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Read, W.

Publications and source records attributed to Read, W..

Assimilation of the Microwave Limb Sounder Radiances

It has been shown that the assimilation of limb-sounder data can significantly improve the representation of ozone in NASA's GEOS Data Assimilation Systems (GEOS-DAS), particularly in the stratosphere. The studies conducted so far utilized retrieved data from the MIPAS, POAM, ILAS and EOS Microwave Limb Sounder (EOS MLS) instruments. Direct assimilation of the radiance data can be seen as the natural next step to those studies. The motivation behind working with radiances is twofold. First, retrieval algorithms use a priori data which are either climatological or are obtained from previous analyses. This introduces additional uncertainty and, in some cases, may lead to "self-contamination"- when the a priori is taken from the same assimilation system in which subsequently ingests the retrieved observations. Second, radiances can be available in near real time thus providing an opportunity for operational assimilation, which could help improve the use of infrared radiance instruments from operational satellite instruments. In this presentation we summarize our ongoing work on an implementation of the assimilation of EOS MLS radiances into the GEOS-5 DAS. This work focuses on assimilation of band 7 brightness temperatures which are sensitive to ozone. Our implementation uses the MLS Callable Forward Model developed by the MLS team at NASA JPL as the observation operator. We will describe our approach and recent results which are not yet final. In particular, we will demonstrate that this approach has a potential to improve the vertical structure of ozone in the lower tropical stratosphere as compared with the retrieved MLS product. We will discuss the computational efficiency of this implementation.

Wargan, K.

Recent Advances in Ozone Data Assimilation at the GMAO - Towards a New Reanalysis

This presentation summarized ongoing work on improving the representation of ozone in the GEOS Data Assimilation Systems. Data from two EOS Aura sensors was used: the total column ozone from the Ozone Monitoring Instrument (OMI) and high vertical resolution stratospheric profiles from Microwave Limb Sounder (MLS, version 3.3). As several previous studies have demonstrated, assimilation of this data can constrain the stratospheric and tropospheric ozone columns with relatively good accuracy. However, the representation of the vertical structures in the troposphere and near tropopause region is often deficient. Since both these layers of the atmosphere are critical to the understanding of the radiative forcing as well as the ozone budget in the troposphere, current work will focus on improving the assimilated product between the surface and the 50 hPa pressure level. The discussion included recent steps that have been taken towards refining the treatment of ozone in GEOS-5. Impacts of improved tropospheric chemistry model were discussed including the introduction of efficiency factors ("averaging kernels") for OMI total ozone, and direct assimilation of radiances from the MLS instrument. In particular, advantages and challenges involved in assimilating limb radiances rather than retrieved product were discussed. This work is, in part, a preparation for a planned reanalysis of the EOS Aura data from 2005 to present.

Krzysztof, Wargan

Validation of MIPAS IMK-IAA Temperature, Water Vapor, and Ozone Profiles with MOHAVE-2009 Campaign Measurements

MIPAS observations of temperature, water vapor, and ozone in October 2009 as derived with the scientific level-2 processor run by Karlsruhe Institute of Technology (KIT), Institute for Meteorology and Climate Research (IMK) and CSIC, Instituto de Astrofısica de Andalucıa (IAA) and retrieved from version 4.67 level-1b data have been compared to co-located field campaign observations obtained during the MOHAVE-2009 campaign at the Table Mountain Facility near Pasadena, California in October 2009. The MIPAS measurements were validated regarding any potential biases of the profiles, and with respect to their precision estimates. The MOHAVE-2009 measurement campaign provided measurements of atmospheric profiles of temperature, water vapor/relative humidity, and ozone from the ground to the mesosphere by a suite of instruments including radiosondes, ozonesondes, frost point hygrometers, lidars, microwave radiometers and Fourier transform infrared (FTIR) spectrometers. For MIPAS temperatures (version V4O_T_204), no significant bias was detected in the middle stratosphere; between 22 km and the tropopause MIPAS temperatures were found to be biased low by up to 2 K, while below the tropopause, they were found to be too high by the same amount. These findings confirm earlier comparisons of MIPAS temperatures to ECMWF data which revealed similar differences. Above 12 km up to 45 km, MIPAS water vapor (version V4O_H2O_203) is well within 10% of the data of all correlative instruments. The well-known dry bias of MIPAS water vapor above 50 km due to neglect of non-LTE effects in the current retrievals has been confirmed. Some instruments indicate that MIPAS water vapor might be biased high by 20 to 40% around 10 km (or 5 km below the tropopause), but a consistent picture from all comparisons could not be derived. MIPAS ozone (version V4O_O3_202) has a high bias of up to +0.9 ppmv around 37 km which is due to a non-identified continuum like radiance contribution. No further significant biases have been detected. Cross-comparison to co-located observations of other satellite instruments (Aura/MLS, ACE-FTS, AIRS) is provided as well.

MIPAS validation

The Carbon Monoxide Tape Recorder

Using Aura MLS data we have identified the stratospheric tape recorder in carbon monoxide (CO). Unlike the water vapor tape recorder, which is controlled by upper troposphere processes, the CO tape recorder is linked to seasonal biomass burning. Since CO has a lifetime of only a few months, the CO tape recorder barely extends above 20 km. The tape head for CO appears to be close to 360K near the same location as the water vapor tape head [Read et al, 20041. Both tape heads are below the equatorial cold point tropopause but above the base of the tropical tropopause layer. The tape recorder signal becomes more distinct from 360K to 380K suggesting that convective detrainment of plays a decreasingly important role with altitude. The Global Modeling Initiative chemical transport model forced by the climatology of biomass burning reproduces the CO tape recorder.

Schoeberl, M. R.

Chemical Observations of a Polar Vortex Intrusion

An intrusion of vortex edge air in D the interior of the Arctic polar vortex was observed on the January 31,2005 flight of the NASA DC-8 aircraft. This intrusion was identified as anomalously high values of ozone by the AROTAL and DIAL lidars. Our analysis shows that this intrusion formed when a blocking feature near Iceland collapsed, allowing edge air to sweep into the vortex interior. along the DC-8 flight track also shows the intrusion in both ozone and HNO3. Polar Stratospheric Clouds (PSCs) were observed by the DIAL lidar on the DC-8. The spatial variability of the PSCs can be explained using MLS HNO3 and H2O observations and meteorological analysis temperatures. We also estimate vortex denitrification using the relationship between N2O and HNO3. Reverse domain fill back trajectory calculations are used to focus on the features in the MLS data. The trajectory results improve the agreement between lidar measured ozone and MLS ozone and also improve the agreement between the HNO3 measurements PSC locations. The back trajectory calculations allow us to compute the local denitrification rate and reduction of HCl within the filament. We estimate a denitrification rate of about lO%/day after exposure to below PSC formation temperature. Analysis of Aura MLS observations made

Schoeberl, M. R.

UARS Microwave Limb Sounder Observations of Upper Atmosphere Ozone and Chlorine Monoxide

UARS MLS observations of stratospheric ozone and chlorine monoxide are described. Enhanced concentrations of ClO, the predominant form of reactive chlorine responsible for ozone depletion, are seen within both the northern and southern winter polar vortices. In the southern hemisphere, this leads directly to the development of the annual Antarctic ozone hole. While ozone depletion is also observed in the north, it is less severe and there is considerable interannual variability.

stratosphere ozone chlorine monoxide Microwave Lim

Validation of UARS MLS C10 Measurements

This paper describes the validation of stratospheric C10 measurements by the MLS on the UARS. The comparisons done to date between MLS and other measurements of C10 indicate general agreement to within the estimated MLS uncertainties and the uncertainties of the comparative measurements.

Microwave Limb Sounder MLS

A 3D simulation of the early winter distribution of reactive chlorine in the north polar vortex

Early in December 1991, high values of ClO are seen by the Microwave Limb Sounder (MLS) on the Upper Atmosphere Research Satellite at latitudes south of areas of temperatures cold enough to form polar stratospheric clouds (PSCs). A 3D simulation shows that the heterogeneous conversion of chlorine reservoirs to reactive chlorine on the surfaces of PSCs (processing) takes place at high latitudes. Often the processed air must be transported to lower latitudes, where the reactive chlorine is photochemically converted to ClO, to be observed by MLS. In this simulation, one incidence of cold temperatures is associated with an anticyclone, and a second with a cyclone. The transport of processed air associated with the anticyclone is marked by shearing; a decrease in the maximum of the processed air is accompanied by growth of the area influenced by the processing. In contrast, the air processed in the cyclonic event spreads more slowly. This shows that transport and shearing is a crucial element to the evolution of reactive chlorine associated with a processing event. In particular, transport and shearing, as well as photochemical processes, can cause variations in observed ClO.

Douglass, A.

A Highly Accurate Voight Function Algorithm

A complex Voight lineshape algorithm is presented whose maximum relative error over the complex plane is less than 1 x 10 super minus 8. The algorithm consists of series, rational approximations and Gauss-Hermite integrations which makes it suitable as a general purpose software module for a wide variety of uses, including a Voight function standard.

Voight lineshape Doppler velocity distribution col