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Roback, R.

Publications and source records attributed to Roback, R..

Evaluation of Engineered Barrier Systems (FY19 Report)

This report describes research and development (R&D) activities conducted during fiscal year 2019 (FY19) specifically related to the Engineered Barrier System (EBS) R&D Work Package in the Spent Fuel and Waste Science and Technology (SFWST) Campaign supported by the United States (U.S.) Department of Eneregy (DOE). The R&D activities focus on understanding EBS component evolution and interactions within the EBS, as well as interactions between the host media and the EBS. A primary goal is to advance the development of process models that can be implemented directly within the Genreric Disposal System Analysis (GDSA) platform or that can contribute to the safety case in some manner such as building confidence, providing further insight into the processes being modeled, establishing better constraints on barrier performance, etc.The FY19 EBS activities involved not only modeling and analysis work, but experimental work as well. The report documents the FY19 progress made in seven different research areas as follows: (1) thermal analysis for the disposal of dual purpose canisters (DPCs) in sedimentary host rock using the semianalytical method, (2) tetravalent uranium solubility and speciation, (3) modeling of high temperature, thermal-hydrologic-mechanical-chemical (THMC) coupled processes, (4) integration of coupled thermalhydrologic- chemical (THC) model with GDSA using a Reduced-Order Model, (5) studying chemical controls on montmorillonite structure and swelling pressure, (6) transmission x-ray microscope for in-situ nanotomography of bentonite and shale, and (7) in-situ electrochemical testing of uranium dioxide under anoxic conditions. The R&D team consisted of subject matter experts from Sandia National Laboratories, Lawrence Berkeley National Laboratory (LBNL), Los Alamos National Laboratory (LANL), Pacific Northwest National Laboratory (PNNL), the Bureau de Recherches Géologiques et Minières (BRGM), the University of California Berkeley, and Mississippi State University. In addition, the EBS R&D work leverages international collaborations to ensure that the DOE program is active and abreast of the latest advances in nuclear waste disposal. For example, the FY19 work on modeling coupled THMC processes at high temperatures relied on the bentonite properties from the Full-scale Engineered Barrier EXperiment (FEBEX) Field Test conducted at the Grimsel Test Site in Switzerland. Overall, significant progress has been made in FY19 towards developing the modeling tools and experimental capabilities needed to investigate the performance of EBS materials and the associated interactions in the drift and the surrounding near-field environment under a variety of conditions including high temperature regimes.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Mass and momentum turbulent transport experiments with swirling confined coaxial jets. II

An experimental study of mixing downstream of swirling coaxial jets discharging into an expanded duct was conducted to obtain data for the evaluation and improvement of turbulent transport models currently used in a variety of computational procedures throughout the combustion community. A combination of laser velocimeter and laser induced fluorescence techniques was employed to obtain mean and fluctuating velocity and concentration distributions at selected axial and radial locations throughout the flow field. Flow visualization techniques were also employed to determine qualitatively the time dependent characteristics of the flow and the scale of turbulence. Simultaneous two component velocity and concentration/velocity measurements provided data which were used to determine the average momentum and mass transport rates for each of three measurement planes. Mixing for swirling flows occurred in several steps of axial and radial mean convective flow and was completed in one-third the length required for nonswirling flow. Comparison of the mass and momentum transport processes for swirling and nonswirling flows indicated that large differences existed in these processes between the two flows.

Roback, R.↗

Turbulent transport and length scale measurement experiments with comfined coaxial jets

A three phase experimental study of mixing downstream of swirling and nonswirling confined coaxial jets was conducted to obtain data for the evaluation and improvement of turbulent transport models currently employed in a variety of computational procedures. The present effort was directed toward the acquisition of length scale and dissipation rate data that provide more accurate inlet boundary conditions for the computational procedures and a data base to evaluate the turbulent transport models in the near jet region where recirculation does not occur, and the acquisition of mass and momentum turbulent transport data for a nonswirling flow condition with a blunt inner jet inlet configuration rather than the tapered inner jet inlet. A measurement technique, generally used to obtain approximate integral length and microscales of turbulence and dissipation rates, was computerized. Results showed the dissipation rate varied by 2 1/2 orders of magnitude across the inlet plane, by 2 orders of magnitude 51 mm from the inlet plane, and by 1 order of magnitude at 102 mm from the inlet plane for a nonswirling flow test conditions.

Johnson, B. V.↗

Mass and Momentum Turbulent Transport Experiments

An experimental study of mixing downstream of axial and swirling coaxial jets is being conducted to obtain data for the evaluation and improvement of turbulent transport models currently employed in a variety of computational procedures used throughout the propulsion community. Effort was directed toward the acquisition of length scale and dissipation rate data that will provide more accurate inlet boundary conditions for the computational procedures and a data base to evaluate the turbulent transport models in the near jet region where recirculation does not occur. Mass and momentum turbulent transport data with a blunt inner-jet inlet configuration will also be acquired.

Johnson, B. V.↗

Mass and momentum turbulent transport experiments with confined swirling coaxial jets. I

An experimental study of mixing downstream of swirling coaxial jets discharging into an expanded duct was conducted to obtain data for the evaluation and improvement of turbulent transport models currently used in a variety of computational procedures throughout the combustion community. A combination of laser velocimeter and laser induced fluorescence techniques was employed to obtain mean and fluctuating velocity and concentration distributions which were used to derive mass and momentum turbulent transport parameters currently incorporated into various combustor flow models. Flow visualization techniques were also employed to determine qualitatively the time dependent characteristics of the flow and the scale of turbulence. Mean and fluctuating velocity profiles and probability density functions were obtained at selected axial and radial locations throughout the flow field. Mixing occurred in several steps of axial and radial mass transport and was coupled with a large radial mean convective flux. Major mixing regions were observed to occur (1) at the interface between the inner stream and the centerline recirculation zone, and (2) at the interface between the inner jet and the annular jet streams. Mixing for swirling flow was completed in one-third the length required for nonswirling flow.

Johnson, B. V.↗

Mass and Momentum Transport Experiments with Swirling Flow

An experimental study of mixing downstream of axial and swirling coaxial jets is being conducted to obtain data for the evaluation and improvement of turbulent transport models currently employed in a variety of computational procedures used throughout the propulsion community. The axial coaxial jet study was completed under Phase 1. The swirling coaxial jet study, which is the subject of this paper, was conducted under Phase 2 of the contract. A TEACH code was acquired, checked out for several test cases, and is reported. A study to measure length scales and to obtain a limited number of measurements with a blunt trailing edge inlet is being conducted under Phase 3 of the contract.

Johnson, B. V.↗

Scalar and momentum turbulent transport experiments with swirling and nonswirling flows

Combustor models for the aircraft gas turbine industry have been obtained because of the need to reduce the costs of developing improved performance and more durable engines. A few years ago, it became apparent that the mass concentration and velocity predictions provided by the computer codes were not representing the data measured in some confined recirculating flows. It is pointed out that errors in the mass concentration distribution are an especially serious problem because of their influence on the heat release, temperature, and reactant distributions. Combined mass and momentum turbulent transport experiments with swirling and nonswirling flow have been conducted with the objective to obtain an experimental data base which can be used to evaluate and improve the turbulent transport submodes employed in the aerothermal models. The present paper is mainly concerned with the overall characteristics of the mass turbulent transport processes in complex flows with recirculation and the deficiencies of the conventional models.

Johnson, B. V.↗

Mass and momentum turbulent transport experiments with confined swirling coaxial jets

Swirling coaxial jets mixing downstream, discharging into an expanded duct was conducted to obtain data for the evaluation and improvement of turbulent transport models currently used in a variety of computational procedures throughout the combustion community. A combination of laser velocimeter (LV) and laser induced fluorescence (LIF) techniques was employed to obtain mean and fluctuating velocity and concentration distributions which were used to derive mass and momentum turbulent transport parameters currently incorporated into various combustor flow models. Flow visualization techniques were also employed to determine qualitatively the time dependent characteristics of the flow and the scale of turbulence. The results of these measurements indicated that the largest momentum turbulent transport was in the r-z plane. Peak momentum turbulent transport rates were approximately the same as those for the nonswirling flow condition. The mass turbulent transport process for swirling flow was complicated. Mixing occurred in several steps of axial and radial mass transport and was coupled with a large radial mean convective flux. Mixing for swirling flow was completed in one-third the length required for nonswirling flow.

Roback, R.↗

Deposit formation in hydrocarbon fuels

The hydrocarbon fuels RP-1, commercial-grade propane, JP-7 and chemically pure propane were subjected to tests in a high pressure fuel coking apparatus in order to evaluate their thermal decomposition limits and carbon deposition rates in heated copper tubes. A fuel thermal stability parametric evaluation was conducted at 136-340 atmospheres, bulk fuel velocities of 6-30 m/sec, and tube wall temperatures of 422-811 K, and the effect of inside wall material on deposit formation was evaluated in tests using nickel-plated tubes. Results show RP-1 deposit formation at wall temperatures between 600 and 800 K, with peak deposit formation near 700 K. Substitution of deoxygenated JP-7 for RP-1 showed no improvement, and the carbon deposition rates for propane fuels were found to be higher than those of either of the kerosene fuels. Nickel plating of the tube walls significantly reduced RP-1 carbon deposition rates.

Roback, R.↗

Deposit formation in hydrocarbon rocket fuels: Executive summary

An experimental program was conducted to study deposit formation in hydrocarbon fuels under flow conditions that exist in high-pressure, rocket engine cooling systems. A high pressure fuel coking test apparatus was designed and developed and was used to evaluate thermal decomposition (coking) limits and carbon deposition rates in heated copper tubes for two hydrocarbon rocket fuels, RP-1 and commercial-grade propane. Tests were also conducted using JP-7 and chemically-pure propane as being representative of more refined cuts of the baseline fuels. A parametric evaluation of fuel thermal stability was performed at pressures of 136 atm to 340 atm, bulk fuel velocities in the range 6 to 30 m/sec, and tube wall temperatures in the range 422 to 811K. In addition, the effect of the inside wall material on deposit formation was evaluated in selected tests which were conducted using nickel-plated tubes. The results of the tests indicated that substantial deposit formation occurs with RP-1 fuel at wall temperatures between 600 and 800K, with peak deposit formation occurring near 700K. No improvements were obtained when de-oxygenated JP-7 fuel was substituted for RP-1. The carbon deposition rates for the propane fuels were generally higher than those obtained for either of the kerosene fuels at any given wall temperature. There appeared to be little difference between commercial-grade and chemically-pure propane with regard to type and quantity of deposit. The results of tests conducted with RP-1 indicated that the rate of deposit formation increased slightly with pressure over the range 136 atm to 340 atm. Finally, plating the inside wall of the tubes with nickel was found to significantly reduce carbon deposition rates for RP-1 fuel.

Roback, R.↗

Deposit formation in hydrocarbon rocket fuels

An experimental program was conducted to study deposit formation in hydrocarbon fuels under flow conditions that exist in high-pressure, rocket engine cooling systems. A high pressure fuel coking test apparatus was designed and developed and was used to evaluate thermal decomposition (coking) limits and carbon deposition rates in heated copper tubes for two hydrocarbon rocket fuels, RP-1 and commercial-grade propane. Tests were also conducted using JP-7 and chemically-pure propane as being representative of more refined cuts of the baseline fuels. A parametric evaluation of fuel thermal stability was performed at pressures of 136 atm to 340 atm, bulk fuel velocities in the range 6 to 30 m/sec, and tube wall temperatures in the range 422 to 811 K. Results indicated that substantial deposit formation occurs with RP-1 fuel at wall temperatures between 600 and 800 K, with peak deposit formation occurring near 700 K. No improvements were obtained when deoxygenated JP-7 fuel was substituted for RP-1. The carbon deposition rates for the propane fuels were generally higher than those obtained for either of the kerosene fuels at any given wall temperature. There appeared to be little difference between commercial-grade and chemically-pure propane with regard to type and quantity of deposit. Results of tests conducted with RP-1 indicated that the rate of deposit formation increased slightly with pressure over the range 136 atm to 340 atm. Finally, lating the inside wall of the tubes with nickel was found to significantly reduce carbon deposition rates for RP-1 fuel.

Roback, R.↗