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Michael Lecours

Publications and source records attributed to Michael Lecours.

Antarctic polar stratospheric cloud composition as observed by ACE, CALIPSO and MIPAS

The composition of polar stratospheric clouds (PSCs) in the Antarctic is measured by infrared absorption spectroscopy by the Atmospheric Chemistry Experiment (ACE) satellite and compared to lidar (CALIPSO) and emission spectroscopy (MIPAS) results. ACE observations are compared first to CALIPSO for the period 2006–2020, then to MIPAS for the period 2005–2011, and then a set of triple coincidences is studied. In both CALIPSO-ACE and MIPAS-ACE comparisons, nitric acid trihydrate (NAT) detections are in excellent agreement (∼80 % of coincident compositions is found). Supercooled ternary solution (STS) detections are in good agreement for CALIPSO-ACE (∼60 %) but in poor agreement for MIPAS-ACE (39 %). This contrasts with ice detections, in poor agreement for CALIPSO-ACE (∼30 %) and in better agreement for MIPAS-ACE (45 %). Triple coincidences show that ACE STS detections are more reliable than MIPAS STS detections. The comparison between ACE observations and homogeneous CALIPSO PSCs shows that for 11 events, CALIPSO reports STS rather than supercooled nitric acid (SNA) clouds.

Atmospheric Chemistry Experiment↗

Comparison between ACE and CALIPSO observations of Antarctic polar stratospheric clouds

The depletion of stratospheric ozone is catalyzed by polar stratospheric clouds (PSCs) that form in the cold polar winter. The space-based lidar onboard CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) has been the reference instrument for measuring PSCs. Recently, the infrared transmission spectra recorded by the Fourier transform instrument on the ACE (Atmospheric Chemistry Experiment) satellite has provided measurements of PSC composition. We report on coincident observations made by the CALIPSO and the ACE satellites for three late winter periods (2016, 2018 and 2019) and evaluate CALIPSO's determination of PSC composition relative to ACE’s findings. We found that CALIPSO and ACE generally agree well for the detection of nitric acid trihydrate (NAT) clouds. However, CALIPSO detects some NAT clouds where ACE detects supercooled ternary solutions of nitric and sulfuric acid (STS). Similarly, CALIPSO only partially detects ice in ACE's ice clouds. Overall, these results seem to show that CALIPSO’s NAT classification might be too inclusive. We also found that supercooled nitric acid (SNA) clouds, a new classification, are labelled as STS by CALIPSO

Léo Lavy↗