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Munakata, Koji

Publications and source records attributed to Munakata, Koji.

In-plane multi-q magnetic ground state of Na 3 Co 2 SbO 6

We report Na 3 Co 2 SbO 6 is a potential Kitaev magnet with a monoclinic layered crystal structure. Recent investigations of the C3-symmetric sister compound Na 2 Co 2 TeO 6 have uncovered a unique triple-q magnetic ground state, as opposed to a single-q (zigzag) one, prompting us to examine the influence of the reduced structural symmetry of Na 3 Co 2 SbO 6 on its ground state. Neutron diffraction data obtained on a twin-free crystal reveal that the ground state remains a multi-q state, despite the system's strong non-C 3 -symmetric anisotropy. This robustness of multi-q orders suggests that they are driven by a common mechanism in the honeycomb cobaltates, such as interactions beyond the bilinear order. Spin-polarized neutron diffraction results show that the ordered moments are entirely in plane, with each staggered component orthogonal to the propagating wave vector. The inferred ground state appears more compatible with the so-called XXZ easy-plane anisotropy than the Kitaev anisotropy, and features unequal ordered moments reduced by strong quantum fluctuations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Oval-cycloidal Magnetic Structure with Phase-shift in the Non-centrosymmetric Tetragonal Compound CePdSi 3

CePdSi 3 with H // [100] exhibits multiple metamagnetic transitions. Since there is no frustration in this system, it is suggested that the origin of the multiple metamagnetic transitions is the influence of the antisymmetric spin–orbit interaction. To clarify the magnetic structure under the influence of the antisymmetric spin–orbit interaction, neutron diffraction experiments have been performed using single crystal samples of CePdSi3. There are observed magnetic reflections with incommensurate magnetic propagation vector q=(0.315,0,0) in the phase I. In addition, additional magnetic reflections were also observed in the phase III. The magnetic structure was found to be an oval-cycloidal structure at the phase III in CePdSi 3 , and we discuss the origin of the unusual magnetic structure.

36 MATERIALS SCIENCE↗