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Pollack, I.

Publications and source records attributed to Pollack, I..

7 records
All sourcesNASA NTRSDOE OSTI
NASA NTRS2016

WRF-Chem Simulations of Lightning-NOx Production and Transport in Oklahoma and Colorado Thunderstorms Observed During DC3

The focus of this analysis is on lightning-generated nitrogen oxides (LNOx) and their distribution for two thunderstorms observed during the Deep Convective Clouds and Chemistry (DC3) field campaign in May-June 2012. The Weather Research and Forecasting Chemistry (WRF-Chem) model is used to perform cloud-resolved simulations for the May 29-30 Oklahoma severe convection, which contained one supercell, and the June 6-7 Colorado squall line. Aircraft and ground-based observations (e.g., trace gases, lightning and radar) collected during DC3 are used in comparisons against the model-simulated lightning flashes generated by the flash rate parameterization schemes (FRPSs) incorporated into the model, as well as the model-simulated LNOx predicted in the anvil outflow. Newly generated FRPSs based on DC3 radar observations and Lightning Mapping Array data are implemented in the model, along with previously developed schemes from the literature. The results of these analyses will also be compared between storms to investigate which FRPSs were most appropriate for the two types of convection and to examine the variation in the LNOx production. The simulated LNOx results from WRF-Chem will also be compared against other previously studied mid-latitude thunderstorms.

Lightning↗
NASA NTRS2015

Quantifying Sources and Sinks of Reactive Gases in the Lower Atmosphere Using Airborne Flux Observations

Atmospheric composition is governed by the interplay of emissions, chemistry, deposition, and transport. Substantial questions surround each of these processes, especially in forested environments with strong biogenic emissions. Utilizing aircraft observations acquired over a forest in the southeast U.S., we calculate eddy covariance fluxes for a suite of reactive gases and apply the synergistic information derived from this analysis to quantify emission and deposition fluxes, oxidant concentrations, aerosol uptake coefficients, and other key parameters. Evaluation of results against state-of-the-science models and parameterizations provides insight into our current understanding of this system and frames future observational priorities. As a near-direct measurement of fundamental process rates, airborne fluxes offer a new tool to improve biogenic and anthropogenic emissions inventories, photochemical mechanisms, and deposition parameterizations.

emission↗
NASA NTRS2015

A WRF-Chem Analysis of Flash Rates, Lightning-NOx Production and Subsequent Trace Gas Chemistry of the 29-30 May 2012 Convective Event in Oklahoma During DC3

The Deep Convective Clouds and Chemistry (DC3) field campaign in 2012 provided a plethora of aircraft and ground-based observations (e.g., trace gases, lightning and radar) to study deep convective storms, their convective transport of trace gases, and associated lightning occurrence and production of nitrogen oxides (NOx). This is a continuation of previous work, which compared lightning observations (Oklahoma Lightning Mapping Array and National Lightning Detection Network) with flashes generated by various flash rate parameterization schemes (FRPSs) from the literature in a Weather Research and Forecasting Chemistry (WRF-Chem) model simulation of the 29-30 May 2012 Oklahoma thunderstorm. Based on the Oklahoma radar observations and Lightning Mapping Array data, new FRPSs are being generated and incorporated into the model. The focus of this analysis is on estimating the amount of lightning-generated nitrogen oxides (LNOx) produced per flash in this storm through a series of model simulations using different production per flash assumptions and comparisons with DC3 aircraft anvil observations. The result of this analysis will be compared with previously studied mid-latitude storms. Additional model simulations are conducted to investigate the upper troposphere transport, distribution, and chemistry of the LNOx plume during the 24 hours following the convective event to investigate ozone production. These model-simulated mixing ratios are compared against the aircraft observations made on 30 May over the southern Appalachians.

Cummings, Kristin A.↗
NASA NTRS2014

A WRF-Chem Flash Rate Parameterization Scheme and LNOx Analysis of the 29-30 May 2012 Convective Event in Oklahoma During DC3

The Deep Convective Clouds and Chemistry (DC3) field campaign in 2012 provided a plethora of aircraft and ground-based observations (e.g., trace gases, lightning and radar) to study deep convective storms, their convective transport of trace gases, and associated lightning occurrence and production of nitrogen oxides (NOx). Based on the measurements taken of the 29-30 May 2012 Oklahoma thunderstorm, an analysis against a Weather Research and Forecasting Chemistry (WRF-Chem) model simulation of the same event at 3-km horizontal resolution was performed. One of the main objectives was to include various flash rate parameterization schemes (FRPSs) in the model and identify which scheme(s) best captured the flash rates observed by the National Lightning Detection Network (NLDN) and Oklahoma Lightning Mapping Array (LMA). The comparison indicates how well the schemes predicted the timing, location, and number of lightning flashes. The FRPSs implemented in the model were based on the simulated thunderstorms physical features, such as maximum vertical velocity, cloud top height, and updraft volume. Adjustment factors were applied to each FRPS to best capture the observed flash trend and a sensitivity study was performed to compare the range in model-simulated lightning-generated nitrogen oxides (LNOx) generated by each FRPS over the storms lifetime. Based on the best FRPS, model-simulated LNOx was compared against aircraft measured NOx. The trace gas analysis, along with the increased detail in the model specification of the vertical distribution of lightning flashes as suggested by the LMA data, provide guidance in determining the scenario of NO production per intracloud and cloud-to-ground flash that best matches the NOx mixing ratios observed by the aircraft.

Atmospheric chemistry↗
NASA NTRS2014

A Wrf-Chem Flash Rate Parameterization Scheme and LNO(x) Analysis of the 29-30 May 2012 Convective Event in Oklahoma During DC3

The Deep Convective Clouds and Chemistry (DC3) field campaign in 2012 provided a plethora of aircraft and ground-based observations (e.g., trace gases, lightning and radar) to study deep convective storms, their convective transport of trace gases, and associated lightning occurrence and production of nitrogen oxides (NOx). Based on the measurements taken of the 29-30 May 2012 Oklahoma thunderstorm, an analysis against a Weather Research and Forecasting Chemistry (WRF-Chem) model simulation of the same event at 3-km horizontal resolution was performed. One of the main objectives was to include various flash rate parameterization schemes (FRPSs) in the model and identify which scheme(s) best captured the flash rates observed by the National Lightning Detection Network (NLDN) and Oklahoma Lightning Mapping Array (LMA). The comparison indicates how well the schemes predicted the timing, location, and number of lightning flashes. The FRPSs implemented in the model were based on the simulated thunderstorms physical features, such as maximum vertical velocity, cloud top height, and updraft volume. Adjustment factors were added to each FRPS to best capture the observed flash trend and a sensitivity study was performed to compare the range in model-simulated lightning-generated nitrogen oxides (LNOx) generated by each FRPS over the storms lifetime. Based on the best FRPS, model-simulated LNOx was compared against aircraft measured NOx. The trace gas analysis, along with the increased detail in the model specification of the vertical distribution of lightning flashes as suggested by the LMA data, provide guidance in determining the scenario of NO production per intracloud and cloud-to-ground flash that best matches the NOx mixing ratios observed by the aircraft.

Cloud physics↗
NASA NTRS1968

Etching of aluminum for bonding Patent

Etching aluminum alloys with aqueous solution containing sulfuric acid, hydrofluoric acid, and an alkali metal dischromate for adhesive bonding

Emde, W. D.↗