMPO will provide hourly data of total column and vertical profiles of O3 with high spatial resolution to be used as a near-real-time air quality product.TEMPO O3 retrievals will apply the Smithsonian Astrophysical Observatory profile algorithm developed based on work from GOME, GOME-2, and OMI. This algorithm uses a priori O3 profile information from a climatological data-base developed from long-term ozone-sonde measurements (tropopause-based (TB) O3 climatology). It has been shown that satellite O3 retrievals are sensitive to a priori O3 profiles and covariance matrices. During this work we investigate the climatological data to be used in TEMPO algorithms (TB O3) and simulated data from the NASA GMAO Goddard Earth Observing System (GEOS-5) Forward Processing (FP) near-real-time (NRT) model products. These two data products will be evaluated with ground-based lidar data from the Tropospheric Ozone Lidar Network (TOLNet) at various locations of the US. This study evaluates the TB climatology, GEOS-5 climatology, and 3-hourly GEOS-5 data compared to lower tropospheric observations to demonstrate the accuracy of a priori information to potentially be used in TEMPO O3 algorithms. Here we present our initial analysis and the theoretical impact on TEMPO retrievals in the lower troposphere.

TEMPO↗

Development of the Global Ozone Lidar Demonstrator (GOLD) Instrument for Deployment on the NASA Global Hawk

A compact ozone (O3) and aerosol lidar system is being developed for conducting global atmospheric investigations from the NASA Global Hawk Uninhabited Aerial Vehicle (UAV) and for enabling the development and test of a space-based O3 and aerosol lidar. GOLD incorporates advanced technologies and designs to produce a compact, autonomously operating O3 and aerosol Differential Absorption Lidar (DIAL) system for a UAV platform. The GOLD system leverages advanced Nd:YAG and optical parametric oscillator laser technologies and receiver optics, detectors, and electronics. Significant progress has been made toward the development of the GOLD system, and this paper describes the objectives of this program, basic design of the GOLD system, and results from initial ground-based atmospheric tests.

Hair, Jonathan W.↗

Lidar Temperature Measurements During the SOLVE Campaign and the Absence of PSCs from Regions of Very Cold Air

NASA Goddard Space Flight Center's Airborne Raman Ozone, Temperature and Aerosol Lidar (AROTEL) measured extremely cold temperatures during all three deployments (December 1-16, 1999, January 14-29, 2000 and February 27-March 15, 2000) of the Sage III Ozone Loss and Validation Experiment (SOLVE). Temperatures were significantly below values observed in previous years with large regions regularly below 191 K and frequent temperature retrievals yielding values at or below 187 K. Temperatures well below the saturation point of type I polar stratospheric clouds (PSCs) were regularly encountered but their presence was not well correlated with PSCs observed by the NASA Langley Research Center's Aerosol Lidar co-located with AROTEL. Temperature measurements by meteorological sondes launched within areas traversed by the DC-8 showed minimum temperatures consistent in time and vertical extent with those derived from AROTEL data. Calculations to establish whether PSCs could exist at measured AROTEL temperatures and observed mixing ratios of nitric acid and water vapor showed large regions favorable to PSC formation. On several occasions measured AROTEL temperatures up to 10 K below the NAT saturation temperature were insufficient to produce PSCs even though measured values of nitric acid and water were sufficient for their formation.

Burris, John↗

Validation of Temperature Measurements from the Airborne Raman Ozone Temperature and Aerosol Lidar During SOLVE

The Airborne Raman Ozone, Temperature and Aerosol Lidar (AROTEL) participated in the recent Sage III Ozone Loss and Validation Experiment (SOLVE) by providing profiles of aerosols, polar stratospheric clouds (PSCs), ozone and temperature with high vertical and horizontal resolution. Temperatures were derived from just above the aircraft to approximately 60 kilometers geometric altitude with a reported vertical resolution of between 0.5 and 1.5 km. The horizontal footprint varied from 4 to 70 km. This paper explores the measurement uncertainties associated with the temperature retrievals and makes comparisons with independent, coincident, measurements of temperature. Measurement uncertainties range from 0.1 K to approximately 4 K depending on altitude and integration time. Comparisons between AROTEL and balloon sonde temperatures retrieved under clear sky conditions using both Rayleigh and Raman scattered data showed AROTEL approximately 1 K colder than sonde values. Comparisons between AROTEL and the Meteorological Measurement System (MMS) on NASA's ER-2 show AROTEL being from 2-3 K colder for altitudes ranging from 14 to 18 km. Temperature comparisons between AROTEL and the United Kingdom Meteorological Office's model showed differences of approximately 1 K below approximately 25 km and a very strong cold bias of approximately 12 K at altitudes between 30 and 35 km.

Burris, John↗

AROTEL Temperature Retrievals Within PSC's Using Raman Scattering

NASA Goddard Space Flight Center's Airborne Raman Ozone Temperature Lidar (AROTEL) made temperature retrievals within Polar Stratospheric Clouds (PSCs) on several flights during the SAGE III Ozone Loss and Validation Experiment (SOLVE) campaign. The location of the PSCs was confirmed using simultaneously acquired data from the NASA Langley Aerosol lidar. Retrievals were made on flight dates 991207, 991210 and 000127 from just above the aircraft to 25 kilometers geometric altitude. Raman temperature retrievals are, to first order, insensitive to Mie interference because the Raman signals are red shifted by 2331 cm(exp -1) from the initial laser wavelength. Backscattering from clouds and aerosols is consequently not observed by the detector; however, extinction does impact the measurement and limits retrievals to optically thin clouds. Comparisons between retrievals employing Rayleigh and Raman scattering show the Raman temperatures to be significantly warmer than those employing Rayleigh scattering. Uncertainties are a function of altitude: at 25 km they were approximately 3 K. Temperature profiles could not be retrieved for optically thick clouds.

Burris, John↗