Mathematical efficiency calibration with uncertain source geometries using smart optimization
The In Situ Object Counting Software (ISOCS), a mathematical method developed by CANBERRA, is a well established technique for computing High Purity Germanium (HPGe) detector efficiencies for a wide variety of source shapes and sizes. In the ISOCS method, the user needs to input the geometry related parameters such as: the source dimensions, matrix composition and density, along with the source-to-detector distance. In many applications, the source dimensions, the matrix material and density may not be well known. Under such circumstances, the efficiencies may not be very accurate since the modeled source geometry may not be very representative of the measured geometry. CANBERRA developed an efficiency optimization software known as 'Advanced ISOCS' that varies the not well known parameters within user specified intervals and determines the optimal efficiency shape and magnitude based on available benchmarks in the measured spectra. The benchmarks could be results from isotopic codes such as MGAU, MGA, IGA, or FRAM, activities from multi-line nuclides, and multiple counts of the same item taken in different geometries (from the side, bottom, top etc). The efficiency optimization is carried out using either a random search based on standard probability distributions, or using numerical techniques that carry out a more directed (referred to as 'smart' in this paper) search. Measurements were carried out using representative source geometries and radionuclide distributions. The radionuclide activities were determined using the optimum efficiency and compared against the true activities. The 'Advanced ISOCS' method has many applications among which are: Safeguards, Decommissioning and Decontamination, Non-Destructive Assay systems and Nuclear reactor outages maintenance. (authors)