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Negres, R. A.

Publications and source records attributed to Negres, R. A..

Investigation of UV, ns-laser damage resistance of hafnia films produced by electron beam evaporation and ion beam sputtering deposition methods

Laser-induced damage in coating materials with a high index of refraction, such as hafnia, limits the performance of high power and high energy laser systems. Understanding the underlying physics responsible for laser damage holds the key for developing damage-resistant optical films. Previous studies have reported a substantial difference in laser damage onset for hafnia films produced by different deposition methods, yet the underlying mechanisms for the observed difference remain elusive. We combined laser damage testing with analytical characterizations and theoretical simulations to investigate the response of hafnia films produced by electron (e-) beam evaporation vs ion beam sputtering (IBS) methods upon UV ns-laser exposure. We found that e-beam produced hafnia films were overall more damage resistant; in addition, we observed a polarization anisotropy associated with the onset of damage in the e-beam films, while this effect was absent in the latter films. The observed differences can be attributed to the stark contrast in the pressure inside the pores inherent in both films. The high pressure inside the IBS-induced nanobubbles has been shown to reduce the threshold for laser-induced plasma breakdown leading to film damage. The polarization effects in the e-beam coatings can be related to the asymmetric electric field intensification induced by the columnar void structure. Our findings provide a fundamental basis for developing strategies to produce laser damage-resistant coatings for UV pulsed laser applications.

36 MATERIALS SCIENCE↗

Determination of the Raman polarizability tensor in the optically anisotropic crystal potassium dihydrogen phosphate and its deuterated analog

Abstract The Raman tensor of the dominant A 1 modes of the nonlinear optical crystalline material potassium dihydrogen phosphate and its 70% deuterated analog have been ascertained. Challenges in determining the A 1 mode tensor element values based on previous reports have been resolved using a specially designed experimental setup that makes use of spherical crystal samples. This novel experimental design enabled the determination of measurement artifacts, including polarization rotation of the pump and/or scattered light propagating through the sample and the contribution of additional overlapping phonon modes, which have hindered previous efforts. Results confirmed that the polarization tensor is diagonal, and matrix elements were determined with high accuracy.

36 MATERIALS SCIENCE↗

Mirrors for petawatt lasers: Design principles, limitations, and solutions

High intensity and high energy laser facilities place increasing demands on optical components, requiring large surface area optics with exacting specifications. Petawatt lasers are high energy, short-pulse laser systems generally based on chirped-pulse amplification, where an initial low energy short pulse is stretched, amplified, and then recompressed to produce fs to ps high-power laser pulses. In such petawatt lasers, the highest demands are placed on the final optics, including gratings which compress the pulses and mirrors which direct and focus the final high-power beams. The limiting factor in these optical components is generally laser-induced damage. Designing and fabricating these optical components to meet reflection, dispersion, and other requirements while meeting laser-induced damage requirements is the primary challenge discussed in this tutorial. We will introduce the reader to the technical challenges and tradeoffs required to produce mirrors for petawatt lasers and discuss current research directions.

47 OTHER INSTRUMENTATION↗