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Orbe, Clara

Publications and source records attributed to Orbe, Clara.

Lower-Stratospheric Tracer Trends and Variability from Reanalyses

Previous studies have robustly identified a decrease since 1998 in lower stratospheric ozone in the Northern Hemisphere (NH). While this ozone decrease is qualitatively explained as resulting from changes in the large-scale circulation, there is not yet a quantitative mechanistic explanation of these changes. Here we explore the drivers of recent ozone changes using two different configurations of the Goddard Earth Observing System (GEOS) general circulation model. The first configuration of GEOS includes a full chemistry module and is constrained with meteorological fields from the MERRA-2 reanalysis. This configuration (M2GMI) is used to analyze an idealized tracer that covaries closely with ozone on interannual and decadal timescales, revealing that recent ozone decreases in the NH subtropics are associated with a poleward expansion of upwelling in the NH LS, with reduced (enhanced) downwelling over northern subtropics (midlatitudes). The second configuration of GEOS is a free-running version of the GEOS Chemistry-Climate Model (CCM) that is used to perform a ten-member ensemble of free-running simulations. Comparisons of the two configurations reveal that, while the free-running model can produce negative ozone changes in the NH LS, the magnitude of these changes is significantly weaker, relative to both M2GMI and MERRA-2; moreover, these weaker ozone decreases are consistent with weaker simulated changes in the residual circulation. Finally, we examine the GEOS model results in the broader context of the hindcast simulations performed as part of Phase 1 of the Chemistry Climate Modeling Initiative. We show that the majority of the free-running simulations considered here also exhibit weaker long-term residual circulation changes, compared to reanalyses.

Wargan, Kris↗

Large-Scale Transport into the Arctic: The Roles of the Midlatitude Jet and the Hadley Cell

Transport from the Northern Hemisphere (NH) midlatitudes to the Arctic plays a crucial role in determining the abundance of trace gases and aerosols that are important to Arctic climate via impacts on radiation and chemistry. Here we examine this transport using an idealized tracer with a fixed lifetime and predominantly midlatitude land-based sources in models participating in the Chemistry Climate Model Initiative (CCMI). We show that there is a 25%-45% difference in the Arctic concentrations of this tracer among the models. This spread is correlated with the spread in the location of the Pacific jet, as well as the spread in the location of the Hadley Cell (HC) edge, which varies consistently with jet latitude. Our results suggest that it is likely that the HC-related zonal-mean meridional transport rather than the jet-related eddy mixing is the major contributor to the inter-model spread in the transport of land-based tracers into the Arctic. Specifically, in models with a more northern jet, the HC generally extends further north and the tracer source region is mostly covered by surface southward flow associated with the lower branch of the HC, resulting in less efficient transport poleward to the Arctic. During boreal summer, there are poleward biases in jet location in free-running models, and these models likely underestimate the rate of transport into the Arctic. Models using specified dynamics do not have biases in the jet location, but do have biases in the surface meridional flow, which may result in differences in transport into the Arctic. In addition to the land-based tracer, the midlatitude-to-Arctic transport is further examined by another idealized tracer with zonally uniform sources. With equal sources from both land and ocean, the inter-model spread of this zonally uniform tracer is more related to variations in parameterized convection over oceans rather than variations in HC extent, particularly during boreal winter. This suggests that transport of land-based and oceanic tracers or aerosols towards the Arctic differs in pathways and therefore their corresponding inter-model variabilities result from different physical processes.

chemistry climate models↗

Long-Term Ozone Variability and Trends from Reanalyses: Can It Be Done?

Stratospheric ozone concentrations have begun to show early signs of recovery following the implementation of the Montreal Protocol and its amendments as well as in response to decreasing upper-stratospheric temperatures. Secular trends in stratospheric ozone are modulated by considerable interannual variability and systematic changes in transport patterns that are expected under increasing concentrations of greenhouse gases, especially in the lower stratosphere. These factors necessitate the continued close monitoring of stratospheric ozone in upcoming decades, with a special focus on the lower stratosphere.As highly resolved data sets combining a plethora of observations with model simulations atmospheric reanalyses are, in principle, well suited for the task. All major reanalyses generate ozone output. However, significant spurious discontinuities that arise from step changes in the observing systems prevent a straightforward analysis of ozone trends and long-term variability. Building on our recent work, in this presentation we will demonstrate that trend detection is nonetheless possible using the ozone record from NASA's MERRA-2 (Modern-Era Retrospective Analysis for Research and Applications, Version 2) reanalysis bias-corrected using a chemistry model simulation as a transfer function. Next, we will outline several strategies to reduce artificial discontinuities in the ozone record in future NASA reanalyses. This discussion will be illustrated by an example of joint assimilation of bias-corrected ozone profiles from the Microwave Limb Sounder (MLS) on the Aura satellite (2004 to present) and the Ozone Mapping Profiler Suite Limb Profiler (OMPS-LP) sensors that are expected to operate on future NOAA platforms.

Wargan, Krzysztof↗

Multidecadal Changes in Lower Stratospheric Ozone: Variability Vs. Trends

As upper stratospheric ozone appears to be recovering as a result of decreasing chlorine loading following the implementation of the Montreal Protocol and its amendments and in agreement with model projections, several recent studies report an apparent decline of ozone concentrations in the lower stratosphere in the last two decades, particularly in the extratropics. Our previous work as well as at least two other studies provide evidence that this decline results from transport changes rather than an intensification of chemical depletion. It remains unclear whether these changes represent long-term internal variability or are a consequence of a climate forcing. Here we perform free-running ensembles of the recent past (1980-2016) using the Goddard Earth Observing System Model (GEOS) at the cubed sphere C180 (approximately half degree) resolution. Two suites of 10-member ensembles are performed, one in which observed sea surface temperature (SSTs) are fully prescribed, and the other in which the linear SST trend over the recent past is removed so as to only retain internal variability. We evaluate the trends in both ozone as well as two idealized tracers with prescribed uniform loss that are used to isolate the role of transport from chemistry and emissions. Probability-distribution-functions of the trends in both ozone and idealized tracers are compared among ensemble members and with observed trends in order to evaluate the likelihood of recent observed declines in lower stratospheric ozone, relative to large internal variability. Moreover, comparisons among simulations with and without imposed SST trends indicate the extent to which dynamically-driven ozone trends reflect forced trends or internal variability in lower stratospheric dynamics.

Wargan, Krzysztof↗

Overview of Large-scale Tropospheric Transport in the Chemistry Climate Model Initiative (CCMI) Simulations

The transport of chemicals is a major uncertainty in the modeling of tropospheric composition. Here we compare the large-scale tropospheric transport properties among different models in the Chemistry Climate Modeling Initiative (CCMI) with a focus on transport defined with respect to the Northern Hemisphere (NH) midlatitude surface. Among simulations of the recent past (1980-2010) we show that there are substantial differences in their global-scale tropospheric transport properties. For example, the mean transit time since southern hemisphere air last contacted the NH midlatitude surface differs by ~30-40% among simulations. We show that these differences are most likely associated with differences in parameterized convection over the oceans, such that the spread in transport among simulations constrained with analysis fields is as large as the spread among free-running simulations.

large-scale tropospheric transport↗

Air Quality Forecasts Using the NASA GEOS Model

We provide an introduction to a new high-resolution (0.25 degree) global composition forecast produced by NASA's Global Modeling and Assimilation office. The NASA Goddard Earth Observing System version 5 (GEOS-5) model has been expanded to provide global near-real-time forecasts of atmospheric composition at a horizontal resolution of 0.25 degrees (~25 km). Previously, this combination of detailed chemistry and resolution was only provided by regional models. This system combines the operational GEOS-5 weather forecasting model with the state-of-the-science GEOS-Chem chemistry module (version 11) to provide detailed chemical analysis of a wide range of air pollutants such as ozone, carbon monoxide, nitrogen oxides, and fine particulate matter (PM2.5).

Knowland, K. Emma↗

Large-Scale Tropospheric Transport in the Chemistry-Climate Model Initiative (CCMI) Simulations

Understanding and modeling the large-scale transport of trace gases and aerosols is important for interpreting past (and projecting future) changes in atmospheric composition. Here we show that there are large differences in the global-scale atmospheric transport properties among the models participating in the IGAC SPARC Chemistry–Climate Model Initiative (CCMI). Specifically, we find up to 40% differences in the transport timescales connecting the Northern Hemisphere (NH) midlatitude surface to the Arctic and to Southern Hemisphere high latitudes, where the mean age ranges between 1.7 and 2.6 years. We show that these differences are related to large differences in vertical transport among the simulations, in particular to differences in parameterized convection over the oceans. While stronger convection over NH midlatitudes is associated with slower transport to the Arctic, stronger convection in the tropics and subtropics is associated with faster interhemispheric transport. We also show that the differences among simulations constrained with fields derived from the same reanalysis products are as large as (and in some cases larger than) the differences among free-running simulations, most likely due to larger differences in parameterized convection. Our results indicate that care must be taken when using simulations constrained with analyzed winds to interpret the influence of meteorology on tropospheric composition.

Orbe, Clara↗

Recent Decline in Extratropical Lower Stratospheric Ozone Attributed to Circulation Changes

The 1998-2016 ozone trends in the lower stratosphere are examined using the Modern-Era Retrospective Analysis for Research and Applications Version 2 (MERRA-2) and related National Aeronautics and Space Administration products. After removing biases resulting from step changes in the MERRA-2 ozone observations, a discernible negative trend of 1.67 +/- 0.54 Dobson units per decade (DU/decade) is found in the 10-km layer above the tropopause between 20 deg N and 60 deg N. A weaker but statistically significant trend of 1.17 +/- 0.33 DU/decade exists between 50 deg S and 20 deg S. In the Tropics, a positive trend is seen in a 5-km layer above the tropopause. Analysis of an idealized tracer in a model simulation constrained by MERRA-2 meteorological fields provides strong evidence that these trends are driven by enhanced isentropic transport between the tropical (20 deg S-20 deg N) and extratropical lower stratosphere in the past two decades. This is the first time that a reanalysis data set has been used to detect and attribute trends in lower stratospheric ozone.

trend↗

Multidecadal Changes in the UTLS Ozone from the MERRA-2 Reanalysis and the GMI Chemistry Model

Long-term changes of ozone in the UTLS (Upper Troposphere / Lower Stratosphere) reflect the response to decreases in the stratospheric concentrations of ozone-depleting substances as well as changes in the stratospheric circulation induced by climate change. To date, studies of UTLS ozone changes and variability have relied mainly on satellite and in-situ observations as well as chemistry-climate model simulations. By comparison, the potential of reanalysis ozone data remains relatively untapped. This is despite evidence from recent studies, including detailed analyses conducted under SPARC (Scalable Processor Architecture) Reanalysis Intercomparison Project (S-RIP), that demonstrate that stratospheric ozone fields from modern atmospheric reanalyses exhibit good agreement with independent data while delineating issues related to inhomogeneities in the assimilated observations. In this presentation, we will explore the possibility of inferring long-term geographically and vertically resolved behavior of the lower stratospheric (LS) ozone from NASA's MERRA-2 (Modern-Era Retrospective Analysis for Research and Applications -2) reanalysis after accounting for the few known discontinuities and gaps in its assimilated input data. This work builds upon previous studies that have documented excellent agreement between MERRA-2 ozone and ozonesonde observations in the LS. Of particular importance is a relatively good vertical resolution of MERRA-2 allowing precise separation of tropospheric and stratospheric ozone contents. We also compare the MERRA-2 LS ozone results with the recently completed 37-year simulation produced using Goddard Earth Observing System in "replay" mode coupled with the GMI (Global Modeling Initiative) chemistry mechanism. Replay mode dynamically constrains the model with the MERRA-2 reanalysis winds, temperature, and pressure. We will emphasize the areas of agreement of the reanalysis and replay and interpret differences between them in the context of our increasing understanding of model transport driven by assimilated winds.

Ozone↗

Air Quality Forecasts Using the NASA GEOS Model

We provide an introduction to a new high-resolution (0.25 degree) global composition forecast produced by NASA's Global Modeling and Assimilation office. The NASA Goddard Earth Observing System version 5 (GEOS-5) model has been expanded to provide global near-real-time forecasts of atmospheric composition at a horizontal resolution of 0.25 degrees (~25 km). Previously, this combination of detailed chemistry and resolution was only provided by regional models. This system combines the operational GEOS-5 weather forecasting model with the state-of-the-science GEOS-Chem chemistry module (version 11) to provide detailed chemical analysis of a wide range of air pollutants such as ozone, carbon monoxide, nitrogen oxides, and fine particulate matter (PM2.5). The resolution of the forecasts is the highest resolution compared to current, publically-available global composition forecasts. Evaluation and validation of modeled trace gases and aerosols compared to surface and satellite observations will be presented for constituents relative to health air quality standards. Comparisons of modeled trace gases and aerosols against satellite observations show that the model produces realistic concentrations of atmospheric constituents in the free troposphere. Model comparisons against surface observations highlight the model's capability to capture the diurnal variability of air pollutants under a variety of meteorological conditions. The GEOS-5 composition forecasting system offers a new tool for scientists and the public health community, and is being developed jointly with several government and non-profit partners. Potential applications include air quality warnings, flight campaign planning and exposure studies using the archived analysis fields.

Keller, Christoph A.↗

Air Quality Forecasts Using the NASA GEOS Model: A Unified Tool from Local to Global Scales

We provide an introduction to a new high-resolution (0.25 degree) global composition forecast produced by NASA's Global Modeling and Assimilation office. The NASA Goddard Earth Observing System version 5 (GEOS-5) model has been expanded to provide global near-real-time forecasts of atmospheric composition at a horizontal resolution of 0.25 degrees (approximately 25 km). Previously, this combination of detailed chemistry and resolution was only provided by regional models. This system combines the operational GEOS-5 weather forecasting model with the state-of-the-science GEOS-Chem chemistry module (version 11) to provide detailed chemical analysis of a wide range of air pollutants such as ozone, carbon monoxide, nitrogen oxides, and fine particulate matter (PM2.5). The resolution of the forecasts is the highest resolution compared to current, publically-available global composition forecasts. Evaluation and validation of modeled trace gases and aerosols compared to surface and satellite observations will be presented for constituents relative to health air quality standards. Comparisons of modeled trace gases and aerosols against satellite observations show that the model produces realistic concentrations of atmospheric constituents in the free troposphere. Model comparisons against surface observations highlight the model's capability to capture the diurnal variability of air pollutants under a variety of meteorological conditions. The GEOS-5 composition forecasting system offers a new tool for scientists and the public health community, and is being developed jointly with several government and non-profit partners. Potential applications include air quality warnings, flight campaign planning and exposure studies using the archived analysis fields.

Knowland, E. Emma↗

Large-Scale Transport Responses to Tropospheric Circulation Changes Using GEOS-5

The mean age since air was last at the Northern Hemisphere midlatitude surface is a fundamental property of tropospheric transport. Recent comparisons among chemistry climate models, however, reveal that there are large differences in the mean age among models and that these differences are most likely related to differences in tropical (parameterized) convection. Here we use aquaplanet simulations of the Goddard Earth Observing System Model Version 5 (GEOS-5) to explore the sensitivity of the mean age to changes in the tropical circulation. Tropical circulation changes are forced by prescribed localized off-equatorial warm sea surface temperature anomalies that (qualitatively) reproduce the convection and circulation differences among the comprehensive models. Idealized chemical species subject to prescribed OH loss are also integrated in parallel in order to illustrate the impact of tropical transport changes on interhemispheric constituent transport.

Orbe, Clara↗

Multi-Model Impacts of Climate Change on Pollution Transport from Global Emission Source Regions

The impacts of climate change on tropospheric transport, diagnosed from a carbon monoxide (CO)-like tracer species emitted from global CO sources, are evaluated from an ensemble of four chemistry-climate model (CCMs) contributing to the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP). Model time-slice simulations for present-day and end of the 21st century conditions were performed under the Representative Concentrations Pathways (RCP) climate scenario RCP 8.5. All simulations reveal a strong seasonality in transport, especially over the tropics. The highest CO-tracer mixing ratios aloft occur during boreal winter when strong vertical transport is co-located with biomass burning emission source regions. A consistent and robust decrease in future CO-tracer mixing ratios throughout most of the troposphere, especially in the tropics, and an increase around the tropopause is found across the four CCMs in both winter and summer. Decreases in CO-tracer mixing ratios in the tropical troposphere are associated with reduced convective mass fluxes in this region, which in turn may reflect a weaker Hadley Cell circulation in the future climate. Increases in CO-tracer mixing ratios near the tropopause are largely attributable to a rise in tropopause height, although a poleward shift in the midlatitude jets may also play an important role in the extra-tropical upper troposphere. An increase in CO-tracer mixing ratios also occurs near the Equator, centred over EquatorialCentral Africa, extending from the surface to the mid troposphere which is most likely related to localised decreases in convection in the vicinity of the Intertropical Convergence Zone, resulting in larger CO-tracer mixing ratios over biomass burning regions and smaller mixing ratios downwind.

Tropospheric Transport↗

The Transit-Time Distribution from the Northern Hemisphere Midlatitude Surface

The distribution of transit times from the Northern Hemisphere (NH) midlatitude surface is a fundamental property of tropospheric transport. Here we present an analysis of the transit time distribution (TTD) since air last contacted the northern midlatitude surface layer, as simulated by the NASA Global Modeling Initiative Chemistry Transport Model. We find that throughout the troposphere the TTD is characterized by long flat tails that reflect the recirculation of old air from the Southern Hemisphere and results in mean ages that are significantly larger than the modal age. Key aspects of the TTD -- its mode, mean and spectral width -- are interpreted in terms of tropospheric dynamics, including seasonal shifts in the location and strength of tropical convection and variations in quasi-isentropic transport out of the northern midlatitude surface layer. Our results indicate that current diagnostics of tropospheric transport are insufficient for comparing model transport and that the full distribution of transit times is a more appropriate constraint.

model transport↗

Air Mass Origin in the Arctic and its Response to Future Warming

We present the first climatology of air mass origin in the Arctic in terms of rigorously defined air mass fractions that partition air according to where it last contacted the planetary boundary layer (PBL). Results from a present-day climate integration of the GEOSCCM general circulation model reveal that the Arctic lower troposphere below 700 mb is dominated year round by air whose last PBL contact occurred poleward of 60degN, (Arctic air, or air of Arctic origin). By comparison, approx. 63% of the Arctic troposphere above 700 mb originates in the NH midlatitude PBL, (midlatitude air). Although seasonal changes in the total fraction of midlatitude air are small, there are dramatic changes in where that air last contacted the PBL, especially above 700 mb. Specifically, during winter air in the Arctic originates preferentially over the oceans, approx. 26% in the East Pacific, and approx. 20% in the Atlantic PBL. By comparison, during summer air in the Arctic last contacted the midlatitude PBL primarily over land, overwhelmingly so in Asia (approx. 40 %) and, to a lesser extent, in North America (approx. 24%). Seasonal changes in air-mass origin are interpreted in terms of seasonal variations in the large-scale ventilation of the midlatitude boundary layer and lower troposphere, namely changes in the midlatitude tropospheric jet and associated transient eddies during winter and large scale convective motions over midlatitudes during summer.

tropospheric transport↗

Seasonal Ventilation of the Stratosphere: Robust Diagnostics from One-Way Flux Distributions

We present an analysis of the seasonally varying ventilation of the stratosphere using one-way flux distributions. Robust transport diagnostics are computed using GEOSCCM subject to fixed present-day climate forcings. From the one-way flux, we determine the mass of the stratosphere that is in transit since entry through the tropical tropopause to its exit back into the troposphere, partitioned according to stratospheric residence time and exit location. The seasonalities of all diagnostics are quantified with respect to the month of year (a) when air enters the stratosphere, (b) when the mass of the stratosphere is partitioned, and (c) when air exits back into the troposphere. We find that the return flux, within 3 months since entry, depends strongly on when entry occurred: (34 +/- 10)% more of the air entering the stratosphere in July leaves poleward of 45 deg N compared to air that enters in January. The month of year when the air mass is partitioned is also found to be important: The stratosphere contains about six times more air of tropical origin during late summer and early fall that will leave poleward of 45 deg within 6 months since entering the stratosphere compared to during late winter to late spring. When the entire mass of the air that entered the stratosphere at the tropics regardless of its residence time is considered, we find that (51 +/- 1)% and (39 +/- 2)% will leave poleward of 10 deg in the Northern Hemisphere (NH) and Southern Hemisphere (SH), respectively.

Stratosphere-Troposphere Exchange↗